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Linearly polarized spectra of far-infrared (IR) transmission in HoMn2O5 multiferroic single crystals have been studied in the frequency range between 8.5 and 105 cm-1 and for temperatures between 5 K and 300 K. Polarization of IR-active…

强关联电子 · 物理学 2009-11-13 A. A. Sirenko , S. M. O Malley , K. H. Ahn , S. Park , G. L. Carr , S-W. Cheong

Far-infrared spectra of magneto-dielectric Dy3Fe5O12 garnet were studied between 13 and 100 cm-1 and at low temperatures between 5 and 80 K. A combination of transmission, reflectivity, and rotating analyzer ellipsometry was used to…

Low energy excitations in the multiferroic material TbMnO3 have been investigated by Raman spectroscopy. Our observations reveal the existence of two peaks at 30 cm-1 and 60 cm-1. They are observed in the cycloidal phase below the Curie…

强关联电子 · 物理学 2010-10-12 P. Rovillain , M. Cazayous , Y. Gallais , A. Sacuto , M-A. Measson , H. Sakata

We report a comprehensive study of the low-level substitution of Mn$^{3+}$ by Fe$^{3+}$ effect on the static and dynamic magnetoelectric coupling in TbMn$_{1-x}$Fe$_x$O$_3$ ($x=0$, 0.02 and 0.04). The cationic substitution has a large…

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

材料科学 · 物理学 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

Our measured dielectric constant and mechanical response of multiferroic BiFeO3 indicate four phase transitions below room temperature. Features correlate with those reported at 50K (from a peak in the zero-field-cooled magnetic…

材料科学 · 物理学 2008-06-23 S. A. T. Redfern , C. Wang , J. W. Hong , G. Catalan , J. F. Scott

We have studied the thermodynamic properties of single-crystalline TbFe3(BO3)4. Magnetization measurements have been carried out as a function of magnetic field (up to 50 T) and temperature up to 350K with the magnetic field both parallel…

We provide a detailed study of the reflectivity of multiferroic TbMnO_3 for wave numbers from 40 cm^{-1} to 1000 cm^{-1} and temperatures 5 K < T < 300 K. Excitations are studied for polarization directions E || a, the polarization where…

强关联电子 · 物理学 2010-01-22 M. Schmidt , Ch. Kant , T. Rudolf , F. Mayr , A. A. Mukhin , A. M. Balbashov , J. Deisenhofer , A. Loidl

In the garnet structure compound Yb3Ga5O12, the Yb3+ ions (ground state effective spin S' = 1/2) are situated on two interpenetrating corner sharing triangular sublattices such that frustrated magnetic interactions are possible. Previous…

凝聚态物理 · 物理学 2009-11-10 J. A. Hodges , P. Bonville , M. Rams , K. Krolas

Single crystals of Nd_{1-x}Pb_{x}MnO_{3} with x=0.2 are grown by high temperature solution growth technique using PbO-PbF_{2} flux. Magnetization studies on the samples show a transition to a ferromagnetic state below T_c ~ 125 K and the…

强关联电子 · 物理学 2009-11-07 Anika Kumar , Nilotpal Ghosh , Janhavi P. Joshi , H. L. Bhat , S. V. Bhat

We have measured the optical conductivity of single crystal LuMnO3 from 10 to 45000 cm-1 at temperatures between 4 and 300 K. A symmetry allowed on-site Mn $d$-$d$ transition near 1.7 eV is observed to blue shift (~0.1 eV) in the…

强关联电子 · 物理学 2009-11-07 A. B. Souchkov , J. R. Simpson , H. D. Drew , M. Quijada , H. Ishibashi , N. Hur , J. S. Ahn , S. W. Cheong , A. J. Millis

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

强关联电子 · 物理学 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

Crystal-field excitations, for example in transition-metal oxides where a rare-earth element is used as a spacer between the transition-metal-oxide tetrahedra and octahedra, are assumed to be extremely robust with respect to external…

Far-infrared optical transmission spectra of the antiferromagnetic resonances, or magnons, and crystal field transitions have been studied in hexagonal REMnO3 (RE = Er, Tm, Yb, Lu) single crystals. The magnon and CF frequencies, their…

材料科学 · 物理学 2015-06-04 E. C. Standard , T. Stanislavchuk , A. A. Sirenko , N. Lee , S. -W. Cheong

Magnetic and magnetoelectric excitations in the multiferroic TbMnO_3 have been investigated at terahertz frequencies. Using different experimental geometries we can clearly separate the electro-active excitations (electromagnons) from the…

强关联电子 · 物理学 2009-03-16 A. Pimenov , A. Shuvaev , A. Loidl , F. Schrettle , A. A. Mukhin , V. D. Travkin , V. Yu. Ivanov , A. M. Balbashov

The magnetic susceptibility between 1.5 and 800 K, the infrared reflectivity at room temperature and the temperature dependence of the dielectric constant at mm-wavelengths are reported for single crystalline BiFeO3. A well developed…

强关联电子 · 物理学 2010-07-22 Jun Lu , M Schmidt , P Lunkenheimer , A Pimenov , A A Mukhin , V D Travkin , A Loidl

The possibility to control the magnetic properties of a material with an electric field at room temperature is highly desirable for modern applications. Moreover, a coupling between magnetic and electric orders within a single material…

We have studied the impact of the magnetic field on the electromagnon excitations in TbMnO3 crystal. Applying magnetic field along the c axis, we show that the electromagnons transform into pure antiferromagnetic modes, losing their polar…

材料科学 · 物理学 2011-07-06 P. Rovillain , M. Cazayous , Y. Gallais , M-A. Measson , A. Sacuto , H. Sakata , M. Mochizuki

The magnetic moment induced by an external magnetic field of 5.8 T on the Co3+ ions in LaCoO3 has been measured by polarized neutron diffraction. Measurements were made at 100 K, near to the spin-state transition, at 1.5 K and at 285 K. The…

强关联电子 · 物理学 2015-06-25 V. P. Plakhty , P. J. Brown , B. Grenier , S. V. Shiryaev , S. N. Barilo , S. V. Gavrilov , E. Ressouche

Low-temperature magnetization (M) measurements down to 0.1 K have been performed in magnetic fields up to 14.5 T for a single piece of a tiny single-crystalline sample (0.2 mg weight) of the spin-gap system YbAl3C3. At the base temperature…

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