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We investigate the bulk magnetic, electron paramagnetic resonance, and magneto-optical properties of {Ni4Mo12}, a magnetic molecule with antiferromagnetically coupled tetrahedral {Ni4Mo12} in a diamagnetic molybdenum matrix. The…

Magnetic excitations in a Ni$_4$ magnetic molecule were investigated by inelastic neutron scattering and bulk susceptibility ($\chi_\text{bulk}$) techniques. The magnetic excitation spectrum obtained from the inelastic neutron scattering…

强关联电子 · 物理学 2015-06-04 K. Iida , S. -H. Lee , T. Onimaru , K. Matsubayashi , T. J. Sato

Inelastic neutron scattering provides a powerful probe of the magnetic excitations of quantum magnets. Altermagnets have recently emerged as a new class of magnets with vanishing net magnetization characteristic of antiferromagnets and with…

强关联电子 · 物理学 2023-09-29 Thomas A. Maier , Satoshi Okamoto

We present results of inelastic neutron scattering experiments performed for the compound Magnetic and neutron spectroscopic properties of the tetrameric nickel compound $[Mo_{12}O_{28}(\mu_2-OH)_9(\mu_3-OH)_3{Ni(H_2O)_3}_4] $\cdot$…

强关联电子 · 物理学 2015-05-18 A. Furrer , K. W. Krämer , Th. Strässle , D. Biner , J. Hauser , H. -U. Güdel

A high resolution inelastic neutron scattering (INS) study of fully deuterated Mn$_{12}$-acetate provides the most accurate spin Hamiltonian parameters for this prototype single molecule magnet so far. The Mn$_{12}$-clusters deviate from…

强关联电子 · 物理学 2009-11-10 Roland Bircher , Gregory Chaboussant , Andreas Sieber , Hans U. Guedel , Hannu Mutka

Magnetic properties of a tetrahedral "Ni_4" molecule are discussed in terms of the Heisenberg model, with magnetic anisotropy terms included, and on the basis of first-principle calculations within the density functional theory. It is shown…

材料科学 · 物理学 2007-05-23 A. V. Postnikov , M. Brueger , J. Schnack

Single crystal inelastic neutron scattering is used to study spin wave excitations in the fully polarized state of the frustrated quantum ferro-antiferromagnet BaCdVO(PO$_4$)$_2$. The data analysis is based on a Heisenberg spin Hamiltonian…

强关联电子 · 物理学 2021-04-07 V. K. Bhartiya , S. Hayashida , K. Yu. Povarov , Z. Yan , Y. Qiu , S. Raymond , A. Zheludev

Molecular Nanomagnets have attracted the attention of the scientific community since the rich physics behind their magnetic behaviour make them ideal test-beds for fundamental concepts in quantum mechanics. Sophisticated experiments and…

介观与纳米尺度物理 · 物理学 2021-01-19 Elena Garlatti , Alessandro Chiesa , Tatiana Guidi , Giuseppe Amoretti , Paolo Santini , Stefano Carretta

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Molecular nanomagnets are among the first examples of spin systems of finite size and have been test-beds for addressing a range of elusive but important phenomena in quantum dynamics. In fact, for short-enough timescales the spin…

介观与纳米尺度物理 · 物理学 2015-06-11 M. L. Baker , T. Guidi , S. Carretta , J. Ollivier , H. Mutka , H. U. Güdel , G. A. Timco , E. J. L. McInnes , G. Amoretti , R. E. P. Winpenny , P. Santini

Inelastic neutron scattering is used to investigate magnetic excitations in the quasi-one-dimensional quantum spin-liquid system Cu2Cl4 D8C4SO2. Contrary to previously conjectured models that relied on bond-alternating nearest neighbor…

强关联电子 · 物理学 2007-11-14 V. O. Garlea , A. Zheludev , L. -P. Regnault , J. -H. Chung , Y. Qiu , M. Boehm , K. Habicht , M. Meissner

Inelastic neutron scattering (INS) experiments have been performed on the Cu$_3$ triangular molecular nanomagnet using powder samples. In the medium resolution INS spectrum measured, there are two peaks at $\hbar\omega=0.5$ and 0.6 meV.…

其他凝聚态物理 · 物理学 2015-05-19 Kazuki Iida , Yiming Qiu , Taku J Sato

Inelastic neutron scattering has been applied to the study of the spin dynamics of Cr-based antiferromagnetic octanuclear rings where a finite total spin of the ground state is obtained by substituting one Cr(III) ion (s = 3/2) with Zn (s =…

We performed inelastic neutron scattering measurements on single crystals of NdFe$_{3}$($^{11}$BO$_{3}$)$_{4}$ to explore the magnetic excitations, to establish the underlying Hamiltonian, and to reveal the detailed nature of hybridization…

强关联电子 · 物理学 2015-07-23 S. Hayashida , M. Soda , S. Itoh , T. Yokoo , K. Ohgushi , D. Kawana , H. M. Rønnow , T. Masuda

We report inelastic and elastic neutron scattering, magnetic susceptibility, and heat capacity measurements of polycrystalline sodium ruthenate (Na$_3$RuO$_4$). Previous work suggests this material consists of isolated tetramers of $S=3/2$…

In this paper we report results for magnetic observables of finite spin clusters composed of S=1/2 ions. We consider clusters of two, three and four spins in distinct spatial arrangements, with isotropic Heisenberg interactions of various…

强关联电子 · 物理学 2009-11-10 J. T. Haraldsen , T. Barnes , J. L. Musfeldt

Inelastic neutron scattering has been used to determine the microscopic Hamiltonian describing two high-spin variants of the high-anisotropy Mn$_6$ nanomagnet. The energy spectrum of both systems is characterized by the presence of several…

Inelastic neutron scattering experiments have been carried out on a powder sample of Cu2PO4OH, which consists of diamond-shaped tetramer spin units with S=1/2. We have observed two nearly dispersionless magnetic excitations at E1~12 and…

材料科学 · 物理学 2015-12-09 M. Matsuda , S. E. Dissanayake , D. L. Abernathy , K. Totsuka , A. A. Belik

We investigate the spectroscopic magnetic excitations in molecular magnets with complex intermediate structure among the magnetic ions. Our approach consists in introducing a modified spin Hamiltonian that allows for discrete coupling…

强关联电子 · 物理学 2019-09-02 M. Georgiev , H. Chamati

In this communication we consider the doping dependence of the strong antiferromagnetic spin fluctuations in the cuprate superconductors. We investigate the effect of an incommensurate magnetic response, as recently observed in inelastic…

超导电性 · 物理学 2016-08-15 Dirk K. Morr , Jörg Schmalian , David Pines
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