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We report on evaluation of lattice thermal conductivity of GeTe/Sb$_{2}$Te$_{3}$ superlattice (SL) by using femtosecond coherent phonon spectroscopy at various lattice temperatures. The time-resolved transient reflectivity obtained in…

材料科学 · 物理学 2011-07-21 Muneaki Hase , Junji Tominaga

Anharmonic decay of coherent optical phonons in semimetal Sb has been investigated by using a femtosecond pump-probe technique. The coherent $A_{1g}$ mode is observed in time domain in a wide temperature range of 7 - 290 K. The decay rate…

材料科学 · 物理学 2015-01-12 Muneaki Hase , Kiminori Ushida , Masahiro Kitajima

We have performed ultrafast pump-probe spectroscopy studies on a series of InAs/GaSb-based short-period superlattice (SL) samples with periods ranging from 46 \AA to 71 \AA. We observe two types of oscillations in the differential…

材料科学 · 物理学 2012-11-26 G. T. Noe , H. J. Haugan , G. J. Brown , G. D. Sanders , C. J. Stanton , J. Kono

The femtosecond optical pump-probe technique was used to study dynamics of photoexcited electrons and coherent optical phonons in transition metals Zn and Cd as a function of temperature and excitation level. The optical response in time…

强关联电子 · 物理学 2009-11-11 Muneaki Hase , Kunie Ishioka , Jure Demsar , Kiminori Ushida , Masahiro Kitajima

We investigate ultrafast phonon dynamics in the Bi$_{1-x}$Sb$_{x}$ alloy system for various compositions $x$ using a reflective femtosecond pump-probe technique. The coherent optical phonons corresponding to the A$_{1g}$ local vibrational…

材料科学 · 物理学 2021-02-05 Yuta Komori , Yuta Saito , Paul Fons , Muneaki Hase

Chalcogenide superlattices (SL) consist of alternate stacking of GeTe and Sb$_{2}$Te$_{3}$ layers. The structure can become a 3D topological insulator depending on the constituent layer thicknesses, making the design of the SL period a…

材料科学 · 物理学 2019-07-30 Takara Suzuki , Yuta Saito , Paul Fons , Alexander V. Kolobov , Junji Tominaga , Muneaki Hase

We report on the dynamics of coherent phonons in semimetal 1T'-MoTe2 using femtosecond pump-probe spectroscopy. On an ultrafast sub-picosecond time scale at room temperature, a low frequency and long-lifetime shear phonon mode was observed…

材料科学 · 物理学 2020-03-09 T. Fukuda , K. Makino , Y. Saito , P. Fons , A. V. Kolobov , K. Ueno , M. Hase

We examine the ultrafast optical response of the crystalline and amorphous phases of the phase change material Ge$_2$Sb$_2$Te$_5$ below the phase transformation threshold. Simultaneous measurement of the transmissivity and reflectivity of…

材料科学 · 物理学 2016-07-19 Timothy A. Miller , Miquel Rudé , Valerio Pruneri , Simon Wall

A coherent THz optical lattice mode is triggered by femtosecond laser pulses in the antiferromagnetic van der Waals semiconductor FePS$_3$. The 380 nm thick exfoliated flake was placed on a substrate and laser-driven lattice and spin…

Spintronics is postulated on the possibility to employ the magnetic degree of freedom of electrons for computation and couple it to charges. In this view, the combination of the high-frequency of spin manipulations offered by…

We investigate the ultrafast lattice dynamics in ${1T-TiSe_2}$ using femtosecond reflection pump-probe and pump-pump-probe techniques at room temperature. The time-domain signals and Fourier-transformed spectra show the $A_{1g}$ phonon mode…

材料科学 · 物理学 2023-06-12 Yu Mizukoshi , Takumi Fukuda , Yuta Komori , Ryo Ishikawa , Keiji Ueno , Muneaki Hase

The excitation and detection of coherent phonons has given unique insights into condensed matter, in particular for materials with strong electron-phonon coupling. We report a study of coherent phonons in the layered charge density wave…

We reported the quasiparticle relaxation dynamics of an optimally doped triclinic iron-based superconductor (Ca$_{0.85}$La$_{0.15}$)$_{10}$(Pt$_3$As$_8$)(Fe$_2$As$_2$)$_5$ with bulk $T_c$ = 30 K using polarized ultrafast optical pump-probe…

1$T$-TaSe$_{2}$ is host to coexisting strongly-correlated phases including charge density waves (CDWs) and an unusual Mott transition at low temperature. Here, we investigate coherent phonon oscillations in 1$T$-TaSe$_{2}$ using a…

This work investigates the impact of device length on thermal conductivity in periodic and aperiodic superlattices (SLs). While it is well known that thermal conductivity in aperiodic SLs exhibits a weaker dependence on device length…

材料科学 · 物理学 2024-12-23 Theodore Maranets , Yan Wang

Quantum coherent coupling between a zone-center phonon and two acoustic phonons was observed in two GaAs/AlAs superlattices (8 nm/8 nm and 5.4 nm/5.4 nm) at ambient temperature. Using degenerate coherent phonon spectroscopy, a multi-cycle…

材料科学 · 物理学 2019-07-25 Feng He , Nathanial Sheehan , Seth R Bank , Raymond L Orbach , Yaguo Wang

In this study, we have used atomistic phonon wave-packet simulations to investigate the manifestation of coherent phonons and phonon transmission in gradient superlattices (SL) based on ordered arrangements of varied SL period sizes. We…

材料科学 · 物理学 2026-03-17 Evan Wallace Doe , Theodore Maranets , Yan Wang

Using $\approx$40 fs ultrashort laser pulses, we investigate the picosecond acoustic response from a prototypical phase change material, thin Ge$_{2}$Sb$_{2}$Te$_{5}$ (GST) films with various thicknesses. After excitation with a 1.53…

材料科学 · 物理学 2015-11-18 Muneaki Hase , Paul Fons , Alexander V. Kolobov , Junji Tominaga

Intense ultrafast laser excitation can produce transient states of condensed matter that would otherwise be inaccessible. At high excitation level, the interatomic forces can be altered resulting in an unusual lattice dynamics. Here we…

材料科学 · 物理学 2011-03-18 O. V. Misochko , M. V. Lebedev

Ultrafast lattice dynamics of few quintuple layers of topological insulator (TI) Bi$_2$Te$_3$ is studied with time-resolved optical pump-probe spectroscopy. Both optical and acoustic phonons are photogenerated and detected. Here, in order…

材料科学 · 物理学 2015-07-09 W. Weiss , K. Balin , R. Rapacz , A. Nowak , J. Szade , M. Lejman , P. Ruello
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