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Modern theories of quantum magnetism predict exotic multipolar states in weakly interacting strongly frustrated spin-1/2 Heisenberg chains with ferromagnetic nearest neighbor (NN) inchain exchange in high magnetic fields. Experimentally…

We report a single-crystal study on the magnetism of the rare-earth compound PrTiNbO$_6$ that experimentally realizes the zigzag pseudospin-$\frac{1}{2}$ quantum antiferromagnetic chain model. Random crystal electric field caused by the…

强关联电子 · 物理学 2018-06-05 Yuesheng Li , Sebastian Bachus , Yoshifumi Tokiwa , Alexander A. Tsirlin , Philipp Gegenwart

Single crystals of a new silver and-cobalt based vanadate AgCo2V3O10 were grown from a melted mixture. The crystal structure determination reveals that this new vanadate crystallizes in triclinic system with space group P-1. The structure…

Spin-1/2 Heisenberg model on kagome lattice is a typical frustrated quantum spin system. A basic structure of kagome lattice is also present in kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus…

强关联电子 · 物理学 2018-01-19 K. Morita , T. Sugimoto , S. Sota , T. Tohyama

We report a new peculiar effect of the interaction between a sublattice of frustrated quantum spin-1/2 chains and a sublattice of pseudospin-1/2 centers (quantum electric dipoles) uniquely co-existing in the complex oxide Li2ZrCuO4. 7Li…

The strong corrugation of the V4O9 layer in the spin gap system CaV4O9 is examined for its impact on the exchange coupling constants between the spin 1/2 V ions. Local spin density (LSD) calculations show that the V spin occupies a…

强关联电子 · 物理学 2008-02-03 W. E. Pickett

We report $^{63}$Cu nuclear magnetic resonance and muon spin rotation measurements on the S=1/2 antiferromagnetic Heisenberg spin chain compound Sr$_{1.9}$Ca$_{0.1}$CuO$_3$. An exponentially decreasing spin-lattice relaxation rate 1/T$_1$…

Electron spin resonance experiments in the quasi-1D S=1/2 antiferromagnet K$_2$CuSO$_4$Cl$_2$ reveal opening of a gap in absence of magnetic ordering, as well as an anisotropic shift of the resonance magnetic field. These features of…

强关联电子 · 物理学 2018-11-14 T. A. Soldatov , A. I. Smirnov , K. Yu. Povarov , M. Hälg , W. E. A. Lorenz , A. Zheludev

In a frustrated J_1-J_2 chain with the nearest-neighbor ferromagnetic interaction J_1 and the next-nearest-neighbor antiferromagnetic interaction J_2, novel magnetic states such as a spin-nematic state are theoretically expected. However,…

NaOsO3 hosts a rare manifestation of a metal-insulator transition driven by magnetic correlations, placing the magnetic exchange interactions in a central role. We use resonant inelastic x-ray scattering to directly probe these magnetic…

We study the spin gap of the S=1/2 Heisenberg model on the distorted diamond chain, which is recently proposed to represent magnetic properties of Cu_3 Cl_6 (H_2 O)_2 2H_8 C_4 SO_2. This model is composed of stacked trimers and has three…

强关联电子 · 物理学 2009-10-31 Kazuhiro Sano , Ken'ichi Takano

The temperature dependent ac and dc magnetization and heat capacity data of Ca$_3$CoIrO$_6$, a spin-chain compound crystallizing in a K$_4$CdCl$_6$-derived rhombohedral structure, show the features due to magnetic ordering of a…

强关联电子 · 物理学 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran

We present a detailed investigation of the magnetic properties of the spin-$\frac{3}{2}$ system Li$_2$Co(WO$_4$)$_2$ by means of magnetic susceptibility and specific heat. Our experimental results show that in Li$_2$Co(WO$_4$)$_2$ a…

Motivated by recent interest in quasi-one-dimensional compound CaV2O4, we study the ground states of a spin-orbital chain characterized by an Ising-like orbital Hamiltonian and frustrated interactions between S=1 spins. The on-site…

强关联电子 · 物理学 2010-07-13 Gia-Wei Chern , Natalia Perkins

In both spinel compounds GeCo$_2$O$_4$ and GeNi$_2$O$_4$ which order antiferromagnetically (at $T_N = 23.5 K$ and $T_{N_1} = 12.13 K$, $T_{N_2} = 11.46 K$) with different Curie Weiss temperatures ($T_{CW}$=80.5 K and -15 K), the usual…

强关联电子 · 物理学 2009-11-11 Sébastien Diaz , Sophie De Brion , G. Chouteau , Benjamin Canals , Virginie Simonet , P. Strobel

The spin-1/2 Cu2+ ions of LiCuVO4 form one-dimensional chains along the b-direction, and the spin frustration in LiCuVO4 is described in terms of the nearest-neighbor ferromagnetic exchange J1 and the next-nearest-neighbor antiferromagnetic…

强关联电子 · 物理学 2011-03-09 Hyun-Joo Koo , Changhoon Lee , Myung-Hwan Whangbo , Garry J. McIntyre , Reinhard K. Kremer

We have studied the structural, magnetic properties, and electronic structure of the compound InCuPO5 synthesized by solid state reaction method. The structure of InCuPO5 comprises of S = 1/2 uniform spin chains formed by corner-shared CuO4…

强关联电子 · 物理学 2017-05-30 B. Koteswararao , Binoy K. Hazra , Dibyata Rout , P. V. Srinivasarao , S. Srinath , S. K. Panda

We develop a microscopic theory of finite-temperature spin-nematic orderings in three-dimensional spatially anisotropic magnets consisting of weakly-coupled frustrated spin-1/2 chains with nearest-neighbor and next-nearest-neighbor…

强关联电子 · 物理学 2013-02-19 Masahiro Sato , Toshiya Hikihara , Tsutomu Momoi

We study the phase diagram of a frustrated spin-1/2 ferromagnetic chain with anisotropic exchange interactions in an external magnetic field, using the density matrix renormalization group method. We show that an easy-axis anisotropy…

强关联电子 · 物理学 2009-10-29 F. Heidrich-Meisner , I. P. McCulloch , A. K. Kolezhuk

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…