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A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

量子物理 · 物理学 2009-11-13 Yulian V. Vanne , Alejandro Saenz

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

数学物理 · 物理学 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

A new quantum dynamical model has been developed to describe the dissociative ionization of deuterium molecular ions by intense laser pulses ($\tau=10$ fs, $\lambda=200$ nm and $I=3\times10^{13}$ W/cm$^{2}$). We calculated the ionization…

原子与分子团簇 · 物理学 2017-02-08 Attila Tóth , Sándor Borbély , Zsolt G. Kiss , Gábor J. Halász , Ágnes Vibók

The alignment dependence of the ionization behavior of H$_2$ exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schr\"odinger equation within the fixed-nuclei and dipole…

量子物理 · 物理学 2013-05-29 Yulian V. Vanne , Alejandro Saenz

The ionization of atomic hydrogen in intense laser fields is studied theoretically. The calculations were performed applying both quantummechanical and classical approaches. Treating the problem quantummechanically, the time dependent…

原子物理 · 物理学 2009-11-13 S. Borbély , K. Tőkési , L. Nagy

Intense-field ionization of the hydrogen molecular ion by linearly-polarized light is modelled by direct solution of the fixed-nuclei time-dependent Schr\"odinger equation and compared with recent experiments. Parallel transitions are…

计算物理 · 物理学 2009-11-10 Liang-You Peng , Daniel Dundas , J F McCann , K T Taylor , I D Williams

The alignment- and internuclear-distance dependent ionization of H$_2$ exposed to intense, ultrashort laser fields is studied by solving the time-dependent two-electron Schr\"odinger equation. In the regime of perturbative few-photon…

原子物理 · 物理学 2015-06-23 Johann Förster , Yulian V. Vanne , Alejandro Saenz

The dissociation spectrum of the hydrogen molecular ion by short intense pulses of infrared light is calculated. The time-dependent Schr\"odinger equation is discretized and integrated in position and momentum space. For few-cycle pulses…

原子物理 · 物理学 2009-11-10 Liang-You Peng , I D Williams , J F McCann

A new simulation box setup is introduced for the precise description of the wavepacket evolution of two electronic systems in intense laser pulses. In this box, the regions of the hydrogen molecule H$_{2} $, and singly and doubly ionized…

原子物理 · 物理学 2016-03-03 Mohsen Vafaee , Firoozeh Sami , Babak Shokri , Behnaz Buzari , Hassan Sabzyan

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

原子物理 · 物理学 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

We discuss a method of solving the time dependent Schrodinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997)] to calculate…

原子物理 · 物理学 2014-05-19 Armin Scrinzi , Bernard Piraux

The dynamics of molecular electron excitation and ionisation is studied in real-time for ultra-short IR laser pulses of intensity I>10^{13} W/cm^{2}. The multi-electron molecule is modeled by a system of two active electrons moving in a…

光学 · 物理学 2015-06-26 A. I. Pegarkov

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · 物理学 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

Ionization and excitation of water molecules in intense laser pulses is studied theoretically by solving the three-dimensional time-dependent electronic Schr\"odinger equation within the single-active-electron approximation. The possibility…

原子物理 · 物理学 2011-12-13 Simon Petretti , Alejandro Saenz , Alberto Castro , Piero Decleva

We perform ab initio calculations for the hydrogen atom initially in one of the six circular bound states with the principal quantum numbers n = 2, 3 and 4, irradiated by a short circularly polarized laser pulse of 400 nm. The field…

原子物理 · 物理学 2020-07-01 Jarosław H. Bauer , Zbigniew Walczak

Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…

原子物理 · 物理学 2016-09-08 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

原子物理 · 物理学 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

The ionization of hydrogen Rydberg atoms by circularly polarized microwaves is studied quantum mechanically in a model two dimensional atom. We apply a combination of a transformation to the coordinate frame rotating with the field, with…

chao-dyn · 物理学 2009-10-28 Jakub Zakrzewski , Robert Gebarowski , Dominique Delande

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

原子物理 · 物理学 2016-04-12 Lun Yue , Lars Bojer Madsen

The ionization energy of D$_2$ has been determined experimentally from measurements involving two-photon Doppler-free vacuum-ultraviolet pulsed laser excitation and near-infrared continuous-wave laser excitation to yield…

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