相关论文: A Bright, Slow Cryogenic Molecular Beam Source for…
We demonstrate buffer gas cooling of carbon atoms to cryogenic temperatures. By employing pulsed two-photon excitation followed by vacuum ultraviolet fluorescence detection, we measured the arrival time distribution of the ablated carbon…
We study laser cooling of atomic gases by collisional redistribution of fluorescence. In a high pressure buffer gas regime, frequent collisions perturb the energy levels of alkali atoms, which allows for the absorption of a far red detuned…
Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…
It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…
We report the slowing of a supersonic beam by elastic reflection from a receding atomic mirror. We use a pulsed supersonic nozzle to generate a 511 +/- 9 m/s beam of helium that we slow by reflection from a Si(111)-H(1x1) crystal placed on…
We demonstrate experimentally the continuous and pulsed loading of a slow and cold atomic beam into a magnetic guide. The slow beam is produced using a vapor loaded laser trap, which ensures two-dimensional magneto-optical trapping, as well…
Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…
Using the Green Bank Telescope (GBT), we have detected the (J,K) = (1,1) to (10,10) ammonia inversion lines, up to 1030 K above the ground state, in a face-on spiral galaxy viewed against the radio continuum of the lensed background source…
A high-intensity supersonic beam source has been a key component in studies of molecular collisions, molecule-surface interaction, chemical reactions, and precision spectroscopy. However, the molecular density available for experiments in a…
We detail the design of a variable energy, x-ray fluorescence source using a low activity (1.8$\times10^6$~dpm) \nuc{99}{Tc} $\beta$ source that irradiates thin foils. By rotating the source among foils of Ti, Zn, Nb, Ag, and Au, the device…
We describe an instrument which can be used to analyze complex chemical mixtures at high resolution and high sensitivity. Molecules are collisionally cooled with helium gas at cryogenic temperatures (~ 4-7 K), and subsequently detected…
We demonstrate rotational excitation of molecular ions that are sympathetically cooled by laser-cooled atomic ions to a temperature as low as ca. 10 mK. The molecular hydrogen ions HD+ and the fundamental rotational transition $(v=0,\,…
The biphotons, generated from a hot atomic vapor via the process of spontaneous four-wave mixing (SFWM), have the following merits: stable and tunable frequencies as well as linewidth. Such merits are very useful in the applications of…
We have focused and decelerated benzonitrile (C$_7$H$_5$N) molecules from a molecular beam, using an array of time-varying inhomogeneous electric fields in alternating gradient configuration. Benzonitrile is prototypical for large…
We use narrow-band laser excitation of Yb to substantially enhance the brightness of a cold beam of YbOH, a polyatomic molecule with high sensitivity to physics beyond the Standard Model (BSM). By exciting atomic Yb to the metastable…
We report a novel source of twin beams based on modulational instability in high-pressure argon-filled hollow-core kagom\'e-style photonic-crystal fibre. The source is Raman-free and manifests strong photon-number correlations for…
The cryogenic buffer gas beam (CBGB) is an important tool in the study of cold and ultracold molecules. While there are known techniques to enhance desired beam properties, such as high flux, low velocity, or reduced divergence, they have…
We present a new method for the generation of rotationally and vibrationally state-selected, translationally cold molecular ions in ion traps. Our technique is based on the state-selective threshold photoionization of neutral molecules…
High fluxes of cold polar molecules are efficiently produced by electric guiding and velocity filtering. Here, we investigate different aspects of the beam formation. Variations of the source parameters such as density and temperature…
We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…