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Iron (II) complexes with substituted tris(pyrazolyl) ligands, which exhibit a thermally driven transition from a low-spin state at low temperatures to a high-spin state at elevated temperatures, have been studied by M\"ossbauer spectroscopy…

Very recently, a 3$d$ based honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has garnered tremendous attention due to the proposed proximity to the Kitaev spin-liquid state as its 4$d$/5$d$ counterparts. Here, we use Zn to substitute Co in a broad…

High-quality single crystals of CoTiO$_3$ are grown and used to elucidate in detail structural and magnetostructural effects by means of high-resolution capacitance dilatometry studies in fields up to 15 T which are complemented by specific…

强关联电子 · 物理学 2021-07-19 M. Hoffmann , K. Dey , J. Werner , R. Bag , J. Kaiser , H. Wadepohl , Y. Skourski , M. Abdel-Hafiez , S. Singh , R. Klingeler

We report the results of low-temperature magnetization and specific heat measurements of Sr$_3$CoTa$_2$O$_9$ powder, in which Co$^{2+}$ ions with effective spin-1/2 form a uniform triangular lattice in the $ab$ plane. It was found that…

强关联电子 · 物理学 2023-05-24 Iori Nishizawa , Nobuyuki Kurita , Hidekazu Tanaka , Takayuki Goto

We present a detailed magnetic study of the perovskite manganite Pr0.7Ca0.3MnO3 at low temperatures including magnetization and a.c. susceptibility measurements. The data appear to exclude a conventional spin glass phase at low fields,…

强关联电子 · 物理学 2009-10-31 I. G. Deac , J. F. Mitchell , P. Schiffer

Co10Ge3O16 crystallizes in an intergrowth structure featuring alternating layers of spinel and rock salt. Variable-temperature powder synchrotron X-ray and neutron diffraction, magnetometry, and heat capacity experiments reveal a…

材料科学 · 物理学 2013-07-12 Phillip T. Barton , Ram Seshadri , Anna Llobet , Matthew R. Suchomel

Magneto-dielectric spectra of La0.95Ca0.05CoO3 covering the crossover of spin states reveals strong coupling of its spin and dipolar degrees of freedom. Signature of spin-state transition at 30K clearly manifests in magnetization, supported…

材料科学 · 物理学 2016-02-29 Suchita Pandey , Jitender Kumar , A. M. Awasthi

We have investigated the temperature dependence of the magnetic susceptibility $\chi(T)$ of rare-earth cobaltites RCoO$_3$ (R= La, Pr, Nd, Sm, Eu) in the temperature range $4.2-300$ K and also the influence of hydrostatic pressure up to 2…

We report on the evolution of the average and depth-dependent magnetic order in thin film samples of biaxially stressed and electron-doped EuTiO$_3$ for samples across a doping range $<$0.1 to 7.8 $\times 10^{20}$ cm$^{-3}$. Under an…

We have investigated the temperature and magnetic field dependence of magnetization ($M$), specific heat ($C_p$), and relative sample length change ($\Delta L/L_0$) for understanding the field-induced metamagnetic transitions in…

强关联电子 · 物理学 2016-01-20 M. Nandi , P. Mandal

The solid solution 122 compounds, Eu(Co$_{1-x}$Ni$_{x}$)$_{2}$P$_{2}$, show valence transition between divalent state and intermediate valence states at Eu, which is firmly correlated to multiple degrees of freedom in the solid such as the…

The oxygen-deficient perovskite cobaltite SrCo1-xNbxO3-d was synthesized by direct solid-state reaction and its magnetotransport properties were investigated. This cobaltite exhibits an unusual ferromagnetic behavior with a transition…

强关联电子 · 物理学 2009-11-11 T. Motohashi , V. Caignaert , V. Pralong , M. Hervieu , A. Maignan , B. Raveau

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

We propose the realization of linear crystals of cold ions which contain different atomic species for investigating quantum phase transitions and frustration effects in spin system beyond the commonly discussed case of $s=1/2$. Mutual…

量子物理 · 物理学 2015-05-28 Peter A. Ivanov , Ferdinand Schmidt-Kaler

We study single crystals of Dy$_2$Ti$_2$O$_7$ and Ho$_2$Ti$_2$O$_7$ under magnetic field and stress applied along their [001] direction. We find that many of the features that the emergent gauge field of spin ice confers to the macroscopic…

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

强关联电子 · 物理学 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

We use transport and neutron-scattering measurements to show that a magnetic-field-induced transition from noncollinear to collinear spin arrangement in adjacent CuO_{2} planes of lightly electron-doped Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4}…

The pyrochlore oxides Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ are well studied spin ice systems and have shown the evidences of magnetic monopole excitations. Unlike these, Dy$_{2}$Zr$_{2}$O$_{7}$ is reported to crystallize in a…

强关联电子 · 物理学 2020-08-26 Sheetal , Anzar Ali , Sarita Rajput , Yogesh Singh , Tulika Maitra , C. S. Yadav

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

强关联电子 · 物理学 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

Within the framework of a realistic multi-band p-d-model, we derived an effective Hamiltonian to describe the exchange interaction effects near the spin crossover in magnetic Mott-Hubbard insulators under pressure. It is shown that…

强关联电子 · 物理学 2017-10-18 Alexander I. Nesterov , Yuri S. Orlov , Sergey G. Ovchinnikov , Sergey V. Nikolaev