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A core-softened model of a glass forming fluid is numerically studied in the limit of very low temperatures. The model shows two qualitatively different behaviors depending on the strength of the attraction between particles. For no or low…

统计力学 · 物理学 2009-11-07 E. A. Jagla

This paper is the fifth in a series exploring the physical consequences of the solidity of glass-forming liquids. Paper IV proposed a model where the density field is described by a time-dependent Ginzburg-Landau equation of the…

软凝聚态物质 · 物理学 2009-11-13 Jeppe C. Dyre

We use the isoconfigurational (IC) ensemble to show the connection between emerging heterogeneities in the tetrahedral order parameter and the dynamic propensity in a mildly undercooled glass-forming liquid. We observe that spatially…

软凝聚态物质 · 物理学 2021-01-18 M Shajahan G Razul , Gurpreet S Matharoo , Balakrishnan Viswanathan

We investigate the connection between local structure and dynamical heterogeneity in supercooled liquids. Through the study of four different models we show that the correlation between a particle's mobility and the degree of local order in…

统计力学 · 物理学 2014-10-20 Glen M. Hocky , Daniele Coslovich , Atsushi Ikeda , David R. Reichman

The glassy dynamics in confluent epithelial monolayers is crucial for several biological processes, such as wound healing, embryogenesis, cancer progression, etc. Several experiments have indicated that, unlike particulate systems, the…

软凝聚态物质 · 物理学 2024-07-24 Satyam Pandey , Soumitra Kolya , Padmashree Devendran , Souvik Sadhukhan , Tamal Das , Saroj Kumar Nandi

We use a standard Monte-Carlo algorithm to study the slow dynamics of a binary Lennard-Jones glass-forming mixture at low temperature. We find that Monte-Carlo is by far the most efficient way to simulate a stochastic dynamics since…

统计力学 · 物理学 2015-06-25 Ludovic Berthier , Walter Kob

Enormous enhancement in the viscosity of a liquid near its glass transition is generally connected to the growing many-body static correlations near the transition, often coined as `amorphous ordering'. Estimating the length scales of such…

We examined dynamic heterogeneity in a model tetrahedral network glass-forming liquid. We used four-point correlation functions to extract dynamic correlation lengths xi_4^a(t) and susceptibilities chi_4^a(t) corresponding to structural…

软凝聚态物质 · 物理学 2016-01-20 Hannah Staley , Elijah Flenner , Grzegorz Szamel

It has been a long-standing materials science challenge to establish structure-property relations in amorphous solids. Here we introduce a rotation-variant local structure representation that enables different predictions for different…

材料科学 · 物理学 2022-03-15 Zhao Fan , Evan Ma

We study colloidal particle dynamics of a model glass system using confocal and fluorescence microscopy as the sample evolves from a hard-sphere glass to a liquid with attractive interparticle interactions. The transition from hard-sphere…

软凝聚态物质 · 物理学 2015-05-13 Andrzej Latka , Yilong Han , Ahmed M. Alsayed , Andrew B. Schofield , A. G. Yodh , Piotr Habdas

Koperwas {\it et al.} showed in a recent paper, Phys. Rev. Lett. {\bf 111}, 125701 (2013), that the dynamic susceptibility $\chi_4$ as estimated by dielectric measurements for certain glass-forming liquids decreases substantially with…

统计力学 · 物理学 2014-10-29 Nicholas P. Bailey , Thomas B. Schrøder , Jeppe C. Dyre

Identifying the conditions under which glass formation occurs is crucial for a fundamental understanding of the glass transition mechanism. Pure liquids devoid of any frustration avoid glass transition and undergo crystallization. In this…

软凝聚态物质 · 物理学 2026-03-04 Saumya Suvarna , Prabhat K. Jaiswal , Madhu Priya

We study the relation between short-time vibrational modes and long-time relaxational dynamics in a kinetically constrained lattice gas with harmonic interactions between neighbouring particles. We find a correlation between the location of…

统计力学 · 物理学 2014-03-14 Douglas J. Ashton , Juan P. Garrahan

Glasses obtained from vapor deposition on a cold substrate have superior thermodynamic and kinetic stability with respect to ordinary glasses. Here we perform molecular dynamics simulations of vapor deposition of a model glass-former and…

软凝聚态物质 · 物理学 2023-05-24 Fabio Leoni , Fausto Martelli , C. Patrick Royall , John Russo

Recent work has demonstrated the strong qualitative differences between the dynamics near a glass transition driven by short-ranged repulsion and one governed by short-ranged attraction. Here, we study in detail the behavior of non-linear,…

统计力学 · 物理学 2010-04-16 P. Charbonneau , D. R. Reichman

Dynamics that are microscopic in space and time, in which particles commit to a position, so-called excitations, are considered the elementary unit of relaxation in the Dynamic Facilitation (DF) theory of the glass transition. Meanwhile,…

软凝聚态物质 · 物理学 2024-09-13 Danqi Lang , Camille Scalliet , C. Patrick Royall

We study the influence of the softness of the interparticle interactions on the fragility of a glass former, by considering three model binary mixture glass formers. The interaction potential between particles is a modified Lennard-Jones…

无序系统与神经网络 · 物理学 2012-06-19 Shiladitya Sengupta , Filipe Vasconcelos , Frédéric Affouard , Srikanth Sastry

The mechanism of hydrodynamics-induced pairing of soft particles, namely closed bilayer membranes (vesicles, a model system for red blood cells) and drops, is studied numerically with a special attention paid to the role of the confinement…

The elusive connection between dynamics and local structure in supercooled liquids is an important piece of the puzzle in the unsolved problem of the glass transition. The Johari-Goldstein beta relaxation, ubiquitous in glass-forming…

软凝聚态物质 · 物理学 2017-03-08 D. Fragiadakis , C. M. Roland

The interrelations between short range structural and elastic aspects in glasses and glass forming liquids pose important and yet unresolved questions. In this paper these relations are analyzed for mono-atomic glasses and stressed liquids…

无序系统与神经网络 · 物理学 2009-10-31 Tamar Kustanovich , Zeev Olami
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