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相关论文: Kinetic Heterogeneities at Dynamical Crossovers

200 篇论文

In this paper the phenomenon of dynamic heterogeneity in supercooled liquid systems is considered in terms of the recently proposed gauge theory of glass transition. The physical interpretation of the dynamic scaling is considered. It is…

统计力学 · 物理学 2015-06-23 Mikhail Vasin

A two-dimensional bidisperse granular fluid is shown to exhibit pronounced long-ranged dynamical heterogeneities as dynamical arrest is approached. Here we focus on the most direct approach to study these heterogeneities: we identify…

无序系统与神经网络 · 物理学 2017-10-27 Karina E. Avila , Horacio E. Castillo , Katharina Vollmayr-Lee , Annette Zippelius

We examine the phenomenon of dynamical heterogeneity in computer simulations of an equilibrium, glass-forming liquid. We describe several approaches to quantify the spatial correlation of single-particle motion, and show that spatial…

软凝聚态物质 · 物理学 2009-09-25 Sharon C. Glotzer , Claudio Donati

Molecular dynamics simulations are performed to investigate heterogeneous dynamics in amorphous glassy materials under oscillatory shear strain. We consider three-dimensional binary Lennard-Jones mixture well below the glass transition…

软凝聚态物质 · 物理学 2013-05-10 Nikolai V. Priezjev

Molecular dynamics simulations are performed to study spatially heterogeneous dynamics in a model of viscous silica above and below the critical temperature of the mode coupling theory, $T_{MCT}$. Specifically, we follow the evolution of…

软凝聚态物质 · 物理学 2009-11-10 M. Vogel , S. C. Glotzer

One of the most controversial hypotheses for explaining the heterogeneous dynamics of glasses postulates the temporary coexistence of two phases characterized by a high and by a low diffusivity. In this scenario, two phases with different…

软凝聚态物质 · 物理学 2015-07-16 R. Pastore , A. Coniglio , M. Pica Ciamarra

As approaching the glass transition, particle motion in liquids becomes highly heterogeneous and regions with virtually no mobility coexist with liquid-like domains. This complex dynamics is believed to be responsible for different…

软凝聚态物质 · 物理学 2018-03-28 F. Puosi , N. Jakse , A. Pasturel

Clusters of fast and slow correlated particles, identified as dynamical heterogeneities (DHs), con-stitute a central aspect of glassy dynamics. A key ingredient of the glass transition scenario is asignificant increase of the cluster size…

软凝聚态物质 · 物理学 2015-09-11 Rémy Colin , Ahmed Alsayed , Cyprien Gay , Bérengère Abou

We numerically study the aging properties of the dynamical heterogeneities in the Ising spin glass. We find that a phase transition takes place during the aging process. Statics-dynamics correspondence implies that systems of finite size in…

We compare dynamical heterogeneities in equilibrated supercooled liquids and in the nonequilibrium glassy state within the framework of the random first order transition theory. Fluctuating mobility generation and transport in the glass are…

统计力学 · 物理学 2014-01-21 Apiwat Wisitsorasak , Peter G. Wolynes

We perform extensive numerical simulations of a paradigmatic model glass former, the hard-sphere fluid with 10% polydispersity. We sample from the ensemble of trajectories with fixed observation time, whereby single trajectories are…

统计力学 · 物理学 2020-01-28 Matteo Campo , Thomas Speck

We develop a transferable machine learning model which predicts structural relaxation from amorphous supercooled liquid structures. The trained networks are able to predict dynamic heterogeneity across a broad range of temperatures and time…

软凝聚态物质 · 物理学 2024-02-27 Gerhard Jung , Giulio Biroli , Ludovic Berthier

Dynamical heterogeneity, in which transitory local fluctuations occur in the conformation and dynamics of constituent particles, is widely hypothesized to be essential to evolution of supercooled liquids into the structural glass state. Yet…

The presence of dynamical heterogeneities, i.e. nanometer-scale regions containing molecules rearranging cooperatively at very different rates compared to the bulk, is increasingly being recognized as crucial in our understanding of the…

无序系统与神经网络 · 物理学 2015-06-25 Horacio E. Castillo , Azita Parsaeian

In this paper we consider in detail the properties of dynamical heterogeneity in lattice glass models (LGMs). LGMs are lattice models whose dynamical rules are based on thermodynamic, as opposed to purely kinetic, considerations. We devise…

统计力学 · 物理学 2012-10-02 Richard K. Darst , David R. Reichman , Giulio Biroli

We experimentally study the vicinity of the Jamming transition by investigating the statics and the dynamics of the contact network of an horizontally shaken bi-disperse packing of photo-elastic discs. Compressing the packing very slowly,…

软凝聚态物质 · 物理学 2015-06-04 C. Coulais , R. P. Behringer , O. Dauchot

Slow relaxation and plastic deformation in disordered materials such as metallic glasses and supercooled liquids occur at dynamical heterogeneities, or neighboring particles that rearrange in a correlated, cooperative manner. Dynamical…

统计力学 · 物理学 2022-05-20 Charles K. C. Lieou , Takeshi Egami

We investigate the heterogeneous dynamics in a model, where chemical gelation and glass transition interplay, focusing on the dynamical susceptibility. Two independent mechanisms give raise to the correlations, which are manifested in the…

软凝聚态物质 · 物理学 2017-05-09 Antonio de Candia , Annalisa Fierro , Raffaele Pastore , Massimo Pica Ciamarra , Antonio Coniglio

Many amorphous glassy materials exhibit complex spatio-temporal mechanical response and rheology, characterized by an intermittent stress-strain response and a fluctuating velocity profile. Under quasistatic and athermal deformation…

软凝聚态物质 · 物理学 2010-02-01 Michel Tsamados

We study the glass transition by exploring a broad class of kinetic rules that can significantly modify the normal dynamics of super-cooled liquids, while maintaining thermal equilibrium. Beyond the usual dynamics of liquids, this class…

软凝聚态物质 · 物理学 2024-06-14 Cristina Gavazzoni , Carolina Brito , Matthieu Wyart