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We study the effect of electron-vibron interactions on the inelastic transport properties of single-molecule nanojunctions. We use the non-equilibrium Green's functions technique and a model Hamiltonian to calculate the effects of…

介观与纳米尺度物理 · 物理学 2015-03-19 L. K. Dash , H. Ness , R. W. Godby

We present an application of a new formalism to treat the quantum transport properties of fully interacting nanoscale junctions [Phys. Rev. B {\bf 84}, 235428 (2011)]. We consider a model single-molecule nanojunction in the presence of two…

介观与纳米尺度物理 · 物理学 2012-10-15 H. Ness , L. K. Dash

We present an application of a new formalism to treat the quantum transport properties of fully interacting nanoscale junctions. We consider a model single-molecule nanojunction in the presence of two kinds of electron-vibron interactions.…

介观与纳米尺度物理 · 物理学 2013-04-08 H. Ness , L. K. Dash

Quantum transport through single molecules is essentially affected by molecular vibrations. We investigate the behavior of the prototype single-level model with intermediate electron-vibron coupling and arbitrary coupling to the leads. We…

介观与纳米尺度物理 · 物理学 2009-11-13 Dmitry A. Ryndyk , Gianaurelio Cuniberti

We consider the nonequilibrium quantum vibrations of a molecule clamped between two macroscopic leads in a current-carrying state at finite voltages. Our approach is based on the nonequilibrium Green function technique and the…

介观与纳米尺度物理 · 物理学 2007-05-23 D. A. Ryndyk , M. Hartung , G. Cuniberti

Vibrational nonequilibrium effects in charge transport through single-molecule junctions are investigated. Focusing on molecular bridges with multiple electronic states, it is shown that electronic-vibrational coupling triggers a variety of…

介观与纳米尺度物理 · 物理学 2011-03-15 R. Härtle , C. Benesch , M. Thoss

The interaction between electronic and vibrational degrees of freedom is an important mechanism in nonequilibrium charge transport through molecular nanojunctions. While adiabatic polaron-type coupling has been studied in great detail, new…

介观与纳米尺度物理 · 物理学 2022-06-10 Christoph Kaspar , André Erpenbeck , Jakob Bätge , Christian Schinabeck , Michael Thoss

The interaction between electronic and vibrational degrees of freedom in single-molecule junctions may result from the dependence of the electronic energies or the electronic states of the molecular bridge on the nuclear displacement. The…

介观与纳米尺度物理 · 物理学 2015-06-09 A. Erpenbeck , R. Härtle , M. Thoss

The role of multimode vibrational dynamics in electron transport through single molecule junctions is investigated. The study is based on a generic model, which describes charge transport through a single molecule that is attached to metal…

介观与纳米尺度物理 · 物理学 2010-10-26 R. Härtle , C. Benesch , M. Thoss

We investigate the role of electronic-vibrational coupling in resonant electron transport through single-molecule junctions, taking into account that the corresponding coupling strengths may depend on the charge and excitation state of the…

介观与纳米尺度物理 · 物理学 2016-03-23 Andre Erpenbeck , Rainer Härtle , Michel Bockstedte , Michael Thoss

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

介观与纳米尺度物理 · 物理学 2013-02-18 R. Härtle , M. Butzin , M. Thoss

The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to…

介观与纳米尺度物理 · 物理学 2017-02-01 A. Ueda , Y. Utsumi , Y. Tokura , O. Entin-Wohlman , A. Aharony

Vibronic effects in resonant electron transport through single-molecule junctions are analyzed. The study is based on generic models for molecular junctions, which include electronic states on the molecular bridge that are vibrationally…

介观与纳米尺度物理 · 物理学 2011-03-15 R. Härtle , M. Thoss

We investigate the non-equilibrium transport properties of a disordered molecular nanowire. The nanowire is regarded as a quasi-one-dimensional organic crystal composed of self-assembled molecules. One orbital and a single random energy are…

介观与纳米尺度物理 · 物理学 2017-06-07 P. Thiessen , E. Diaz , R. A. Roemer , F. Dominguez-Adame

Quantum interference effects and decoherence mechanisms in single-molecule junctions are analyzed employing a nonequilibrium Green's function approach. Electrons tunneling through quasi-degenerate states of a nanoscale molecular junction…

介观与纳米尺度物理 · 物理学 2011-07-25 R. Härtle , M. Butzin , O. Rubio-Pons , M. Thoss

We analyze how functionality could be obtained within single-molecule devices by using a combination of non-equilibrium Green's functions and ab-initio calculations to study the inelastic transport properties of single-molecule junctions.…

介观与纳米尺度物理 · 物理学 2015-06-03 L. K. Dash , H. Ness , M. J. Verstraete , R. W. Godby

We propose a simple scheme that describes accurately essential non-equilibrium effects in nanoscale electronics devices using equilibrium transport theory. The scheme, which is based on the alignment and dealignment of the junction…

介观与纳米尺度物理 · 物理学 2012-10-01 V. M. García-Suárez , J. Ferrer

In the present work, we theoretically analyze the steady-state thermoelectric transport through a single-molecule junction with a vibrating bridge. Thermally induced charge current in the system is explored using a nonequilibrium Green's…

介观与纳米尺度物理 · 物理学 2016-06-21 Natalya A. Zimbovskaya

We investigate chemical bond formation and conductance in a molecular C60-junction under finite bias voltage using first-principles calculations based on density functional theory and nonequilibrium Green's functions (DFT-NEGF). At the…

介观与纳米尺度物理 · 物理学 2013-02-04 Søren Ulstrup , Thomas Frederiksen , Mads Brandbyge

The influence of vibrational motion on electron conduction through single molecules bound to metal electrodes is investigated employing first-principles electronic-structure calculations and projection-operator Green's function methods.…

介观与纳米尺度物理 · 物理学 2009-11-11 C. Benesch , M. Thoss , W. Domcke , M. Cizek
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