相关论文: Deflection of field-free aligned molecules
We consider optical properties of a gas of molecules that are brought to fast unidirectional spinning by a pulsed laser field. It is shown that a circularly polarized probe light passing through the medium inverts its polarization…
Supersonic beams of polar molecules are deflected using inhomogeneous electric fields. The quantum-state selectivity of the deflection is used to spatially separate molecules according to their quantum state. A detailed analysis of the…
Semiclassical catastrophes in the dynamics of a quantum rotor (molecule) driven by a strong time-varying field are considered. We show that for strong enough fields, a sharp peak in the rotor angular distribution can be achieved via…
We provide a theoretical analysis for the intermediate scattering function typically measured in depolarized dynamic light scattering experiments. We calculate the field autocorrelation function $g_1^{\rm VH}(Q,t)$ in dependence on the wave…
Photoelectron angular distributions (PADs) of oriented polar molecules in response to different polarized lasers are systematically investigated. It is found that the PADs of polar CO molecules show three distinct styles excited by…
We use an optical centrifuge to align asymmetric top $\mathrm{SO_2}$ molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the rotating frame confines sulfur atoms to the plane of the…
We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…
The control of ultrafast molecular rotational motion has benefited from the development of innovative techniques in strong-field laser physics. Here, we theoretically demonstrate a novel type of coherent control by inducing rotation of an…
We consider electron-atom scattering in a circularly polarized laser field at sufficiently high electron energies, permitting to describe the scattering process by the first order Born approximation. Assuming the radiation field has…
A new technique based on superposition of two speckle patterns is proposed and demonstrated for controlled modulation of the spatial polarization distribution of the resultant speckle. It is demonstrated both theoretically and…
We demonstrate experimentally a method of varying the degree of directionality in laser-induced molecular rotation. To control the ratio between the number of clockwise and counter-clockwise rotating molecules (with respect to a fixed…
Scattering of starlight by dust, molecules and electrons in spiral galaxies will produce a modification of the direct intensity and a polarization in the observed light. We treat the case where the distribution of scatterers can be…
We study the scattering properties of optical dipole-mode vector solitons recently predicted theoretically and generated in a laboratory. We demonstrate that such a radially asymmetric composite self-trapped state resembles ``a molecule of…
We show that the polarization state of coherent light propagating through an optically thick multiple-scattering medium, can be controlled by wavefront shaping, i.e. by controlling only the spatial phase of the incoming field with a spatial…
We report the first experimental observation of non-adiabatic field-free orientation of a heteronuclear diatomic molecule (CO) induced by an intense two-color (800 and 400 nm) femtosecond laser field. We monitor orientation by measuring…
Freely oriented small anisotropic grains and molecules depolarize radiation both in single scattering and in the process of multiple scattering. Especially large depolarization occurs for resonant scattering corresponding to the electron…
We have investigated the angle-resolved ATI spectrum of oriented molecules in the IR+XUV co-rotating circular laser fields. According to the different roles of IR and XUV laser in the ionization process, we purposefully adjust the photon…
We present a theoretical investigation of the resonant elastic scattering of laser photons by ultra-relativistic partially stripped ions, that is the core process of the Gamma Factory project. Special emphasis in our study is placed on the…
The mixed-field orientation of an asymmetric-rotor molecule with its permanent dipole moment non-parallel to the principal axes of polarizability is investigated experimentally and theoretically. We find that for the typical case of a…
Linear scattering processes are usually described as a function of the parameters of the incident beam. The wavelength, the intensity distribution, the polarization or the phase are among them. Here, we discuss and experimentally…