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We study the surface plasmon (SP) resonance energy of isolated spherical Ag nanoparticles dispersed on a silicon nitride substrate in the diameter range 3.5-26 nm with monochromated electron energy-loss spectroscopy. A significant blueshift…

Electron energy loss spectroscopy (EELS) can be used to probe plasmon excitations in nanostructured materials with atomic-scale spatial resolution. For structures smaller than a few nanometers quantum effects are expected to be important,…

介观与纳米尺度物理 · 物理学 2013-01-03 Kirsten Andersen , Karsten W. Jacobsen , Kristian S. Thygesen

We investigate surface plasmon modes supported by flat-top silver nano-ridges. We calculate the mode electromagnetic field distribution, the dispersion curve, the travel range, and the figure-of-merit of the nano-ridge mode. We find that…

光学 · 物理学 2015-03-13 Zeyu Pan , Junpeng Guo , Richard Soref , Walter Buchwald , Greg Sun

Electron microscopy techniques such as electron energy-loss spectroscopy (EELS) facilitate the spatio-spectral characterization of plasmonic nanostructures. In this work, a time-dependent perspective is presented, which significantly…

Cathodoluminescence spectroscopy has been performed on silver nanoparticles in a scanning electron microscopy setup. Peaks appearing in the visible range for particles fabricated on silicon substrate are shown to arrive from excitation of…

光学 · 物理学 2009-06-08 Pratik Chaturvedi , Keng Hsu , Anil Kumar , James C. Mabon , Nicholas Fang

Raza et al. recently observed the extraordinarily large energy blueshifts of localized surface plasmon resonances and additional surface plasmon resonances in silver nanoparticles encapsulated in silicon nitride, which are not fully…

介观与纳米尺度物理 · 物理学 2021-05-19 Guozhong Wang

In electron energy-loss spectroscopy (EELS) of individual silver nanoparticles encapsulated in silicon nitride, we observe besides the usual dipole resonance an additional surface plasmon (SP) resonance corresponding to higher angular…

We theoretically investigated electron energy loss spectroscopy (EELS) of ultraviolet surface plasmon modes in aluminum nanodisks. Using full-wave simulations, we studied the impact of diameter on the resonant modes of the nanodisks. We…

光学 · 物理学 2023-07-19 Yujia Yang , Richard G. Hobbs , Phillip D. Keathley , Karl K. Berggren

Electromagnetic theory predicts that the optimal value of the localized plasmon resonance (LPR) wavelength for the maximal SERS enhancement factor (EF) is half the sum of the laser and Raman wavelengths. For small Raman shifts, the…

Nano-composite films of Tin Sulfide (SnS) and silver (Ag) fabricated by thermal evaporation showed two prominent peaks in the visible region of their extinction spectra. Theoretical modeling of the extinction spectra suggest that these two…

材料科学 · 物理学 2015-06-19 Priyal Jain , P. Arun

A new type of excitations by highly focused electron beams in scanning transmission electron microscopes is predicted for nanoparticles. The calculated electron energy loss spectra of metallic (silver) and insulating (SiO(sub2))…

材料科学 · 物理学 2011-11-09 M. A. Itskovsky , H. Cohen , T. Maniv

In this paper we discuss the field enhancement due to surface plasmons resonances of metallic nanostructures, in particular nano spheres on top of a metal, and find maximum field enhancement of the order of 10^2, intensities enhancement of…

介观与纳米尺度物理 · 物理学 2012-12-06 Nicolas Garcia , Ming Bai

Tightly confined plasmon waveguide modes supported by semicircular cross section top silver nanoridges are investigated in this paper. Mode field profiles, dispersion curves, propagation distances, confinement factors, and figure-of-merits…

光学 · 物理学 2015-06-05 Junpeng Guo , Zeyu Pan

Noble metal nanoparticles have been utilized for a vast amount of optical applications. For the applications that used metal nanoparticles as nanosensors and optical labeling, larger radiation damping is preferred (higher optical signal).…

光学 · 物理学 2022-03-02 Yanhe Yang , Weihai Ni , Hao Xie , Jian You , Weixiang Ye

We report on a combined far- and near-field study of surface plasmon polaritons on freestanding perforated gold films. The samples are fabricated by focused ion beam milling of {a periodic hole array into} a carbon membrane followed by…

材料科学 · 物理学 2021-03-10 M. Prämassing , T. Kiel , S. Irsen , K. Busch , S. Linden

Electron energy loss spectra have been measured on hexagonal boron nitride single crystals employing a novel electron energy loss spectroscopic set-up composed by an electron microscope equipped with a monochromator and an in-column filter.…

Plasmonic nanoparticles influence the absorption and emission processes of nearby emitters due to local enhancements of the illuminating radiation and the photonic density of states. Here, we use the plasmon resonance of metal nanoparticles…

We investigate surface plasmons from a solid-state standpoint and highlight their ultra electron density sensitivity. When a surface plasmon is excited on a planar gold film by an evanescent wave from 625 nm incident light, only a minute…

光学 · 物理学 2023-07-12 Wei Liu , Meng Li , Yu Niu , Ziren Luo

For distances less 10 nm, a total energy transfer occurs from a quantum emitter to a nearby metallic surface, producing evanescent surface waves that are plasmonic in nature. When investigating a metallic nanohole supported on an optically…

光学 · 物理学 2019-07-16 Amir Djalalian-Assl

This study examines the Raman scattering and charge transfer properties of molecules adsorbed on the surface of a tetrahedral Au$_{120}$ nanoparticle based on the time-dependent density functional tight-binding (TD-DFTB) method. We study…

化学物理 · 物理学 2024-09-18 Sajal Kumar Giri , George C. Schatz
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