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Experimental data obtained with the perovskite compounds Pr$_{0.55}$Sr$_{0.45}$MnO$_{3}$ show that the magnetization decreases with increasing temperature $T$ and undergoes a very sharp phase transition to the paramagnetic phase. The sharp…

材料科学 · 物理学 2024-01-12 Yethreb Essouda , Hung T. Diep , Mohamed Ellouze

The breaking of orbital degeneracy on a transition metal cation and the resulting unequal electronic occupations of these orbitals provide a powerful lever over electron density and spin ordering in metal oxides. Here, we show how to…

A lightly doped perovskite mangantite La_{0.88}Sr_{0.12}MnO_3 exhibits a phase transition at T_{OO}=145 K from a ferromagnetic metal (T_C=172 K) to a novel ferromagnetic insulator.We identify that the key parameter in the transition is the…

强关联电子 · 物理学 2019-08-17 Y. Endoh , K. Hirota , S. Ishihara , S. Okamoto , Y. Murakami , A. Nishizawa , T. Fukuda , H. Kimura , H. Nojiri , K. Kaneko , S. Maekawa

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

Understanding the atomic structure of magnetite-carboxylic acid interfaces is crucial for tailoring nanocomposites involving this interface. We present a Monte Carlo (MC)-based method utilizing iron oxidation state exchange to model…

材料科学 · 物理学 2025-07-08 Emre Gürsoy , Robert H. Meißner , Gregor B. Vonbun-Feldbauer

The three dimensional perovskite manganites in the range of hole-doping $x > 0.5$ are studied in detail using a double exchange model with degenerate $e_g$ orbitals including intra- and inter-orbital correlations and near-neighbour Coulomb…

强关联电子 · 物理学 2009-11-10 Tulika Maitra , A. Taraphder

Neutron spectroscopy was applied to study the magnetic interactions of orbitally degenerate Co$^{2+}$ on a host MgO rocksalt lattice where no long range spin or orbital order exists. The paramagnetic nature of the substituted monoxide…

We investigate a magnetization-dependent voltage that appears at the interface between garnets and various metals. The voltage is even in the applied magnetic field and is dependent on the surface roughness and the pressure holding the…

材料科学 · 物理学 2010-07-09 L. R. Hunter , K. A. Virgien , A. W. Bridges , B. J. Heidenreich , J. E. Gordon , A. O. Sushkov

Investigation of the oxygen-deficient 112-type ordered oxides of the type LnBaCoMnO5+\delta (Ln = Nd, Eu) evidences certain unusual magnetic behavior at low temperatures, compared to the LnBaCo2O5+\delta cobaltites. One observes that the…

材料科学 · 物理学 2015-05-18 Asish K. Kundu , V. Pralong , B. Raveau , V. Caignaert

We calculate the nature of magnetic interactions in transition-metal doped ZnO using the local spin density approximation and LSDA+\textit{U} method of density functional theory. We investigate the following four cases: (i) single…

材料科学 · 物理学 2009-11-11 Priya Gopal , Nicola A. Spaldin

The role of elastic interactions between Jahn-Teller ions in formation of various orbital- and charge-ordered structures in manganites and related compounds is analyzed. It is shown that such interactions alone are often sufficient to…

强关联电子 · 物理学 2009-11-07 D. I. Khomskii , K. I. Kugel

Magnetic and transport properties of the perovskite-type $3d$ transition-metal oxide (La,Sr)MnO$_3$ are theoretically studied using the double-exchange model in infinite dimension. Magnetoresistance properties as well as the magnetic…

凝聚态物理 · 物理学 2009-10-28 Nobuo Furukawa

The nature of magnetic order and transport properties near surfaces is a topic of great current interest. Here we model metal-insulator interfaces with a multi-layer system governed by a tight-binding Hamiltonian in which the interaction is…

强关联电子 · 物理学 2012-06-14 A. Euverte , F. Hébert , S. Chiesa , R. T. Scalettar , G. G. Batrouni

The mechanisms of magnetic and orbital interactions due to double exchange (DE) and superexchange (SE) in transition metal oxides with degenerate e_g orbitals are presented. Specifically, we study the effective spin-orbital models derived…

强关联电子 · 物理学 2009-10-31 A. M. Oles , M. Cuoco , N. B. Perkins

Here we study the electronic properties of cuprate/manganite interfaces. By means of atomic resolution electron microscopy and spectroscopy, we produce a subnanometer scale map of the transition metal oxidation state profile across the…

Roles of Coulomb interaction, orbital degeneracy and Jahn-Teller coupling in double-exchange models are examined for Mn perovskite oxides. We study the undoped Mott insulator as well as metal-insulator transitions by hole doping, and…

强关联电子 · 物理学 2009-10-31 Yukitoshi Motome , Masatoshi Imada

We use ab initio electronic structure calculations in combination with Monte Carlo simulations to investigate the magnetic and ferroelectric properties of bulk orthorhombic HoMnO$_3$ and ErMnO$_3$. Our goals are to explain the…

材料科学 · 物理学 2018-12-12 Natalya S. Fedorova , Amadé Bortis , Christoph Findler , Nicola A. Spaldin

The effect of cobalt and nickel substitutions for manganese on the physical properties of the perovskite manganite La1.2Bi0.8Mn2-x(Ni/Co)xO6+d, with x = 0.0-0.8, has been investigated. It is observed that the ferromagnetism is enhanced, TC…

材料科学 · 物理学 2008-09-04 Asish K. Kundu , R. Ranjith , V. Pralong , V. Caignaert , B. Raveau

Electronic, lattice, and spin interactions at the interfaces between crystalline complex transition metal oxides can give rise to a wide range of functional electronic and magnetic phenomena not found in bulk. At hetero-interfaces, these…

强关联电子 · 物理学 2017-08-03 S. Koohfar , A. S. Disa , M. Marshall , F. J. Walker , C. H. Ahn , D. P. Kumah

The electronic properties of many transition metal oxide systems require new ideas concerning the behaviour of electrons in solids for their explanation. A recent example, subsequent to that of cuprate superconductors, is of rare earth…

强关联电子 · 物理学 2007-05-23 T. V. Ramakrishnan , H. R. Krishnamurthy , S. R. Hassan , G. Venketeswara Pai