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We discuss the discrepancy between the measured optical Drude weight and band structure calculations in LaFePO and other iron-based superconductors. This discrepancy is mostly due to mass renormalization arising from electronic correlation…

超导电性 · 物理学 2010-01-06 M. M. Qazilbash , J. J. Hamlin , R. E. Baumbach , Lijun Zhang , D. J. Singh , M. B. Maple , D. N. Basov

Electronic interactions in multiorbital systems lead to non-trivial features in the optical spectrum. In iron superconductors the Drude weight is strongly suppressed with hole-doping. We discuss why the common association of the…

强关联电子 · 物理学 2014-09-22 M. J. Calderón , L. de' Medici , B. Valenzuela , E. Bascones

Recent measurements of Fermi surface with de Haas-van Alphen oscillations in LaFePO showed a shrinking of the Fermi pockets with respect to first-principle LDA calculations, suggesting an energy shift of the hole and electrons bands with…

超导电性 · 物理学 2009-07-24 L. Ortenzi , E. Cappelluti , L. Benfatto , L. Pietronero

These brief comments on the article in Phys. Rev. B 93, 155116 (2016), address an inadvertent misrepresentation of the capabilities of density functional theory (DFT) and of its local density approximation (LDA) in describing electronic and…

材料科学 · 物理学 2016-10-18 Diola Bagayoko , Yacouba Issa Diakité , Chinedu E. Ekuma , Lashounda Franklin

We present an approach that combines the local density approximation (LDA) and the dynamical mean-field theory (DMFT) in the framework of the full-potential linear augmented plane waves (FLAPW) method. Wannier-like functions for the…

The effects of electron-electron correlations on the low-energy electronic structure and their relationship with unconventional superconductivity are central aspects in the research on the iron-based pnictide superconductors. Here we use…

We present the results of extended theoretical LDA+DMFT calculations for a new iron-pnictide high temperature superconductor NaFeAs compared with the recent high quality angle-resolved photoemission (ARPES) experiments on this system [1].…

强关联电子 · 物理学 2016-03-11 I. A. Nekrasov , N. S. Pavlov , M. V. Sadovskii

LDA+DMFT (Local Density Approximation combined with Dynamical Mean-Field Theory) computation scheme has been used to calculate spectral properties of LaFeAsO -- the parent compound of the new high-T_c iron oxypnictides. The average Coulomb…

强关联电子 · 物理学 2009-06-18 V. I. Anisimov , E. Z. Kurmaev , A. Moewes , I. A. Izyumov

Deviations of low-energy electronic structure of iron-based superconductors from density functional theory predictions have been parametrized in terms of band- and orbital-dependent mass renormalizations and energy shifts. The former have…

Correlated electron systems often show strong bosonic fluctuations, e.g., of antiferromagnetic nature, around a large wave vector such as $\mathbf{q}=(\pi,\pi\ldots)$. These fluctuations can give rise to vertex corrections to the optical…

强关联电子 · 物理学 2025-04-29 J. Krsnik , O. Simard , P. Werner , A. Kauch , K. Held

Accurate treatment of amide resonance is important in electronic structure calculation of protein, for Resonance-Assisted Hydrogen Bonding in the hydrogen bonded chains of backbone amides of protein secondary structures such as beta sheets…

化学物理 · 物理学 2016-10-03 John N. Sharley

Scattering by slowly fluctuating degrees of freedom can cause a transient localization of the current-carrying electrons in metals, driving the system away from normal metallic behavior. We illustrate and characterize this general…

强关联电子 · 物理学 2021-08-25 S. Fratini , S. Ciuchi

We explore the anisotropy in low frequency conductivity as a function of hole doping in multiorbital models of pnictides by analyzing the Drude weight in the $x$ and $y$ directions of a ($\pi$, 0) spin-density wave state. A reduction in the…

强关联电子 · 物理学 2018-11-28 Dheeraj Kumar Singh , Pinaki Majumdar

We have investigated the electron correlation effect on the electronic structures and transport properties of the iron-based superconductors using the density functional theory (DFT) and dynamical mean field theory (DMFT). By considering…

强关联电子 · 物理学 2011-08-19 Hyo Seok Ji , Geunsik Lee , Ji Hoon Shim

We carried out combined transport and optical measurements for BaFe2As2 and five isostructural transition-metal (TM) pnictides. The low-energy optical conductivity spectra of these compounds are, to a good approximation, decomposed into a…

Plutonium is a critically important material as the behavior of its 5f-electrons stands midway between the metallic-like itinerant character of the light actinides and localized atomic-core-like character of the heavy actinides. The…

强关联电子 · 物理学 2020-07-01 Roxanne Tutchton , Wei-ting Chiu , R. C. Albers , G. Kotliar , Jian-Xin Zhu

In correlated metals derived from Mott insulators, the motion of an electron is impeded by Coulomb repulsion due to other electrons. This phenomenon causes a substantial reduction in the electron's kinetic energy leading to remarkable…

强关联电子 · 物理学 2015-05-14 M. M. Qazilbash , J. J. Hamlin , R. E. Baumbach , Lijun Zhang , D. J. Singh , M. B. Maple , D. N. Basov

Electronic correlations in the Fe-pnictide BaFe2As2 are explored within LDA+DMFT, the combination of density functional theory with dynamical mean-field theory. While the correlated band structure is substantially renormalized there is only…

To perform a local orbital analysis of electronic and magnetic interactions, we construct the Wannier functions (WFs) of the Fe $3d$ orbitals in the parent compound of the recently discovered iron pnictide superconductors, LaFeAsO, and a…

超导电性 · 物理学 2010-07-20 Z. P. Yin , W. E. Pickett

By combining DFT-based computational analysis and symmetry constraints in terms of group-subgroup relations, we analysed the formation of the native crystalline structure of loellingite FeAs$_2$. We showed that the ground state of the…

材料科学 · 物理学 2016-03-10 A. Pishtshev , P. Rubin
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