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We point out that single electron charging effects such as Coulomb Blockade (CB) and high-bias staircases play a crucial role in transport through single ultrashort molecules. A treatment of Coulomb Blockade through a prototypical molecule,…

介观与纳米尺度物理 · 物理学 2009-11-11 Bhaskaran Muralidharan , Avik W Ghosh , Swapan K Pati , Supriyo Datta

The renormalization method is applied to investigate the electron transmission properties of a circuit containing a benzene molecule, in which one of the carbon atoms has been modified so as to simulate displacement in position or…

介观与纳米尺度物理 · 物理学 2016-07-08 Dong Qiu , Kenneth W. Sulston

We discuss the key steps that have to be followed to calculate coherent quantum transport in molecular and atomic-scale systems, making emphasis on the ab-initio Gaussian Embedded Cluster Method recently developed by the authors. We present…

材料科学 · 物理学 2007-05-23 J. J. Palacios , A. J. Perez-Jimenez , E. Louis , J. A. Verges , E. SanFabian

Motivated by the ever-improving performance of deep learning techniques, we design a mixed input convolutional neural network approach to predict transport properties in deformed nanoscale materials using a height map of deformations (from…

介观与纳米尺度物理 · 物理学 2022-09-09 Jack G. Nedell , Jonah Spector , Adel Abbout , Michael Vogl , Gregory A. Fiete

We present a procedure to determine transmission eigenchannels for coherent phonon transport in nanoscale devices using the framework of nonequilibrium Green's functions. We illustrate our procedure by analyzing a one-dimensional chain,…

介观与纳米尺度物理 · 物理学 2018-05-02 J. C. Klöckner , J. C. Cuevas , F. Pauly

We present a novel model to describe conduction band of GaN_xAs_{1-x} (GaNAs). As well known, GaNAs shows exotic behavior such as large band gap bowing. Although there are various models to describe the conduction band of GaNAs, origin of…

材料科学 · 物理学 2014-12-30 Masato Morifuji , Fumitaro Ishikawa

A method for the calculation of the conductance of nanoscale electrical junctions is extended to ab-initio electronic structure methods and applied to realistic models of metallic wires and break-junctions of sodium and gold. The method is…

材料科学 · 物理学 2014-05-13 Matthieu J. Verstraete , P. Bokes , R. W. Godby

The recent paper by Fujimoto and Hirose makes an unfortunate error in discussing the use of the jellium model for the electrodes, which has the effect of making it appear that this model is not adequate to treat the problem of the…

介观与纳米尺度物理 · 物理学 2009-11-10 N. D. Lang , M. Di Ventra

The ability to control the conductance of single molecules will have a major impact in nanoscale electronics. Azobenzene, a molecule that changes conformation as a result of a trans/cis transition when exposed to radiation, could form the…

介观与纳米尺度物理 · 物理学 2008-11-26 Miriam del Valle , Rafael Gutierrez , Carlos Tejedor , Gianaurelio Cuniberti

We propose a mixed analytical-ab-initio method for the accurate calculation of the conductance in monovalent atomic wires. The method relies on the most general formula for ballistic transport through a monovalent wire, whose parameters can…

介观与纳米尺度物理 · 物理学 2016-08-16 Péter Major , V. M. García-Suárez , S. Sirichantaropass , József Cserti , C. J. Lambert , J. Ferrer , Géza Tichy

We present ab initio calculations of transport properties of atomic-sized aluminum contacts in the presence of oxygen. The experimental situation is modeled by considering a single oxygen atom (O) or one of the molecules O2 and O3 bridging…

介观与纳米尺度物理 · 物理学 2009-05-24 S. Wohlthat , F. Pauly , J. K. Viljas , J. C. Cuevas , Gerd Schön

Coherent electronic transport through individual molecules is crucially sensitive to quantum interference. Using exact diagonalization techniques, we investigate the zero-bias and zero-temperature conductance through $\pi$-conjugated…

强关联电子 · 物理学 2015-05-14 Julian Rincon , K. Hallberg , S. Ramasesha

Predicting nanoscale thermal transport in dielectrics requires models, such as the Boltzmann transport equation (BTE), that account for phonon boundary scattering in structures with complex geometries. Although the BTE has been validated…

材料科学 · 物理学 2023-08-03 S. Aria Hosseini , Alex Greaney , Giuseppe Romano

We present a theoretical study of the transport characteristics of molecular junctions, where first-row diatomic molecules are attached to (001) gold and platinum electrodes. We find that the conductance of all of these junctions is of the…

介观与纳米尺度物理 · 物理学 2015-05-13 J. Ferrer , V. M. Garcia-Suarez

One of the fundamental properties of semiconductors is their ability to support highly tunable electric currents in the presence of electric fields or carrier concentration gradients. These properties are described by transport coefficients…

材料科学 · 物理学 2020-02-19 Samuel Poncé , Wenbin Li , Sven Reichardt , Feliciano Giustino

We have investigated the effects of the interfacial bond arrangement on the electronic transport features of metal-nanotube-metal systems. The transport properties of finite, defect-free armchair and zigzag single-walled carbon nanotubes…

材料科学 · 物理学 2007-05-23 Ioannis Deretzis , Antonino La Magna

The effect of vibrational motion on resonant charge transport through single molecule junctions is investigated. The study is based on a combination of first-principles electronic structure calculations to characterize the system and…

其他凝聚态物理 · 物理学 2007-12-24 Claudia Benesch , Martin Cizek , Jiri Klimes , Michael Thoss , Wolfgang Domcke

The anomalous spin transport coefficients of gapped Dirac electrons are studied with application to a quasi-two-dimensional organic conductor $\alpha$-(BETS)$_2$I$_3$ in mind. In the presence of a gap induced by spin-orbit interaction, we…

介观与纳米尺度物理 · 物理学 2022-02-04 Masao Ogata , Soshun Ozaki , Hiroyasu Matsuura

An efficient computational methodology is used to explore charge transport properties in chemically-modified (and randomly disordered) graphene-based materials. The Hamiltonians of various complex forms of graphene are constructed using…

介观与纳米尺度物理 · 物理学 2011-12-16 Nicolas Leconte , Aurélien Lherbier , François Varchon , Pablo Ordejon , Stephan Roche , Jean-Christophe Charlier

Cluster-assembled metallic films show interesting electrical properties, both in the near-to-percolation regime, when deposited clusters do not form a complete layer yet, and when the film thickness is well above the electrical percolation…

介观与纳米尺度物理 · 物理学 2021-12-20 Miquel López-Suárez , Claudio Melis , Luciano Colombo , Walter Tarantino