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High harmonic generation in benzene is studied using a mixed quantum-classical approach in which the electrons are described using time-dependent density functional theory while the ions move classically. The interaction with both…

原子物理 · 物理学 2016-03-02 Abigail Wardlow , Daniel Dundas

We investigate the mechanism of damping and heating of trapped ions associated with the polarization of the residual background gas induced by the oscillating ions themselves. Reasoning by analogy with the physics of surface electrons in…

量子物理 · 物理学 2009-11-07 R. M. Serra , N. G. de Almeida , W. B. da Costa , M. H. Y. Moussa

We discuss the possibility of non-exponential tunneling ionization of atoms irradiated by intense laser field. This effect can occur at times, which are greater than the lifetime of a system under consideration. The mechanism for…

原子物理 · 物理学 2015-03-02 A. M. Ishkhanyan , V. P. Krainov

At high energies, in particle-capture processes between ions and atoms, classical kinematic requirements show that generally double collision Thomas processes dominate. However, for certain mass-ratios these processes are kinematically…

原子物理 · 物理学 2015-05-18 John H. Carter , Michael Lieber

Recent experiments have shown the transfer of orbital angular momentum (OAM) from a non-resonant laser onto an exciton-polariton condensate, despite earlier views that the phase information of such a laser should be lost during the process…

介观与纳米尺度物理 · 物理学 2022-05-16 Huawen Xu , Kevin Dini , Xingran Xu , Rimi Banerjee , Subhaskar Mandal , Timothy C. H. Liew

We discuss a parity nonconserving asymmetry in the cross section of KLL dielectronic recombination of polarized electrons on the hydrogen-like ions with $Z \lesssim 60$. This effect is strongly enhanced because of the near-degeneracy of…

原子物理 · 物理学 2009-09-01 G. F. Gribakin , F. J. Currell , M. G. Kozlov , A. I. Mikhailov

With a classical ensemble model that including electron correlations during the whole ionization process, we investigated strong-field sequential double ionization of Ar by elliptically polarized pulses at the quantitative level. The…

原子物理 · 物理学 2015-06-04 Yueming Zhou , Cheng Huang , Qing Liao , Peixiang Lu

The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with…

We study double ionization of Mg by electron impact through the vantage point of classical mechanics. We consider all electron-electron correlations in a Coulomb four-body problem, where three electrons belong to the atom and the fourth…

原子物理 · 物理学 2020-07-01 Shivan Mittal , Jonathan Dubois , Cristel Chandre , Ahmet Turgay Uzer

Complexation in symmetric solutions of oppositely charged polyelectrolytes is studied theoretically. We include polyion crosslinking due to formation of thermoreversible ionic pairs. The electrostatic free energy is calculated within the…

软凝聚态物质 · 物理学 2009-11-10 Alexander Kudlay , Alexander V. Ermoshkin , Monica Olvera de la Cruz

Quantum calculations of a 1+1-dimensional model for double ionization in strong laser fields are used to trace the time evolution from the ground state through ionization and rescattering to the two electron escape. The subspace of…

原子物理 · 物理学 2009-11-13 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

We study the nonlinear and resonant process of two-photon ionization of atoms (He and H) in a pump-probe scheme. The pump pulse prepares the quantum system in a superposition of the ground state and an excited bound state. By varying the…

Microscopic cascading of second-order nonlinearities between two molecules has been proposed to yield an enhanced third-order molecular nonlinear-optical response. In this contribution, we investigate the two-molecule cascaded second…

Elliptical dichroism is known in atomic photoionization as the difference in the photoelectron angular distributions produced in nonlinear ionization of atoms by left- and right-handed elliptically polarized light. We theoretically…

原子物理 · 物理学 2018-08-07 J. Hofbrucker , A. V. Volotka , S. Fritzsche

Ionization collisions have important consequences in many physical phenomena, and the mechanism that leads to ionization is not universal. Double differential cross sections (DDCSs) are often used to identify ionization mechanisms because…

原子物理 · 物理学 2022-02-23 A. Plumadore , A. L. Harris

We theoretically demonstrate a scheme for tomographic reconstruction of asymmetric molecular orbitals based on high-order harmonic generation with a two-color multicycle laser field. It is shown that by adjusting the relative phase of the…

原子物理 · 物理学 2013-12-30 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Peixiang Lu

We present a simple and general coherence model for multiorbital tunnel ionization of molecules, which we incorporate into our previously developed density matrix approach for sequential double ionization [Yuen and Lin, Phys. Rev. A 106,…

原子物理 · 物理学 2023-09-07 C. H. Yuen , C. D. Lin

The tunneling model of ionization applies only to longitudinal fields: quasistatic electric fields that do not propagate. Laser fields are transverse: plane wave fields that possess the ability to propagate. Although there is an approximate…

原子物理 · 物理学 2015-06-19 H. R. Reiss

We present the theory of a new method to slow a linearly polarized probe pulse as it propagates through a duplicated two-level system driven by an orthogonally polarized control field. The method makes use of Zeeman coherence oscillations…

光学 · 物理学 2009-11-13 F. A. Hashmi , M. A. Bouchene

We have probed the fragmentation dynamics in a bent triatomic molecule, water, a non-planar molecule, methanol, and a planar ring-structured molecule, benzene, using 100 fs duration pulses of linearly and circularly polarized, infrared,…

原子物理 · 物理学 2009-11-10 F A Rajgara , M Krishnamurthy , D Mathur
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