相关论文: Carbon dioxide in silicate melts: A molecular dyna…
Carbon dioxide is one of the major contributors to the radiative forcing, increasing both the temperature and the humidity of Earth's atmosphere. If the stellar irradiance increases and water becomes abundant in the stratosphere of an…
The geological record shows links between glacial cycles and volcanic productivity, both subaerially and at mid-ocean ridges. Sea-level-driven pressure changes could also affect chemical properties of mid-ocean ridge volcanism. We consider…
There is accumulating evidence for the presence of complex molecules, including carbon-bearing and organic molecules, in the interstellar medium. Much of this evidence comes to us from studies of chemical composition, photo- and…
The objective of this study is to use molecular dynamics simulation (MD) to evaluate the vesicularity and noble gas fractionation, and to shed light on bubble formation during MORB degassing. A previous simulation study (Guillot and Sator…
The high-pressure dynamics of a computer-modeled silica melt is studied in the framework of the mode-coupling theory of the glass transition (MCT) using static-structure input from molecular-dynamics (MD) computer simulation. The theory…
Aims: The long-term carbon cycle for planets with a surface entirely covered by oceans works differently from that of the present-day Earth because inefficient erosion leads to a strong dependence of the weathering rate on the rate of…
The dissolution and subsequent mass transfer of carbon dioxide gas into liquid barriers plays a vital role in many environmental and industrial applications. In this work, we study the downward dissolution and propagation dynamics of CO2…
We perform large-scale numerical simulations of convection in 3D porous media at Rayleigh-Darcy numbers up to $Ra=8\times10^4$. To investigate the convective mixing of carbon dioxide (CO$_2$) in geological formations, we consider a…
Observationally inferred crystalline abundance in silicates in comets, which should have been formed in the outer region of a protoplanetary disk, is relatively high (~ 10-60%), although crystalline silicates would be formed by annealing of…
Carbon capture and storage (CCS) has emerged as the most effective method to curb the CO2 concentration in the atmosphere. It can store up to 5 billion tons of CO2 per year. To guarantee a safe and economical geological storage, the well…
We develop a methodological framework and mathematical formulation which yields estimates of the uncertainty associated with the amounts of CO2 generated by carbonate-clays reactions (CCR) in large-scale subsurface systems to assist…
Cycling of carbon dioxide between the atmosphere and interior of rocky planets can stabilize global climate and enable planetary surface temperatures above freezing over geologic time. However, variations in global carbon budget and…
We discuss 3D global simulations of the early Martian climate that we have performed assuming a faint young Sun and denser CO2 atmosphere. We include a self-consistent representation of the water cycle, with atmosphere-surface interactions,…
Weathering of silicate rocks at a planetary surface can draw down CO$_2$ from the atmosphere for eventual burial and long-term storage in the planetary interior. This process is thought to provide an essential negative feedback to the…
Atomistic simulations provide a meaningful way to determine the physico-chemical properties of liquids in a consistent theoretical framework. This approach takes on particular usefulness for the study of molten carbonates, in a context…
Existence of strongly bound water molecules on silicate surfaces, above the desorption temperature of water ice, has been first predicted by computational studies and recently demonstrated by laboratory experiments. Such trapped water may…
Understanding interfacial phenomena in confined systems is important for optimizing CO2 capture technologies. Here, we present a comprehensive investigation of CO2 adsorption in hydrated amorphous silica nanopores through an integrated…
In the conventional habitable zone (HZ) concept, a CO$_{2}$-H$_2$O greenhouse maintains surface liquid water. Through the water-mediated carbonate-silicate weathering cycle, atmospheric CO$_{2}$ partial pressure (pCO$_{2}$) responds to…
The adsorption of volatile molecules onto dust grain surfaces fundamentally influences dust-related processes, including condensation of gas-phase molecules, dust coagulation, and planet formation in protoplanetary disks. Using advanced…
The liquid metal-liquid silicate partitioning of molybdenum and tungsten during core formation must be well-constrained in order to understand the evolution of Earth and other planetary bodies, in particular because the Hf-W isotopic system…