相关论文: Dynamics of photo-activated Coulomb complexes
We theoretically study the process of photoelectron emission of the Helium atom by a high-intensity short-wavelength laser at a resonance condition of the residual singly charged ion. Photoionization followed by strong resonance coupling in…
We consider the model of quantum dots interacting with coherent radiation when the relaxation processes may be neglected. The system under investigation consists of two discrete energy levels of the quantum dots in the presence of strong…
We present efficient and reliable molecular dynamics simulations of the photodissociation of dichloromethane followed by Coulomb explosion. These simulations are performed by calculating trajectories on accurate potential energy surfaces of…
In recent years, Born-Markov master equations based on tracing out the electromagnetic degrees of freedom have been extensively employed in the description of quantum optical phenomena originating from photon-mediated interactions in…
We develop a new model of laser-matter interaction based on Optical Bloch Equations, which includes photo-ionization, impact ionization, and various relaxation processes typical of dielectric materials. This approach is able to describe the…
We use photoluminescence spectroscopy to investigate the ground state of single self-assembled InGaAs lateral quantum dot molecules. We apply a voltage along the growth direction that allows us to control the total charge occupancy of the…
Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…
Entangled photons exhibit non-classical light-matter interactions that create new opportunities in materials and molecular science. For example, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one…
The work examines the effect of multiple photon emission on the quantum mechanical state of an electron emitting synchrotron radiation and on the intensity of that radiation. Calculations are done with the variant of perturbation theory…
A simple analytical solution for the problem of multiphoton detachment from negative ions by a linearly polarized laser field is found. It is valid in the wide range of intensities and frequencies of the field, from the perturbation theory…
We demonstrate that ultrashort pulses carry the possibility for a new regime of light-matter interaction with nonadiabatic electron processes sensitive to the envelope-derivative of the light pulse. A standard single pulse with its two…
The field of laser-matter interaction traditionally deals with the response of atoms, molecules and plasmas to an external light wave. However, the recent sustained technological progress is opening up the possibility of employing intense…
The photorecombination radiation on a neighbor center of an electron ionized in the nonlinear tunneling regime is discussed. In the framework of the active electron model an analytical solution of the problem has been obtained. The…
Exposing a molecule to intense light pulses may bring this molecule to a nonstationary quantum state, thus launching correlated dynamics of electronic and nuclear subsystems. Although much had been achieved in the understanding of…
Probing optical excitations with nanometer resolution is important for understanding their dynamics and interactions down to the atomic scale. Electron microscopes currently offer the unparalleled ability of rendering spatially-resolved…
We show that if the laser is intense enough, it may always ionize an atom or induce transitions between discrete energy levels of the atom, no matter what is its frequency. It means in the quantum transition of an atom interacting with an…
The motion of electrons and ions in medium-sized rare gas clusters (1000 atoms) exposed to intense laser pulses is studied microscopically by means of classical molecular dynamics using a hierarchical tree code. Pulse parameters for optimum…
Motivated by a revision of the classical equations of electromagnetism that allow for the inclusion of solitary waves in the solution space, the material collected in these notes examines the consequences of adopting the modified model in…
While ballistic electrons are a key tool for applications in sensing and flying qubits, sub-nanosecond propagation times and complicated interactions make control of ballistic single electrons challenging. Recent experiments have revealed…
The crystallization of electrons in quasi low-dimensional solids is studied in a model which retains the full three-dimensional nature of the Coulomb interactions. We show that restricting the electron motion to layers (or chains) gives…