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We present magnetization measurements on oriented powder of ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ along and perpendicular to the orienting field. We find a dramatic difference in the magnetization between the two directions. It is biggest at low…

强关联电子 · 物理学 2009-04-21 Oren Ofer , Amit Keren

To capture the high-field magnetization process of herbertsmithite (ZnCu3(OH)6Cl2), Faraday rotation (FR) measurements were carried out on a single crystal in magnetic fields of up to 190 T. The magnetization data evaluated from the FR…

强关联电子 · 物理学 2020-09-29 Ryutaro Okuma , Daisuke Nakamura , Shojiro Takeyama

Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel…

强关联电子 · 物理学 2017-01-06 A. Zorko , M. Herak , M. Gomilšek , J. van Tol , M. Velázquez , P. Khuntia , F. Bert , P. Mendels

Herbertsmithite is known as the archetype of a S=1/2 nearest-neighbor Heisenberg antiferromagnet on the Kagom\'e lattice, theoretically presumed to be a quantum gapless spin liquid. However, more and more experiments reveal that the model…

Magnetization, specific heat, and neutron scattering measurements were performed to study a magnetic transition in jarosite, a spin-5/2 kagome lattice antiferromagnet. When a magnetic field is applied perpendicular to the kagome plane,…

We report 17O NMR measurements in the S=1/2 Cu2+ kagome antiferromagnet Herbertsmithite ZnCu3(OH)6Cl2 down to 45mK in magnetic fields ranging from 2T to 12T. While Herbertsmithite displays a gapless spin-liquid behavior in zero field, we…

强关联电子 · 物理学 2013-09-09 M. Jeong , F. Bert , P. Mendels , F. Duc , J. C. Trombe , M. A. de Vries , A. Harrison

The dc-magnetization of the unique S=1/2 kagome antiferromagnet Herbertsmithite has been measured down to 0.1K. No sign of spin freezing is observed in agreement with former muSR and ac-susceptibility results. The low temperature magnetic…

强关联电子 · 物理学 2009-11-13 F. Bert , S. Nakamae , F. Ladieu , D. L'Hôte , P. Bonville , F. Duc , J. -C. Trombe , P. Mendels

Spin-reorientation phase transitions that involve the rotation of a crystal$'$s magnetization have been well characterized in distorted-perovskite oxides such as the orthoferrites. In these systems spin reorientation occurs due to competing…

强关联电子 · 物理学 2020-06-29 A. M. Vibhakar , D. D. Khalyavin , P. Manuel , J. Liu , A. A. Belik , R. D. Johnson

Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

强关联电子 · 物理学 2016-12-05 M. R. Norman

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

强关联电子 · 物理学 2015-06-18 Oren Ofer , Lital Marcipar , V. Ravi Chandra , Snir Gazit , Daniel Podolsky , Daniel P. Arovas , Amit Keren

Polarised neutron diffraction measurements have been made on HoFeO$_3$ single crystals magnetised in both the [001] and [100] directions ($Pbnm$ setting). The polarisation dependencies of Bragg reflection intensities were measured both with…

强关联电子 · 物理学 2017-09-13 T. Chatterji , A. Stunault , P. J. Brown

We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…

强关联电子 · 物理学 2012-04-16 Tianheng Han , Shaoyan Chu , Young S. Lee

Centrosymmetric GdRu$_2$Si$_2$ exhibits a variety of multi-Q magnetic states as a function of temperature and applied magnetic field, including a square skyrmion-lattice phase. The material's behavior is strongly dependent on the direction…

We prepared a powder sample of edwardsite Cd2Cu3(SO4)2(OH)6 4H2O, which is a new candidate compound for the spin-1/2 kagome antiferromagnet, and studied its magnetic properties by magnetic susceptibility and heat capacity measurements.…

材料科学 · 物理学 2015-06-15 Hajime Ishikawa , Yoshihiko Okamoto , Zenji Hiroi

We report torque magnetometry results on single crystals of karpenkoite Co3(V2O7)(OH)2 2H2O, a model candidate for the kagome antiferromagnet. No field-induced phase transition is detected up to 45 T for B||c and B||a. Instead, the torque…

强关联电子 · 物理学 2026-02-20 Hibiki Kunisawa , Ryuya Watanabe , Jun-ichi Yamaura , Yoshimitsu Kohama , Toshihiro Nomura

Amato {\it et al.} have reported transverse field muon spin rotation experiments performed on single crystal of MnSi in a single magnetic field of 5200 Oe at a single temperature of 50 K. They present the angular dependence of the muon…

强关联电子 · 物理学 2014-11-18 Vyacheslav G. Storchak , Andrey M. Tokmachev

We report a muon spin rotation/relaxation ($\mu$SR) study of single-crystalline samples of the $\alpha$-RuCl$_3$ honeycomb magnet, which is presumed to be a model compound for the Kitaev-Heisenberg interaction. It is inferred from magnetic…

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

强关联电子 · 物理学 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

We use a hydrodynamic approach to investigate dynamic spin susceptibility of the antiferromagnetic spin-$1/2$ Heisenberg chain with a uniform Dzyaloshinskii-Moriya (DM) interaction in the presence of an external magnetic field. We find that…

强关联电子 · 物理学 2022-06-06 Ren-Bo Wang , Anna Keselman , Oleg A. Starykh

Herbertsmithite (ZnCu3(OH)6Cl2) is often discussed as the best realization of the highly frustrated antiferromagnetic kagome lattice known so far. We employ density functional theory calculations to determine eight exchange coupling…

强关联电子 · 物理学 2014-01-31 Harald O. Jeschke , Francesc Salvat-Pujol , Roser Valenti
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