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Using first principles calculations, we study the microscopic origin of ferroelectricity (FE) induced by magnetic order in the orthorhombic HoMnO3. We obtain the largest ferroelectric polarization observed in the whole class of improper…

材料科学 · 物理学 2009-11-13 Silvia Picozzi , Kunihiko Yamauchi , Biplab Sanyal , Ivan A. Sergienko , Elbio Dagotto

The ferroelectricity of multiferroics induced by spin order is commonly explained by considering either purely electronic or ion-displacement contribution. However, there is no general model which includes both effects simultaneously. Here,…

强关联电子 · 物理学 2014-10-01 H. J. Xiang , P. S. Wang , M. -H. Whangbo , X. G. Gong

Ferroelectricity has been found to occur in several insulating systems, such as TbMnO$_3$ (TMO) and Ni$_3$V$_2$O$_8$ (NVO) which have more than one phase with incommensurately modulated long-range magnetic order. Here we give a…

材料科学 · 物理学 2009-11-11 A. Brooks Harris

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

Simultaneous breaking of time reversal and inversion symmetries in multiferroics couples ferroelectricity to magnetism and is a source of unusual physical phenomena that can be used in next-generation electronic devices. A notable example…

Multiferroic TbMnO3 is investigated using x-ray diffraction in high magnetic fields. Measurements on first and second harmonic structural reflections due to modulations induced by the Mn and Tb magnetic order are presented as function of…

Orthorhombic HoMnO3 is a multiferroic in which Mn antiferromagnetic order induces ferroelectricity. A second transition occurs within the multiferroic phase, in which a strong enhancement of the ferroelectric polarization occurs…

强关联电子 · 物理学 2021-01-04 Y. W. Windsor , M. Ramakrishnan , L. Rettig , A. Alberca , T. Lippert , C. W. Schneider , U. Staub

Multiferroic rare earth manganites attracted recent attention because of the coexistence of different types of magnetic and ferroelectric orders resulting in complex phase diagrams and a wealth of physical phenomena. The coupling and mutual…

强关联电子 · 物理学 2007-05-23 B. Lorenz , C. R. dela Cruz , F. Yen , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Multiferroics, showing simultaneous ordering of electrical and magnetic degrees of freedom, are remarkable materials as seen from both the academic and technological points of view. A prominent mechanism of multiferroicity is the…

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

材料科学 · 物理学 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

Ferroelectric and ferromagnetic materials possess spontaneous electric and magnetic order, respectively, which can be switched by the corresponding applied electric and magnetic fields. Multiferroics combine these properties in a single…

Multiferroics, where two or more ferroic order parameters coexist, is one of the hottest fields in condensed matter physics and materials science[1-9]. However, the coexistence of magnetism and conventional ferroelectricity is physically…

材料科学 · 物理学 2016-03-11 Xiangang Wan , Hang-Chen Ding , Sergey Y. Savrasov , Chun-Gang Duan

Within the broad class of multiferroics (compounds showing a coexistence of magnetism and ferroelectricity), we focus on the subclass of "improper electronic ferroelectrics", i.e. correlated materials where electronic degrees of freedom…

材料科学 · 物理学 2012-07-26 Silvia Picozzi , Alessandro Stroppa

An effective model is developed to explain the phase diagram and the mechanism of magnetoelectric coupling in multiferroics, $RMn_2O_5$. We show that the nature of magnetoelectric coupling in $RMn_2O_5$ is a coupling between two Ising-type…

强关联电子 · 物理学 2009-11-13 Chen Fang , Jiangping Hu

The ground state structural, electronic and magnetic properties of multiferroic TbMn$_2$O$_5$ are investigated via first-principles calculations. We show that the ferroelectricity in TbMn$_2$O$_5$ is driven by the non-centrosymmetric…

材料科学 · 物理学 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

Neutron diffraction, magnetic susceptibility, specific heat, and dielectric constant measurements of single crystal Co3TeO6 have been measured to study the interplay between the ferroelectricity and magnetic order. Long range incommensurate…

It is still under intensive discussion, how magnetoelectric coupling actually occurs at the atomic scale in multiferroic BiFeO3. Nuclear solid-state techniques monitor local fields at the atomic scale. Using such an approach, we show that,…

Single-crystal synchrotron x-ray diffraction measurements in strong magnetic fields have been performed for magnetoelectric compounds GdMnO3 and TbMnO3. It has been found that the P || a ferroelectric phase induced by the application of a…

强关联电子 · 物理学 2007-05-23 T. Arima , T. Goto , Y. Yamasaki , S. Miyasaka , K. Ishii , M. Tsubota , T. Inami , Y. Murakami , Y. Tokura

We investigate the crystal structure in multiferroic tetragonal perovskite Sr$_{1/2}$Ba$_{1/2}$MnO$_3$ with high accuracy of the order of 10$^{-3}$ Angstrom for an atomic displacement. The large atomic displacement for Mn ion from the…

材料科学 · 物理学 2020-07-15 D. Okuyama , K. Yamauchi , H. Sakai , Y. Taguchi , Y. Tokura , K. Sugimoto , T. J. Sato , T. Oguchi

We present a unique example of giant magnetoelectric effect in a conventional multiferroic HoMnO3, where polarization is very large (~56 mC/m2) and the ferroelectric transition temperature is higher than the magnetic ordering temperature by…

强关联电子 · 物理学 2015-05-13 N. Hur , I. K. Jeong , M. F. Hundley , S. B. Kim , S. -W. Cheong
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