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Neutron scattering is used to study magnetic field induced ordering in the quasi-1D quantum spin-tube compound Sul--Cu$_2$Cl$_4$ that in zero field has a non-magnetic spin-liquid ground state. The experiments reveal an incommensurate chiral…

强关联电子 · 物理学 2009-11-13 V. O. Garlea , A. Zheludev , K. Habicht , M. Meissner , B. Grenier , L. -P. Regnault , E. Ressouche

Inelastic neutron scattering measurements are reported for the quantum antiferromagnetic material Cu_2(C_5H_12N_2)_2Cl_4 (CuHpCl). The magnetic excitation spectrum forms a band extending from 0.9 meV to 1.4 meV. The spectrum contains two…

强关联电子 · 物理学 2009-11-07 M. B. Stone , Y. Chen , J. Rittner , H. Yardimci , D. H. Reich , C. Broholm , D. V. Ferraris , T. Lectka

A field-induced quantum spin liquid (QSL) state is an extraordinary phenomenon, hitherto unobserved in metallic frustrated compounds. Recent bulk measurements have revealed intriguing field-induced magnetic states in metallic frustrated…

强关联电子 · 物理学 2026-01-12 I. Ishant , Z. Guguchia , V. Fritsch , O. Stockert , M. Majumder

The effect of disorder is studied on the field-induced quantum phase transition in the frustrated spin-ladder compound H8C4SO2Cu2(Cl[1-x]Brx)4 using bulk magnetic and thermodynamic measurements. The parent material (x=0) is a quantum spin…

强关联电子 · 物理学 2011-11-15 E. Wulf , S. Mühlbauer , T. Yankova , A. Zheludev

High degeneracy in ground states leads to the generation of exotic zero-energy modes, a representative example of which is the formation of molecular spin liquid-like fluctuations in a frustrated magnet. Here we present single-crystal…

强关联电子 · 物理学 2014-07-17 K. Tomiyasu , T. Yokobori , Y. Kousaka , R. I. Bewley , T. Guidi , T. Watanabe , J. Akimitsu , K. Yamada

Quantum spin liquids represent a magnetic ground state arising in the presence of strong quantum fluctuations that preclude ordering down to zero temperature and leave clear fingerprints in the excitation spectra. While theory bears a…

A hexamer-type spin excitation seen in spinel chromates $A$Cr$_2$O$_4$ ($A$ = Mg, Zn, or Cd) is the representative spin-liquid-like state caused by geometrical frustration. To clarify an origin of the state, we comparatively studied spin…

强关联电子 · 物理学 2011-08-18 K. Tomiyasu , H. Ueda , M. Matsuda , M. Yokoyama , K. Iwasa , K. Yamada

Investigation of materials that exhibit quantum phase transition provides valuable insights into fundamental problems in physics. We present neutron scattering under pressure in a triangular-lattice antiferromagnet which has a quantum…

Continuum of spin excitations observed in inelastic neutron scattering experiments are often considered as a strong evidence of quantum spin liquid formation. When quantum spin liquid is indeed the ground state of a disorder-free magnetic…

The ground states of the frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied by inelastic neutron scattering experiments. Three single-crystal samples are investigated; one shows no phase transition…

We present results of inelastic neutron scattering study on two bond disordered quasi twodimensional quantum magnets (C$_4$H$_12$N$_2$)Cu$_2$(Cl$_{1-x}$Br$_x$)$_6$ with x=0.035 and 0.075. We observe the increase of spin gap, reduction of…

强关联电子 · 物理学 2013-07-02 D. Huvonen , S. Zhao , G. Ehlers , M. Månsson , S. N. Gvasaliya , A. Zheludev

We report detailed inelastic neutron scattering measurements on single crystals of the frustrated two-leg ladder BiCu2PO6, whose ground state is described as a spin liquid phase with no long-range order down to 6 K. Two branches of steeply…

强关联电子 · 物理学 2013-08-09 K. W. Plumb , Zahra Yamani , M. Matsuda , G. J. Shu , B. Koteswararao , F. C. Chou , Young-June Kim

Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…

Inelastic neutron scattering experiments on the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C9D24N4)(NO2)ClO4 have been performed under magnetic fields below and above a critical field Hc at which the energy gap closes.…

The weakly coupled quasi-one-dimensional spin ladder compound (CH$_3$)$_2$CHNH$_3$CuCl$_3$ is studied by neutron scattering in magnetic fields exceeding the critical field of Bose-Einstein condensation of magnons. Commensurate long-range…

KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

强关联电子 · 物理学 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

When magnetic order is suppressed by frustrated interactions, spins form a highly correlated fluctuating "spin liquid" state down to low temperatures. Magnetic order of local moments can also be suppressed when they are fully screened by…

强关联电子 · 物理学 2014-03-25 Y. Tokiwa , J. J. Ishikawa , S. Nakatsuji , P. Gegenwart

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

强关联电子 · 物理学 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

We introduce a frustrated spin 1/2 Hamiltonian which is an extension of the two dimensional $J_1 - J_2$ Heisenberg model. The ground states of this model are exactly obtained at a first order quantum phase transition between two regions…

强关联电子 · 物理学 2009-11-10 C. D. Batista , S. A. Trugman

We review the interplay of frustration and strong electronic correlations in quasi-two-dimensional organic charge transfer salts, such as k-(BEDT-TTF)_2X and Et_nMe_{4-n}Pn[Pd(dmit)2]2. These two forces drive a range of exotic phases…

强关联电子 · 物理学 2011-05-06 B. J. Powell , Ross H. McKenzie
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