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An analytical expression for the transfer integral HAB between the localized magnetic orbitals in superexchange-coupled dimers as a function of the type of atoms and geometry of the molecule has been derived by explicitly including orbital…

强关联电子 · 物理学 2013-07-02 S. Lebernegg , G. Amthauer , M. Grodzicki

Two perovskite-derived materials, CaCu3Mn4O12 and CaCu3Ti4O12, have drawn much recent interest due to their magnetoresistive, dielectric, and magnetoelectronic characteristics. Here we present initial theoretical insights into each of these…

材料科学 · 物理学 2007-05-23 M. D. Johannes , W. E. Pickett , R. Weht

Magnetization dynamics, which determine the speed of magnetization switching and spin information propagation, play a central role in modern spintronics. Gaining its control will satisfy the different needs of various spintronic devices. In…

材料科学 · 物理学 2024-01-29 Antarjami Sahoo , Haifeng Ding , Antonio Azevedo , Subhankar Bedanta

We study exchange couplings in the organic magnets copper(II) phthalocyanine (Cu(II)Pc) and manganese(II) phthalocyanine (Mn(II)Pc) by a combination of Green's function perturbation theory and \textsl{ab initio} density-functional theory…

材料科学 · 物理学 2009-11-13 Wei Wu , A. Kerridge , A. H. Harker , A. J. Fisher

We present magnetotransport calculations for homogeneous two-dimensional electron systems including the Rashba spin-orbit interaction, which mixes the spin-eigenstates and leads to a modified fan-chart with crossing Landau levels. The…

介观与纳米尺度物理 · 物理学 2016-08-16 M. Langenbuch , M. Suhrke , U. Rössler

In a recent paper by Schmitt et al. (arXiv:1402.1091), signs of two exchange interactions of one-dimensional alternating chains in distorted honeycomb systems of Na3Cu2SbO6 and Na2Cu2TeO6 are argued by theoretical calculations. Although the…

强关联电子 · 物理学 2014-02-28 Masatoshi Sato , Yoshiaki Kobayashi

Recently using Scanning Josephson Tunneling Microscopy (SJTM) in the group of S\'eamus Davis a super-modulation of the superconducting order parameter induced by super-modulation of the distance $\delta$ between planar Cu and apical O was…

超导电性 · 物理学 2026-03-16 Albert M. Varonov , Todor M. Mishonov

We investigated the magnetic properties of the system CuTe2O5 by susceptibility and electron spin resonance measurements. The anisotropy of the effective g-factors and the ESR linewidth indicates that the anticipated structural dimer does…

In this paper, we have focused on a comparison of the different magnetic properties of the three nano-Heusler Ru$_2$Mn$_X$ (X = Nb, Ta or V) compounds using the Blume-Capel Ising model. The Heusler structures are composed by different mixed…

软凝聚态物质 · 物理学 2021-09-07 N. Saber , Z. Fadil , A. Mhirech , B. Kabouchi , L. Bahmad , W. Ousi Benomar

Magnetic susceptibility and microscopic magnetic model of the mineral clinoclase Cu3(AsO4)(OH)3 are reported. This material can be well described as a combination of two nonequivalent spin dimers with the sizable magnetic couplings of J…

强关联电子 · 物理学 2013-07-02 Stefan Lebernegg , Alexander A. Tsirlin , Oleg Janson , Helge Rosner

Periodic and cluster density-functional theory (DFT) calculations, including DFT+U and hybrid functionals, are applied to study magnetostructural correlations in spin-1/2 frustrated chain compounds CuX2: CuCl2, CuBr2, and a fictitious chain…

强关联电子 · 物理学 2013-07-02 S. Lebernegg , M. Schmitt , A. A. Tsirlin , O. Janson , H. Rosner

The spin-1/2 alternating Heisenberg chain system Na$_3$Cu$_2$SbO$_6$ features two relevant exchange couplings: $J_{1a}$ within the structural Cu$_2$O$_6$ dimers and $J_{1b}$ between the dimers. Motivated by the controversially discussed…

强关联电子 · 物理学 2014-11-13 M. Schmitt , O. Janson , S. Golbs , M. Schmidt , W. Schnelle , J. Richter , H. Rosner

A combined theoretical and experimental study of the natural Cu(2+)-mineral callaghanite is presented. Its crystal structure features well separated Cu$_2$(OH)$_6$ structural dimers with weakly bonded carbonate groups and water molecules in…

强关联电子 · 物理学 2014-04-23 Stefan Lebernegg , Alexander A. Tsirlin , Oleg Janson , Helge Rosner

We investigate the properties of CuVOF$_4$(H$_2$O)$_6$$\cdot$H$_2$O, in which two different spin species, Cu(II) and V(IV), form antiferromagnetic spin-1/2 dimers with weak interdimer coupling provided via hydrogen bonding. Using…

A microscopic magnetic model for alpha-Cu2P2O7 is evaluated in a combined theoretical and experimental study. Despite a dominant intradimer coupling J1, sizable interdimer couplings enforce long-range magnetic ordering at T_N=27 K. The spin…

强关联电子 · 物理学 2011-04-05 O. Janson , A. A. Tsirlin , J. Sichelschmidt , Y. Skourski , F. Weickert , H. Rosner

Structural, electronic and magnetic properties of polycrystalline La2-xCaxCoMnO6 (0 $\leq$ x $\leq$ 0.75) compounds are investigated by x-ray diffraction and magnetometry. All the samples have an orthorhombic structure and show a slight…

材料科学 · 物理学 2022-05-11 J. R. Jesus , L. Bufaiçal , E. M. Bittar

Less common ligand coordination of transition-metal centers is often associated with peculiar valence-shell electron configurations and outstanding physical properties. One example is the Fe$^+$ ion with linear coordination, actively…

强关联电子 · 物理学 2020-11-20 R. Murugesan , M. S. Eldeeb , M. Yehia , B. Büchner , V. Kataev , O. Janson , L. Hozoi

A microscopic magnetic model for the spin-1/2 Heisenberg chain compound CuSe2O5 is developed based on the results of a joint experimental and theoretical study. Magnetic susceptibility and specific heat data give evidence for quasi-1D…

强关联电子 · 物理学 2009-11-20 O. Janson , W. Schnelle , M. Schmidt , Yu. Prots , S. -L. Drechsler , S. K. Filatov , H. Rosner

We use synchrotron x-ray diffraction and electrical transport under pressure to probe both the magnetism and the structure of single crystal NiS2 across its Mott-Hubbard transition. In the insulator, the low-temperature antiferromagnetic…

强关联电子 · 物理学 2011-09-02 Yejun Feng , R. Jaramillo , A. Banerjee , J. M. Honig , T. F. Rosenbaum

Theoretical prediction of the 2nd-order magnetic transition temperature (TM) used to be arduous. Here, we develop a first principle-based, fully automatic structure-to-TM method for two-dimensional (2D) magnets whose effective Hamiltonians…

材料科学 · 物理学 2023-12-08 Haichang Lu , Tai Yang , Zhimei Sun , John Robertson , Weisheng Zhao
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