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We demonstrate that in a single molecule magnet (SMM) strongly coupled to electrodes the Kondo effect involves all magnetic excitations. This Kondo effect is induced by the quantum tunneling of the magnetic moment (QTM). Importantly, the…

强关联电子 · 物理学 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

We consider transport through a single-molecule magnet strongly coupled to metallic electrodes. We demonstrate that for half-integer spin of the molecule electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling of the…

强关联电子 · 物理学 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

We study the interplay of the Kondo effect and spin-polarized tunneling in a class of systems exhibiting uniaxial magnetic anisotropy, such as magnetic molecules, magnetic adatoms, or quantum dots coupled to a single localized magnetic…

介观与纳米尺度物理 · 物理学 2012-06-06 Maciej Misiorny , Ireneusz Weymann , Jozef Barnas

Spin-polarized transport through bistable magnetic adatoms or single-molecule magnets (SMMs), which exhibit both uniaxial and transverse magnetic anisotropy, is considered theoretically. The main focus is on the impact of transverse…

介观与纳米尺度物理 · 物理学 2014-07-22 Maciej Misiorny , Józef Barnaś

We analyze the electronic transport through a model spin-1 molecule as a function of temperature, magnetic field and bias voltage. We consider the effect of magnetic anisotropy, which can be generated experimentally by stretching the…

强关联电子 · 物理学 2011-06-24 P. S. Cornaglia , P. Roura Bas , A. A. Aligia , C. A. Balseiro

Quantum spin tunneling (QST) and Kondo effect are two very different quantum phenomena that produce the same effect on quantized spins, namely, the quenching of their magnetization. However, the nature of this quenching is very different so…

介观与纳米尺度物理 · 物理学 2016-10-05 D. Jacob , J. Fernández-Rossier

Non-equilibrium spin transport through an interacting quantum dot is analyzed. The coherent spin oscillations in the dot provide a generating source for spin current. In the interacting regime, the Kondo effect is influenced in a…

介观与纳米尺度物理 · 物理学 2007-05-23 Ping Zhang , Qi-Kun Xue , X. C. Xie

Transport properties in the Kondo regime of a nanosystem displaying uniaxial magnetic anisotropy (such as a magnetic molecule, magnetic adatom or quantum dot coupled to a localized magnetic moment) are analyzed theoretically. In particular,…

介观与纳米尺度物理 · 物理学 2012-06-06 Maciej Misiorny , Ireneusz Weymann , Jozef Barnas

We theoretically analyze the spectrum of a magnetic molecule when its charge and spin can couple to the molecular vibrations. More specifically, we show that the interplay between charge-vibron and spin-vibron coupling leads to a…

介观与纳米尺度物理 · 物理学 2018-07-04 Ahmed Kenawy , Janine Splettstoesser , Maciej Misiorny

We present a careful and thorough microscopic derivation of the Kondo Hamiltonian for single-molecule magnets (SMMs) transistors. When the molecule is strongly coupled to metallic leads, we show that by applying a transverse magnetic field…

强关联电子 · 物理学 2009-11-13 Gabriel Gonzalez , Michael N. Leuenberger , Eduardo R. Mucciolo

We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…

强关联电子 · 物理学 2009-11-11 C. Romeike , M. R. Wegewijs , H. Schoeller

We study electronic transport through a magnetic molecule with an intrinsic spin $S$ coupled to two magnetic electrodes, in the incoherent regime. The molecule is modeled as a single resonant level with large Coulomb repulsion (no double…

介观与纳米尺度物理 · 物理学 2010-11-19 Thibaut Jonckheere , Ken-Ichiro Imura , Thierry Martin

This chapter takes a microscopic view of quantum tunneling of magnetization (QTM) in single-molecule magnets (SMMs), focusing on the interplay between exchange and anisotropy. Careful consideration is given to the relationship between…

介观与纳米尺度物理 · 物理学 2013-03-04 Junjie Liu , Enrique del Barco , Stephen Hill

We explore theoretically the spin transport in nanostructures consisting of a gold quantum dot bridging nonmagnetic electrodes and two Mn12-Ph single molecule magnets (SMMs) that are thiol-bonded to the dot but are not in direct contact…

介观与纳米尺度物理 · 物理学 2015-06-15 Fatemeh Rostamzadeh Renani , George Kirczenow

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical…

介观与纳米尺度物理 · 物理学 2017-05-12 Andrew K. Mitchell , Kim G. L. Pedersen , Per Hedegaard , Jens Paaske

An important consequence of the discovery of giant magnetoresistance in metallic magnetic multilayers is a broad interest in spin dependent effects in electronic transport through magnetic nanostructures. An example of such systems are…

介观与纳米尺度物理 · 物理学 2009-11-13 J. Barnas , I. Weymann

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin…

介观与纳米尺度物理 · 物理学 2013-05-29 Florian Elste , Carsten Timm

We analyze the stationary spin-dependent transport through a single-molecule magnet weakly coupled to external ferromagnetic leads. Using the real-time diagrammatic technique, we calculate the sequential and cotunneling contributions to…

介观与纳米尺度物理 · 物理学 2010-10-29 Maciej Misiorny , Ireneusz Weymann , Jozef Barnas

We discuss the electronic transport through molecules in the Kondo regime. We concentrate here on the influence of molecular vibrations. Two types of vibrations are investigated: (i) the breathing internal molecular modes, where the…

介观与纳米尺度物理 · 物理学 2009-12-21 J. Mravlje , A. Ramsak

The ability to make electrical contact to single molecules creates opportunities to examine fundamental processes governing electron flow on the smallest possible length scales. We report experiments in which we controllably stretch…

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