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In a recent study of the magnetic properties of rare-earth systems the two extreme situations have been considered in which the crystalline electrostatic field is large or small with respect to the spin-orbit interaction. In the first case…

强关联电子 · 物理学 2010-08-17 Keisuke Hatada , Kuniko Hayakawa , Fabrizio Palumbo

Contrary to the well known spin qubits, rare-earth qubits are characterized by a strong influence of crystal field due to large spin-orbit coupling. At low temperature and in the presence of resonance microwaves, it is the magnetic moment…

强关联电子 · 物理学 2009-11-26 Sylvain Bertaina , J. H. Shim , S. Gambarelli , B. Z. Malkin , B. Barbara

Rare-earth (RE) atoms on top of 2D materials represent an interesting platform with the prospect of tailoring the magnetic anisotropy for practical applications. Here, we investigate the ground state and magnetic properties of selected…

介观与纳米尺度物理 · 物理学 2024-07-25 Johanna P. Carbone , Juba Bouaziz , Gustav Bihlmayer , Stefan Blügel

We have used a many-body model Hamiltonian to study the nature of the magnetic ground state of hetero-binuclear complexes involving rare-earth and copper ions. We have taken into account all diagonal repulsions involving the rare-earth 4f…

强关联电子 · 物理学 2009-11-07 Indranil Rudra , C. Raghu , S. Ramasesha

We review recent theoretical developments about the role of spins, electron-electron interactions, and spin-orbit coupling in metal nanoparticles and semiconductor quantum dots. For a closed system, in the absence of spin-orbit coupling or…

介观与纳米尺度物理 · 物理学 2007-05-23 Yuval Oreg , P. W. Brouwer , X. Waintal , Bertrand I. Halperin

A change of orbital state alters the coupling between ions and their surroundings drastically. Orbital excitations are hence key to understand and control interaction of ions. Rare-earth (RE) elements with strong magneto-crystalline…

The physics of spin-orbit entangled magnetic moments of $4d$ and $5d$ transition metal ions on a honeycomb lattice has been much explored in search for unconventional magnetic orders or quantum spin liquids expected for compass spin models,…

We apply the first-principles density functional theory + dynamical mean field theory framework to evaluate the crystal field splitting on rare earth sites in hard magnetic intermetallics. An atomic (Hubbard-I) approximation is employed for…

强关联电子 · 物理学 2017-11-15 Pascal Delange , Silke Biermann , Takashi Miyake , Leonid Pourovskii

Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…

强关联电子 · 物理学 2015-05-30 Sylvain Petit , Pierre Bonville , Isabelle Mirebeau , Hannu Mutka , Julien Robert

We clarify the role of crystalline electric field (CEF) induced magnetic anisotropy in the ground state and spin-wave spectrum of cubic rare-earth materials with dominating isotropic magnetic exchange interactions. In particular we study…

强关联电子 · 物理学 2009-10-31 Gennadi Uimin , Wolfram Brenig

The magnetic pyrochlore oxide materials of general chemical formula R2Ti2O7 and R2Sn2O7 (R = rare earth) display a host of interesting physical behaviours depending on the flavour of rare earth ion. These properties depend on the value of…

统计力学 · 物理学 2015-06-24 Adrian G. Del Maestro , Michel J. P. Gingras

To efficiently manipulate magnetism is a key physical issue for modern condensed matter physics, which is also crucial for magnetic functional applications. Most previous relevant studies rely on the tuning of spin texture, while the spin…

强关联电子 · 物理学 2020-11-04 Yakui Weng , Xing'ao Li , Shuai Dong

Strong magnetic field pulses associated with a relativistic electron bunch can imprint switching patterns in magnetic thin films that have uniaxial in-plane anisotropy. In experiments with Fe and FeCo alloy films the pattern shape reveals…

介观与纳米尺度物理 · 物理学 2017-02-24 Ioan Tudosa

We have investigated the electronic structure of rare-earth tetraborides, $\textrm{RB}_{4}$, using first-principle electronic structure methods (DFT) implemented in Quantum Espresso (QE). In this article we have studied heather-to neglected…

强关联电子 · 物理学 2023-03-22 Ismail Sk , Nandan Pakhira

Density functional theory (DFT), including its extensions designed to treat strongly correlated localized electron systems such as DFT+$U$ and DFT+dynamical mean field theory, has proven exceedingly useful in studying the magnetic…

材料科学 · 物理学 2025-06-09 Y. Lee , Z. Ning , R. Flint , R. J. McQueeney , I. I. Mazin , Liqin Ke

Magnetic excitations of single atoms on surfaces have been widely studied experimentally in the past decade. Lately, systems with unprecedented magnetic stability started to emerge. Here, we present a general theoretical investigation of…

介观与纳米尺度物理 · 物理学 2018-01-17 Timofey Balashov , Christian Karlewski , Tobias Märkl , Gerd Schön , Wulf Wulfhekel

We report inelastic neutron scattering measurements of crystal field transitions in PrFeAsO, PrFeAsO0.87F0.13, and NdFeAsO0.85F0.15. Doping with fluorine produces additional crystal field excitations, providing evidence that there are two…

We study the rare-earth magnets on a honeycomb lattice, and are particularly interested in the experimental consequences of the highly anisotropic spin interaction due to the spin-orbit entanglement. We perform a high-temperature series…

强关联电子 · 物理学 2020-10-06 Zhu-Xi Luo , Gang Chen

We consider the spin correlation functions for rare-earth compounds in their paramagnetic state with the aim to understand the temperature dependence of the quasi-elastic and crystal-field linewidths and the spin-lattice relaxation rates…

材料科学 · 物理学 2009-12-21 A. Yaouanc

Rare-earth materials hold promise to realize exotic magnetic states owing to synergy between electron correlations and spin-orbit coupling. Recently, quasi-two-dimensional honeycomb magnets $A_2$PrO$_3$ ($A$ = alkali metals) were predicted…

强关联电子 · 物理学 2024-10-11 Seong-Hoon Jang , Yukitoshi Motome
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