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Dynamic nuclear polarization (DNP) is an NMR hyperpolarization technique that mediates polarization transfer from highly polarized unpaired electrons to NMR-active nuclei via microwave (mw) irradiation. The ability to generate arbitrarily…

Dynamic nuclear polarization (DNP) is an NMR sensitivity enhancement technique that mediates polarization transfer from unpaired electrons to NMR-active nuclei. Despite its success in elucidating important structural information on…

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…

量子物理 · 物理学 2018-10-24 Q. Chen , Z. -Y. Wang , B. Tratzmiller , I. Schwartz , M. B. Plenio

The frequency splitting between the dip and the peak of the resistively detected nuclear magnetic resonance (RDNMR) dispersive line shape (DLS) has been measured in the quantum Hall effect regime as a function of filling factor, carrier…

介观与纳米尺度物理 · 物理学 2015-06-18 W. Desrat , B. A. Piot , S. Krämer , D. K. Maude , Z. R. Wasilewski , M. Henini , R. Airey

We discuss the polarization dynamics during solid effect dynamic nuclear polarization (DNP) in a central spin model that consists of an electron surrounded by many nuclei. To this end we use a recently developed formalism and validate first…

其他凝聚态物理 · 物理学 2016-03-23 Daniel Wiśniewski , Alexander Karabanov , Igor Lesanovsky , Walter Köckenberger

Dynamic Nuclear Polarization (DNP) is transforming NMR and MRI by significantly enhancing sensitivity through the transfer of polarization from electron spins to nuclear spins via microwave irradiation. However, the use of monochromatic…

量子物理 · 物理学 2024-10-28 Mayur Jhamnani , Sajith V Sadasivan , Sheetal Kumar Jain , Asif Equbal

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

介观与纳米尺度物理 · 物理学 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

介观与纳米尺度物理 · 物理学 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

We theoretically investigate the dynamical nuclear spin polarization in a quantum point contact (QPC) at finite magnetic field. We find that when the QPC is tuned to be spin selective, at the conductance of e^2/h, a finite bias induces a…

介观与纳米尺度物理 · 物理学 2018-03-20 Peter Stano , Tomosuke Aono , Minoru Kawamura

We consider the dynamic nuclear spin polarization (DNP) using two electrons in a double quantum dot in presence of external magnetic field and spin-orbit interaction, in various schemes of periodically repeated sweeps through the S-T+…

介观与纳米尺度物理 · 物理学 2015-06-17 Izhar Neder , Mark S. Rudner , Bertrand I. Halperin

Dynamic nuclear polarization (DNP) can increase nuclear magnetic resonance (NMR) signals by orders of magnitude. DNP in diamond proceeds through different DNP mechanisms with a possible temperature-dependence. We report on 13C dynamic…

It is demonstrated that the now well-established `flip-flop' mechanism of spin exchange between electrons and nuclei in the quantum Hall effect can be reversed. We use a sample geometry which utilizes separately contacted edge states to…

介观与纳米尺度物理 · 物理学 2009-11-11 A. Würtz , T. Müller , A. Lorke , D. Reuter , A. D. Wieck

Dynamic nuclear polarization transfers spin polarization from electrons to nuclei. We have achieved this by a new method, simultaneously exciting transitions of electronic and nuclear spins. The efficiency of this technique improves with…

量子物理 · 物理学 2008-09-11 G. W. Morley , K. Porfyrakis , A. Ardavan , J. van Tol

We study the role of dipolar interactions in the standard protocol used to achieve dynamic nuclear polarization (DNP). In the so-called spin-temperature regime, where the interactions establish an effective thermodynamic behavior in the…

强关联电子 · 物理学 2016-07-13 Andrea De Luca , Inés Rodríguez Arias , Markus Müller , Alberto Rosso

Polarization transfers are crucial building blocks in magnetic resonance experiments, i.e., they can be used to polarize insensitive nuclei and correlate nuclear spins in multidimensional NMR spectroscopy. The polarization can be…

化学物理 · 物理学 2022-08-24 Zhenfeng Pang , Sheetal Jain , Chen Yang , Xueqian Kong , Kong Ooi Tan

In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…

强关联电子 · 物理学 2017-02-28 Filippo Caracciolo , Marta Filibian , Pietro Carretta , Alberto Rosso , Andrea De Luca

In pulsed dynamic nuclear polarization (DNP), enhancement of the polarization of bulk nuclei requires the repeated application of a microwave pulse sequence. So far, analysis of a one-time transfer of electron spin polarization to a…

When the motion of electrons is restricted to a plane under a perpendicular magnetic field B, a variety of quantum phases emerge at low temperatures whose properties are dictated by the Coulomb interaction and its interplay with disorder.…

介观与纳米尺度物理 · 物理学 2015-06-23 L. Tiemann , T. D. Rhone , N. Shibata , K. Muraki

Resistively Detected Nuclear Magnetic Resonance (RD-NMR) has been used to investigate a two-subband electron system in a regime where quantum Hall pseudo-spin ferromagnetic (QHPF) states are prominently developed. It reveals that the…

介观与纳米尺度物理 · 物理学 2015-05-13 G. P. Guo , Y. J. Zhao , T. Tu , X. J. Hao , G. C. Guo , H. W. Jiang