相关论文: Interplay between coherence and decoherence in LHC…
We show that the quantum coherent transfer of excitations between biomolecular chromophores is strongly influenced by spatial correlations of the environmental fluctuations. The latter are due either to propagating environmental modes or to…
Inspired by the works of [F. Caruso, New J. Phys. 16, 055015 (2014)] and [T. Scholak et al, J. Phys. B: At. Mol. Opt. Phys. 44 184012 (2011)], which state that for a large class of complex noisy networks, the optimal efficiency of quantum…
The coupling of excitons with atomic vibrations plays a pivotal role on the nonequilibrium optical properties of layered semiconductors. However, addressing the dynamical interaction between excitons and phonons represents a hard task both…
Recent observations of beating signals in the excitation energy transfer dynamics of photosynthetic complexes have been interpreted as evidence for sustained coherences that are sufficiently long-lived for energy transport and coherence to…
Large scale simulations of light-matter interaction in natural photosynthetic antenna complexes containing more than one hundred thousands chlorophyll molecules, comparable with natural size, have been performed. Photosynthetic antenna…
We report an investigation to establish the physical mechanisms responsible for decoherence in the generation of photon pairs from atomic ensembles, via the protocol of Duan et. al for long distance quantum communication [Nature (London)…
This paper discusses the combined effects of optical excitation power, interface roughness, lattice temperature, and applied magnetic fields on the spin-coherence of excitonic states in GaAs/AlGaAs multiple quantum wells. For low optical…
In this paper we consider the essential electronic excited states in parallel chains of semiconducting polymers that are currently being explored for photovoltaic and light-emitting diode applications. In particular, we focus upon various…
We explore the mechanism for the long-lived quantum coherence by considering the discrete phonon modes: these vibrational modes effectively weaken the exciton-environment interaction, due to the new composite (polaron) formed by excitons…
Time-resolved spectroscopy provides the main tool for analyzing the dynamics of excitonic energy transfer in light-harvesting complexes. To infer time-scales and effective coupling parameters from experimental data requires to develop…
In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…
Entanglement between a quantum system and its environment leads to loss of coherence in the former. In general, the temporal fate of coherences is complicated. Here, we establish the connection between decoherence of a central system and…
We explore an instantaneous decoherence correction (IDC) approach for the decoherence and energy relaxation in the quantum-classical dynamics of charge transport in organic semiconducting crystals. These effects, originating from…
Photosynthesis is a highly efficient process, nearly 100 percent of the red photons falling on the surface of leaves reach the reaction center and get transformed into energy. Most theoretical studies on photosynthetic complexes focus…
In monolayer transition metal dichalcogenide semiconductors, valley coherence degrades rapidly due to a combination of fast scattering and inter-valley exchange interaction. This leads to a sub-picosecond valley coherence time, making…
We analyze the many-particle correlations that affect the optical properties of two-dimensional semiconductors. These correlations manifest themselves through the specific optical resonances such as excitons, trions, etc. Starting from the…
The reflectionless coherent light transport in the coupled resonator array is investigated in the presence of intra-resonator intermodal coupling between the clockwise and counterclockwise modes, which plays a constructive role for…
The exciton dissociation and charge separation occurring on subpicosecond time scales following the photoexcitation are studied in a model donor/acceptor heterojunction using a fully quantum approach. Higher-than-LUMO acceptor orbitals…
We show that the biomolecular exciton dynamics under the influence of slow polarization fluctuations in the solvent cannot be described by approaches which are perturbative in the system-bath coupling. For this, we compare results for the…
In the strong exciton-cavity coupling regime, exciton polaritons play a pivotal role in governing exciton transport. However, the specific contributions of the two branches of polaritons to exciton current remain unexplored. Here, we…