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We used resonant inelastic x-ray scattering to reveal the nature of magnetic interactions in Sr2IrO4, a 5d transition-metal oxide with a spin-orbit entangled ground state and Jeff=1/2 magnetic momemts, referred to as 'isospins'. The magnon…

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

强关联电子 · 物理学 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

We report magnetic susceptibility, specific heat, and Raman scattering investigations of alpha-TeVO4 containing V-O edge-sharing chains. These chains promote a system of ferromagnetic/antiferromagnetic spin-1/2 Heisenberg alternating…

Using Raman spectroscopy to study the correlated 4$d$-electron metal Sr$_2$RhO$_4$, we observe pronounced excitations at 220 meV and 240 meV with $A_\mathrm{1g}$ and $B_\mathrm{1g}$ symmetries, respectively. We identify them as transitions…

In the high spin-orbit coupled Sr2IrO4, the high sensitivity of the ground state to the details of the local lattice structure shows a large potential for the manipulation of the functional properties by inducing local lattice distortions.…

We report a Cu $K$-edge resonant inelastic x-ray scattering (RIXS) study of spin excitations in the $S$=1/2 antiferromagnetic chain system Sr$_2$CuO$_3$. The spectral weight observed below the charge-transfer gap appears in two-spinon…

强关联电子 · 物理学 2025-10-31 Kenji Ishii , Kenji Tsutsui , Takayuki Kawamata , Yoji Koike

The Raman scattering spectra from magnetic excitations in an antiferromagnetic spin-1/2 two leg ladder is investigated for weak and strong interladder coupling. In the first case, a cusp in the Raman intensityis obtained at a frequency…

强关联电子 · 物理学 2007-05-23 E. Orignac , R. Citro

We determine how the elementary excitations of iridium-oxide materials, which are dominated by a strong relativistic spin-orbit coupling, appear in Resonant Inelastic X-ray Scattering (RIXS). Whereas the RIXS spectral weight at the L2 x-ray…

强关联电子 · 物理学 2012-12-03 Luuk J. P. Ament , Giniyat Khaliullin , Jeroen van den Brink

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

强关联电子 · 物理学 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

强关联电子 · 物理学 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

强关联电子 · 物理学 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

High-resolution resonant inelastic X-ray scattering (RIXS) at the oxygen K-edge has been used to study the orbital excitations of Ca2RuO4 and Sr2RuO4. In combination with linear dichroism X-ray absorption spectroscopy, the ruthenium…

The magnetic excitations of the quasi-2D spin-1/2 Heisenberg antiferromagnet on an anisotropic triangular lattice Cs2CuCl4 are explored throughout the 2D Brillouin zone using inelastic neutron scattering. In the spin liquid phase above the…

强关联电子 · 物理学 2009-09-29 R. Coldea , D. A. Tennant , Z. Tylczynski

Using inelastic neutron scattering, we show that the onset of superconductivity in underdoped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ coincides with a crossover from well-defined spin waves to overdamped and diffusive spin excitations. This…

A major focus of experimental interest in Sr2IrO4 has been to clarify how the magnetic excitations of this strongly spin-orbit coupled system differ from the predictions of anisotropic 2D spin-1/2 Heisenberg model and to explore the extent…

强关联电子 · 物理学 2016-01-18 Y. Gim , A. Sethi , Q. Zhao , J. F. Mitchell , G. Cao , S. L. Cooper

We study coherent light scattering from linear crystals with up to twelve $^{40}\text{Ca}^+$ ions, acting as single photon emitters. Light-scattering is induced by two-photon laser excitation, starting from the S$_{1/2}\rightarrow$…

Spin-orbit interaction in Sr$_2$IrO$_4$ leads to the realization of the $J_{\mathrm{eff}}$ = 1/2 state and also induces an insulating behavior. Using large-shift Raman spectroscopy, we found two high-energy excitations of the d-shell…

强关联电子 · 物理学 2015-07-15 Jhih-An Yang , Yi-Ping Huang , Michael Hermele , Tongfei Qi , Gang Cao , Dmitry Reznik

Resonant inelastic x-ray scattering (RIXS) is an evolving tool for investigating spin dynamics of strongly correlated materials, which complements inelastic neutron scattering. Both techniques have found that non-spin-conserving (NSC)…

Motivated by recent interest in quasi-one-dimensional compound CaV2O4, we study the ground states of a spin-orbital chain characterized by an Ising-like orbital Hamiltonian and frustrated interactions between S=1 spins. The on-site…

强关联电子 · 物理学 2010-07-13 Gia-Wei Chern , Natalia Perkins

We report high-resolution inelastic neutron scattering measurements of the excitation spectrum in large single crystals of the spin-1/2 triangular lattice Ising-like antiferromagnet Na2BaCo(PO4)2 in magnetic fields applied transverse to the…

强关联电子 · 物理学 2025-09-16 Leonie Woodland , Ryutaro Okuma , J. Ross Stewart , Christian Balz , Radu Coldea
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