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The magnetoelectric coupling, i.e., cross-correlation between electric and magnetic orders, is a very desirable property to combine functionalities of materials for next-generation switchable devices. Multiferroics with spin-driven…

Magnetic and magnetoelectric excitations in the multiferroic TbMnO_3 have been investigated at terahertz frequencies. Using different experimental geometries we can clearly separate the electro-active excitations (electromagnons) from the…

强关联电子 · 物理学 2009-03-16 A. Pimenov , A. Shuvaev , A. Loidl , F. Schrettle , A. A. Mukhin , V. D. Travkin , V. Yu. Ivanov , A. M. Balbashov

Low energy excitations in the multiferroic material TbMnO3 have been investigated by Raman spectroscopy. Our observations reveal the existence of two peaks at 30 cm-1 and 60 cm-1. They are observed in the cycloidal phase below the Curie…

强关联电子 · 物理学 2010-10-12 P. Rovillain , M. Cazayous , Y. Gallais , A. Sacuto , M-A. Measson , H. Sakata

We summarize the existing experimental data on electromagnons in multiferroic RMn2O5 compounds, where R denotes a rare earth ion, Y or Bi, and discuss a realistic microscopic model of these materials based on assumption that the microscopic…

材料科学 · 物理学 2009-11-13 A. B. Sushkov , M. Mostovoy , R. Valdes Aguilar , S. -W. Cheong , H. D. Drew

Magnetodielectric materials are characterized by a strong coupling of magnetic and dielectric properties and in rare cases simultaneously exhibit both, magnetic and polar order. Among other multiferroics, TbMnO3 and GdMnO3 reveal a strong…

强关联电子 · 物理学 2015-06-25 A. Pimenov , A. A. Mukhin , V. Yu. Ivanov , V. D. Travkin , A. M. Balbashov , A. Loidl

A new type of multiferroicity was experimentally discovered in 2003 in a perovskite manganite TbMnO$_3$ where its ferroelectricity is induced by cycloidally ordered Mn spins. Susequently, such spin-cycloid multiferroic phase was also…

强关联电子 · 物理学 2025-02-14 Masahito Mochizuki

Inelastic neutron scattering has been used to study the magneto-elastic excitations in the multiferroic manganite hexagonal YMnO$_3$. An avoided crossing is found between magnon and phonon modes close to the Brillouin zone boundary in the…

Terahertz electromagnetic excitations in the multiferroic TbMnO3 at the field-induced magnetic transition are investigated for different orientations of the magnetic cycloid. In addition to the electromagnon along the a-axis, the detailed…

强关联电子 · 物理学 2011-03-03 A. M. Shuvaev , V. D. Travkin , V. Yu. Ivanov , A. A. Mukhin , A. Pimenov

The optical spectra in the family of multiferroic manganites RMnO3 is a great puzzle. Current models can not explain the fact that two strong electromagnons are present in the non-collinear spin cycloidal phase, with only one electromagnon…

强关联电子 · 物理学 2013-03-05 Markku P. V. Stenberg , Rogério de Sousa

Recently, oxide multiferroics have attracted much attention due to their large magnetoelectric effect which allows the tuning of magnetic properties with electric field and vice versa and open new venues for future spintronic applications…

强关联电子 · 物理学 2010-10-12 M. Cazayous , Y. Gallais , A. Sacuto , R. De Sousa , D. Lebeugle , D. Colson

We have studied the impact of the magnetic field on the electromagnon excitations in TbMnO3 crystal. Applying magnetic field along the c axis, we show that the electromagnons transform into pure antiferromagnetic modes, losing their polar…

材料科学 · 物理学 2011-07-06 P. Rovillain , M. Cazayous , Y. Gallais , M-A. Measson , A. Sacuto , H. Sakata , M. Mochizuki

The magnetic excitations in multiferroic TbMnO3 have been studied by inelastic neutron scattering in the spiral and sinusoidally ordered phases. At the incommensurate magnetic zone center of the spiral phase, we find three low-lying magnons…

强关联电子 · 物理学 2007-05-23 D. Senff , P. Link , K. Hradil , A. Hiess , L. P. Regnault , Y. Sidis , N. Aliouane , D. N. Argyriou , M. Braden

Using a joint approach of density functional theory and model calculations, we demonstrate that a prototypical charge ordered half-doped manganite, La$_{1/2}$Ca$_{1/2}$MnO$_3$ is multiferroic. The combination of a peculiar charge-orbital…

材料科学 · 物理学 2010-07-15 Gianluca Giovannetti , Sanjeev Kumar , Jeroen van den Brink , Silvia Picozzi

We have performed Raman measurements on TbMnO3 single crystal under magnetic field along the three crystallographic directions. The flip of the spin spiral plane creates an electromagnon excitation. In addition to the electromagnons induced…

强关联电子 · 物理学 2015-06-05 P. Rovillain , J. Liu , M. Cazayous , Y. Gallais , M. -A. Measson , H. Sakata , A. Sacuto

InMnO$_3$ is a peculiar member of the hexagonal manganites h-RMnO$_3$ (where R is a rare earth metal element), showing crystalline, electronic and magnetic properties at variance with the other compounds of the family. We have studied high…

材料科学 · 物理学 2015-03-19 X. Fabrèges , I. Mirebeau , S. Petit , P. Bonville , A. A. Belik

Type-II multiferroics, where spin order induces ferroelectricity, exhibit strong magnetoelectric coupling. However, for the typical 2D type-II multiferroic NiI$_2$, the underlying magnetoelectric mechanism remains unclear. Here, applying…

Magnetic rare earths R have been proven to have a significant effect on the multiferroic properties of the orthorhombic manganites RMnO3. A re-examination of previous results from synchrotron based x-ray scattering experiments suggests that…

强关联电子 · 物理学 2015-05-13 R Feyerherm , E Dudzik , O Prokhnenko , D N Argyriou

The effect of rare-earth ions (R = Er^{3+}, Tb^{3+}) with strong spin-orbit coupling on the dielectric properties and the electric polarization induced by local polar phase separation domains in RMn_2O_5 multiferroics has been studied.…

材料科学 · 物理学 2020-02-14 B. Kh. Khannanov , E. I. Golovenchits , V. A. Sanina

We theoretically study origins of the ferroelectricity in the multiferroic phases of the rare-earth (R) Mn perovskites, RMnO3, by constructing a realistic spin model including the spin-phonon coupling, which reproduces the entire…

强关联电子 · 物理学 2011-02-21 Masahito Mochizuki , Nobuo Furukawa , Naoto Nagaosa

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

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