相关论文: Molecular photodissociation
The 248nm and 193nm photodissociation of submonolayer quantities of CH$_3$Br and CH$_3$I adsorbed on thin layers of n-hexane indicate that the dissociation is caused by dissociative electron attachment from sub-vacuum level photoelectrons…
We present the results of a new calculation for the photodisintegration of ultra-high energy cosmic ray nuclei on soft photon targets. We include all the relevant photodisintegraton processes i.e giant dipole resonance, quasi-deuteron,…
Negative ions have been detected in abundance in recent years by spacecraft across the solar system. These detections were, however, made by instruments not designed for this purpose and, as such, significant uncertainties remain regarding…
We measure the absolute absorption cross section of molecules using a matter-wave interferometer. A nanostructured density distribution is imprinted onto a dilute molecular beam through quantum interference. As the beam crosses the light…
Water is an important molecule in interstellar and circumstellar environments. Previous observations of mid-infrared rotational lines of OH suggest that these lines may be used to probe the photodissociation of water. In this work, cross…
Context. Molecular Clouds (MCs) are the place where stars are formed and their feedback starts to take place, regulating the evolution of galaxies. Therefore, MCs represent the critical scale at which to study how ultra-violet (UV) photons…
Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…
We study the effects of the ionizing and dissociating photons produced by PopIII objects on the surrounding intergalactic medium. We find that the typical size of a H_2 photodissociated region, R_d ~ 1-5 kpc, is smaller than the mean…
It is well-known that water in both liquid and vapor phases exhibits exceptionally weak absorption of light in the visible range. Recent experiments, however, have demonstrated that at the liquid-air interface, absorption in the visible…
Photodissociation Region (PDR) models are computed over a wide range of physical conditions, from those appropriate to giant molecular clouds illuminated by the interstellar radiation field to the conditions experienced by circumstellar…
Quantum interference between multiple pathways in molecular photodissociation often results in angular momentum polarization of atomic products and this can give deep insight into fundamental physical processes. For dissociation of diatomic…
Most exoplanets detected so far have atmospheric T significantly higher than 300K. Often close to their star, they receive an intense UV photons flux that triggers important photodissociation processes. The T dependency of VUV absorption…
We discuss the interstellar absorption from many atomic and molecular species seen in high-resolution $HST$/STIS UV and high-S/N optical spectra of the moderately reddened B3-5~V star HD~62542. This remarkable sight line exhibits both very…
Non-thermal desorption from icy grains containing H$_2$CO has been invoked to explain the observed H$_2$CO gas phase abundances in ProtoPlanetary Disks (PPDs) and Photon Dominated Regions (PDRs). Photodesorption is thought to play a key…
Diffusion of atoms and molecules is a key process for the chemical evolution in the star forming regions of the interstellar medium. Accurate data on the mobility of many important interstellar species is however often not available and…
Photoevaporation is thought to play an important role in the early planetary evolution. In this study, we investigate the diffusion limit of X-ray and ultraviolet induced photoevaporation in primordial atmospheres. We find that…
We calculate the rate of precession of the direction of polarization of a photon traversing a sea of plane-polarized photons moving in the opposed direction, where the interaction is the one-loop "vacuum" Heisenberg-Euler coupling of four…
We investigate the importance of the shielding of chemical photorates by molecular hydrogen photodissociation lines and the carbon photoionization continuum deep within models of photon dominated regions. In particular, the…
Collapse and fragmentation of primordial filamentary clouds under isotropic dissociation radiation is investigated with one-dimensional hydrodynamical calculations. We investigate the effect of dissociation photon on the filamentary clouds…
The requirement of high space-time resolution and brightness is a great challenge for imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright tabletop laser, x-ray and electron sources have enabled the…