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The effect of increased electron-density (from adsorbed Li atoms) in polyacenes and in nano-ribbons with zig-zag edge is discussed in terms of resonance theoretical considerations and in terms edge-localized frontier molecular orbitals. The…

化学物理 · 物理学 2025-11-10 Yenni P. Ortiz , Douglas J. Klein , Thomas H. Seligman

We have studied the small scale distribution of atomic hydrogen (HI) using 21-cm absorption spectra against multiple-component background radio continuum sources from the 21-SPONGE survey and the Millennium Arecibo Absorption Line Survey.…

The recent discovery of H3S and LaH10 superconductors with record high superconducting transition temperatures, Tc, at high pressure, has fueled the search for room-temperature superconductivity in the compressed superhydrides. Here we…

The density of states (DOS) of graphene underneath a metal is estimated through a quantum capacitance measurement of the metal/graphene/SiO2/n+-Si contact structure fabricated by a resist-free metal deposition process. Graphene underneath…

材料科学 · 物理学 2013-07-22 Ryota Ifuku , Kosuke Nagashio , Tomonori Nishimura , Akira Toriumi

This study employs density functional theory (DFT) and density functional tight-binding theory (DFTB) to determine the adsorption properties of carbon dioxide (CO$_2$), methane (CH$_4$), and dihydrogen (H$_2$) in carbophenes functionalized…

With a view towards optimizing gas storage and separation in crystalline and disordered nanoporous carbon-based materials, we use ab initio density functional theory calculations to explore the effect of chemical functionalization on gas…

Knowledge of the atomic geometry of a surface is a prerequisite for any detailed understanding of the surface's electronic structure and chemical properties. Previous studies have convincingly demonstrated that density functional theory…

材料科学 · 物理学 2007-05-23 C. Stampfl , M. Scheffler

The dipole force components in nano-sized metal hydrides are quantitatively determined with curvature and x-ray diffraction measurements. Ab-initio density functional theory is used to calculate the dipole components and the symmetry of the…

介观与纳米尺度物理 · 物理学 2016-05-30 Gunnar K. Pálsson , Moritz Wälde , Martin Amft , Yuanyuan Wu , Martina Ahlberg , Max Wolff , Astrid Pundt , Björgvin Hjörvarsson

The kinetics of hydrogen diffusion in C15 cubic and C14 hexagonal TiCr$_2$H$_x$ (0 < $x$ <= 4) Laves-phase hydrogen storage alloys is investigated with density functional theory (DFT) and machine learning interatomic potentials (MLIPs).…

材料科学 · 物理学 2026-02-26 Pranav Kumar , Fritz Körmann , Kaveh Edalati , Blazej Grabowski , Yuji Ikeda

The effect of solute hydrogen on the stability of vacancy clusters in hexagonal closed packed zirconium is investigated with an ab initio approach, including contributions of H vibrations. Atomistic simulations within the density functional…

材料科学 · 物理学 2015-09-29 Céline Varvenne , Olivier Mackain , Laurent Proville , Emmanuel Clouet

The high critical superconducting temperatures ($T_c$s) of metal hydride phases with clathrate-like hydrogen networks have generated great interest. Herein, we employ the Density Functional Theory-Chemical Pressure (DFT-CP) method to…

超导电性 · 物理学 2022-05-25 Katerina P. Hilleke , Eva Zurek

In this work, the most stable structures of Pt5V clusters are investigated using the successive growth algorithm (SCG) in conjunction with density functional theory (DFT) calculations. The resulting structures are evaluated by various…

材料科学 · 物理学 2024-08-08 P. L. Rodríguez-Kessler

Graphene monolayer grown by Si evaporation from the 0001 surface of SiC displays a moir\'e pattern of corrugation whose structure is ambiguous: different measurements and theoretical studies show either protruding bumps surrounded by…

介观与纳米尺度物理 · 物理学 2018-04-27 Tommaso Cavallucci , Valentina Tozzini

Alkali metal atoms (Li, Na, K, Rb, Cs), dimers and (2$\times$2) monolayers on a graphite (0001) surface have been studied using density functional theory, pseudopotentials, and a periodic substrate. The adatoms bind at the hollow site…

材料科学 · 物理学 2009-11-11 K. Rytkönen , J. Akola , M. Manninen

First-principles plane wave calculations predict that Li can be adsorbed on graphene forming a uniform and stable coverage on both sides. A significant part of the electronic charge of the Li-$2s$ orbital is donated to graphene and is…

介观与纳米尺度物理 · 物理学 2009-11-13 C. Ataca , E. Akturk , S. Ciraci , H. Ustunel

Several dissociated and two non-dissociated adsorption structures of the phenol molecule on the Si(001)-(2 \times 1) surface are studied using density functional theory with various exchange and correlation functionals. The relaxed…

计算物理 · 物理学 2015-05-19 Karen Johnston , Andris Gulans , Tuukka Verho , Martti J. Puska

Due to the presence of strong static correlation effects and noncovalent interactions, accurate prediction of the electronic and hydrogen storage properties of Li-adsorbed acenes with n linearly fused benzene rings (n = 3 - 8) has been very…

化学物理 · 物理学 2016-09-12 Sonai Seenithurai , Jeng-Da Chai

We use our theory of periodized discrete elasticity to characterize defects in graphene as the cores of dislocations or groups of dislocations. Earlier numerical implementations of the theory predicted some of the simpler defect groupings…

介观与纳米尺度物理 · 物理学 2012-07-30 L. L. Bonilla , A. Carpio

Metallenes are atomically thin two-dimensional (2D) materials lacking a layered structure in the bulk form. They can be stabilized by nanoscale constrictions like pores in 2D covalent templates, but the isotropic metallic bonding makes…

材料科学 · 物理学 2024-11-11 Kameyab Raza Abidi , Pekka Koskinen

The recent discovery of graphene has sparked significant interest, which has so far been focused on the peculiar electronic structure of this material, in which charge carriers mimic massless relativistic particle. However, the structure of…

介观与纳米尺度物理 · 物理学 2007-05-23 Jannik C. Meyer , A. K. Geim , M. I. Katsnelson , K. S. Novoselov , T. J. Booth , S. Roth