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Attosecond physics enables the study of ultrafast coherent electron dynamics in matter upon photoexcitation and photoionization, revealing spectacular effects such as hole migration and coherent Auger dynamics in molecules. In the…

原子物理 · 物理学 2024-01-15 Marco Ruberti , Vitali Averbukh , Florian Mintert

As a step toward the full \emph{ab-initio} description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the \emph{ab initio}…

原子物理 · 物理学 2023-08-02 Siddhartha Chattopadhyay , Carlos Marante , Barry Schneider , Luca Argenti

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

原子物理 · 物理学 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…

We scrutinize the behavior of eigenvalues of an electron of Helium atom as it interacts with electric field directed along $z$-axis and exposed to linearly polarized intense laser field radiation. In order to achieve this, we freeze one…

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

化学物理 · 物理学 2010-12-10 Norio Takemoto , Andreas Becker

Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…

原子物理 · 物理学 2007-12-11 P. Johnsson , J. Mauritsson , T. Remetter , A. LHuillier , K. J. Schafer

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

原子物理 · 物理学 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

We present numerical simulations of ultrafast multiphoton ionization dynamics in a two-dimensional atomic model driven by co- and counterrotating circularly polarized single-color and bichromatic carrier envelope phase (CEP) stable…

原子物理 · 物理学 2020-07-15 T. Bayer , Ch. Philipp , K. Eickhoff , M. Wollenhaupt

The dissociative ionization of H2+ interacting with intense, femtosecond extreme-ultraviolet laser pulses is investigated theoretically. This is done by numerical propagation of the time-dependent Schr\"{o}dinger equation for a colinear…

原子物理 · 物理学 2015-02-25 Lun Yue , Lars Bojer Madsen

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

原子物理 · 物理学 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…

We calculate the photo-ionization cross-section from the ground state of the helium atom, using the complex rotation method and diagonalization of sparse matrices. This produces directly the positions and widths of the doubly excited 1Po…

chao-dyn · 物理学 2009-10-31 Benoit Gremaud , Dominique Delande

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime…

原子物理 · 物理学 2010-01-19 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

We study theoretically the photoabsorption spectra of an attosecond XUV pulse by a laserdressed atomic system. A weak XUV excites an autoionizing state which is strongly coupled to another autoionizing state by a laser. The theory was…

原子物理 · 物理学 2012-05-23 Wei-Chun Chu , C. D. Lin

Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…

原子物理 · 物理学 2021-06-30 Saad Mehmood , Eva Lindroth , Luca Argenti

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

原子物理 · 物理学 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen