相关论文: On the classical theory of molecular optical activ…
Recently, it was predicted theoretically and verified experimentally that a pair of delayed and cross-polarized short laser pulses can create molecular ensembles with a well defined sense of rotation (clockwise or counterclockwise). Here we…
Classical and quantum correlation functions are derived for a system of non-interacting particles moving on a circle. It is shown that the decaying behaviour of the classical expression for the correlation function can be recovered from the…
Optical activity is the ability of chiral materials to rotate linearly-polarized (LP) electromagnetic waves. Because of their intrinsic asymmetry, traditional chiral molecules usually lack isotropic performance, or at best only possess a…
Conventional scattering theory is incomplete in that it does not adequately describe the behaviour of the wave function at macroscopic distances from the scattering reaction volume. In scattering experiments particles are incident from…
Optical activity is ubiquitous across natural and artificial media and is conventionally understood in terms of scattering from electric and magnetic moments. Here we demonstrate experimentally and confirm numerically a type of optical…
A classical field theory is proposed for the electric current and the electromagnetic field interpolating between microscopic and macroscopic domains. It represents a generalization of the density functional for the dynamics of the current…
Motional narrowing refers to the striking phenomenon where the resonance line of a system coupled to a reservoir becomes narrower when increasing the reservoir fluctuation. A textbook example is found in nuclear magnetic resonance, where…
While optics and mechanics are two distinct branches of physics, they are connected. It is well known that geometrical/ray treatment of light has direct analogies to mechanical descriptions of particle motion. However, connections between…
Molecular chirality plays an important role in chemistry and biology, allows control of biological interactions, affects drugs efficacy and safety, and promotes synthesis of new materials. In general, chirality manifests itself in optical…
Torque is ubiquitous in many molecular systems, including collisions, chemical reactions, vibrations, electronic excitations and especially rotor molecules. We present a straightforward theoretical method based on forces acting on atoms and…
The standard closed-orbit theory is extended for the photodetachment of negative ions in a time-dependent electric field. The time-dependent photodetachment rate is specifically studied in the presence of a single-cycle terahertz pulse,…
The methods of mathematical control theory are widely used in the modern physics, but still they are less popular in quantum science. We will discuss the aspects of control theory, which are the most useful in applications to the real…
We present a theoretical analysis of the connection between classical polarization optics and quantum mechanics of two-level systems. First, we review the matrix formalism of classical polarization optics from a quantum information…
We present a brief review of the classical density functional theory of atomic and molecular fluids. We focus on the application of the theory to the determination of the solvation properties of arbitrary molecular solutes in arbitrary…
The fundamental processes of absorption, stimulated and spontaneous emission, and elastic as well as inelastic scattering involving light and atoms, molecules, and nano-particles have been studied for decades using both classical and…
We demonstrate natural optical activity in disordered ensembles of non-chiral plasmonic resonators. We show that the statistical distributions of rotatory power and spatial dichroism are strongly dependent on the scattering mean free path…
Single-layer transition-metal dichalcogenides provide an unique intrinsic entanglement between the spin/valley/orbital degrees of freedom and the polarization of scattered photons. This scenario gives rise to the well-assessed optical…
We consider the energy averaged two-point correlator of spectral determinants and calculate contributions beyond the diagonal approximation using semiclassical methods. Evaluating the contributions originating from pseudo-orbit correlations…
We consider the quantum kinetic-theory description for interacting massive spin-half fermions using the Wigner function formalism. We derive a general kinetic theory description assuming that the spin effects appear at the classical and…
When light originating from a laser diode driven by non-fluctuating electrical currents is incident on a photo-detector, the photo-current does not fluctuate much. Precisely, this means that the variance of the number of photo-electrons…