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Neutron powder diffraction measurements, combined with magnetization and resistivity data, have been carried out in the doped perovskite La$_{1-x}$Ca$_x$MnO$_3$ ($x=0.47$, 0.50, and 0.53) to elucidate the structural, magnetic, and…

强关联电子 · 物理学 2009-10-31 Q. Huang , J. W. Lynn , R. W. Erwin , A. Santoro , D. C. Dender , V. N. Smolyaninova , K. Ghosh , R. L. Greene

We show that the valence electrons of Ba3NaRu2O9, which has a quasi-molecular structure, completely crystallize below 210 K. Using an extended Hubbard model, we show that the charge ordering instability results from long-range Coulomb…

We investigated the crystal structure, magnetic behavior, and optical properties of the layered honeycomb compound Na2Cu2TeO6. X-ray and neutron diffraction confirmed a monoclinic structure, with Cu ions arranged in dimerized chains.…

强关联电子 · 物理学 2025-08-25 Shubham Patil , S. D. Kaushik

We have investigated the electronic structure of CaCu3Ru4O12 and LaCu3Ru4O12 using soft x-ray photoelectron and absorption spectroscopy together with band structure and cluster configuration interaction calculations. We found the Cu to be…

强关联电子 · 物理学 2015-06-12 N. Hollmann , Z. Hu , A. Maignan , A. Günther , L. -Y. Jang , A. Tanaka , H. -J. Lin , C. T. Chen , P. Thalmeier , L. H. Tjeng

The structural, electrical transport and magnetic properties of perovskite oxides La1-xTexMnO3 have been investigated and thus the magnetic phase diagram of La1-xTexMnO3 compounds as a function of temperature and the doping level x has been…

强关联电子 · 物理学 2007-05-23 J. Yang , W. H. Song , Y. Q. Ma , R. L. Zhang , B. C. Zhao , Z. G. Sheng , G. H. Zheng , J. M. Dai , Y. P. Sun

Magnetic fluctuations in transition metal oxides are a subject of intensive research because of the key role they are expected to play in the transition from the Mott insulator to the unconventional metallic phase of these materials, and…

强关联电子 · 物理学 2016-01-06 J. Gunasekera , L. Harriger , A. Dahal , T. Heitmann , G. Vignale , D. K. Singh

We investigated the electronic structures of the perovskite-type 4$d$ transition metal oxides Sr$M$O$_3$ ($M$ = Zr, Mo, Ru, and Rh) using their optical conductivity spectra $\sigma (\omega)$. The interband transitions in $\sigma (\omega)$…

强关联电子 · 物理学 2009-11-07 Y. S. Lee , J. S. Lee , T. W. Noh , Douck-Young Byun , Kwang Soo Yoo , K. Yamaura , E. Takayama-Muromachi

We report a comprehensive study of dc susceptibility, specific heat, neutron diffraction, and inelastic neutron scattering measurements on polycrystalline Ba3(Cr1-xVx)2O8 samples, where x=0, 0.06, 0.15, and 0.53. A Jahn-Teller structure…

Valence transition could induce structural, insulator-metal, nonmagnetic-magnetic and superconducting transitions in rare-earth metals and compounds, while the underlying physics remains unclear due to the complex interaction of localized…

We report the first electron paramagnetic resonance studies of single crystals and powders of Pr_{0.6}Ca_{0.4}MnO_{3} in the 300-4.2 K range, covering the charge ordering transition at ~ 240 K and antiferromagnetic transition (T_N) at ~ 170…

强关联电子 · 物理学 2009-10-31 Rajeev Gupta , Janhavi P. Joshi , S. V. Bhat , A. K. Sood , C. N. R. Rao

The phase diagram of Ca$_{2-x}$Sr$_x$RuO$_4$ has been studied by neutron diffraction on powder and single-crystalline samples. The experiments reveal antiferromagnetic order and structural distortions characterized by tilts and rotations of…

超导电性 · 物理学 2009-10-31 O. Friedt , M. Braden , G. Andre , P. Adelmann , S. Nakatsuji , Y. Maeno

We have investigated the electronic structure of the transition metal oxide Ca3Ru2O7 within density functional theory using the generalized gradient approximation while considering strong Coulomb correlations in the framework of the fully…

强关联电子 · 物理学 2024-04-22 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

Here, we study the electrical transport and specific heat in 4$d$ based ferromagnetic material SrRuO$_3$ and its Ti substituted SrRu$_{1-x}$Ti$_x$O$_3$ series ($x$ $\le$ 0.7). The SrRuO$_3$ is a metal and shows itinerant ferromagnetism with…

强关联电子 · 物理学 2020-09-02 Renu Gupta , R. Rawat , A. K. Pramanik

Dielectric spectroscopy of CaCu3Ti4O12 was performed spanning broad ranges of temperature (10-300K) and frequency (0.5Hz-2MHz). We attribute the permittivity step-fall to the evolution of Kirkwood-Fr\"oehlich dipole-correlations; reducing…

材料科学 · 物理学 2014-09-23 A. M. Awasthi , Jitender Kumar

Cu(pz)$_2$(ClO$_4$)$_2$ (with pz denoting pyrazine C$_4$H$_4$N$_2$) is a two-dimensional spin-1/2 square-lattice antiferromagnet with $T_{\mathrm{N}}$ = 4.24 K. Due to a persisting focus on the low-temperature magnetic properties, its…

材料科学 · 物理学 2023-10-24 N. Barbero , M. Medarde , T. Shang , D. Sheptyakov , C. P. Landee , J. Mesot , H. -R. Ott , T. Shiroka

We have investigated the influence of Ca ions substitution on the structural and superconducting properties of (Nd1-xCax)(Ba1.6La0.4)Cu3Oz system. Magnetization, X-ray diffraction and neutron diffraction studies have been carried out on a…

超导电性 · 物理学 2010-05-14 Amish G. Joshi , R. G. Kulkarni , W. B. Yelon , Ram Prasad , M. R. Gonal

The fragile-to-strong crossover seems to be a general feature of metallic glass-forming liquids. Here, we study the behavior of shear viscosity, diffusion coefficient and vibrational density of states for…

软凝聚态物质 · 物理学 2019-08-07 René Alvarez Donado , Samuel Cajahuaringa , Alex Antonelli

Single crystal X-ray diffraction measurements were performed on one-dimensional mixed valence vanadium bronze $\beta$-SrV$_6$O$_{15}$ in which a metal-insulator transition exists at 170 K. Above 170 K the P2$_1$/a structure with zigzag…

强关联电子 · 物理学 2009-11-10 Claire Sellier , Florent Boucher , Etienne Janod

Neutron scattering has been used to study the nature of the ferromagnetic transition in single crystals of La_0.7Ca_0.3MnO_3 and La_0.8Ca_0.2MnO_3, and polycrystalline samples of La_0.67Ca_0.33MnO_3 and La_5/8Ca_3/8MnO_3 where the naturally…

The critical fluctuations in SrTiO$_3$ near its $105 K$ structural phase transition were studied with triple axis diffractometry using high energy ($\ge 100 keV$) synchrotron radiation in different SrTiO$_3$ crystals with different oxygen…

材料科学 · 物理学 2007-05-23 H. Hünnefeld , T. Niemöller , J. R. Schneider , B. A. Kaufmann , F. Schwabl