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We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the…

原子物理 · 物理学 2010-04-21 C. B. Madsen , M. Abu-samha , L. B. Madsen

We report on an experimental study on the interaction of a high-contrast 40 fs duration 2.5 TW laser pulse with an argon cluster target. A high-charge, homogeneous, large divergence electron beam with moderate kinetic energy (~2 MeV) is…

We show that two-color high-harmonic spectroscopy can reveal finite-size and edge-state-induced dynamic electron correlation effects in a generic nanostructured band-gap material. Compared to the response of a bulk sample, we demonstrate a…

原子物理 · 物理学 2021-05-28 Simon Vendelbo Bylling Jensen , Hossein Iravani , Lars Bojer Madsen

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

光学 · 物理学 2023-12-01 Shicheng Jiang , Mahesh Gudem , Markus Kowalewski , Konstantin Dorfman

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

原子物理 · 物理学 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

材料科学 · 物理学 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

High-harmonic generation by a highly non-linear interaction of infrared laser fields with matter allows for the generation of attosecond pulses in the XUV spectral regime. This process, well established for atoms, has been recently extended…

The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…

原子物理 · 物理学 2011-06-14 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

We investigate the possibility to deduce momentum space properties from time-dependent density functional calculations. Electron and ion momentum distributions after double ionization of a model Helium atom in a strong few-cycle laser pulse…

原子物理 · 物理学 2009-11-13 F. Wilken , D. Bauer

Using time-dependent density functional theory, high-harmonic generation (HHG) is studied in one-dimensional structures of sizes from a single nucleus up to hundreds of nuclei. The HHG cutoff is observed to extent linearly with the system…

原子物理 · 物理学 2018-04-27 Kenneth K. Hansen , Dieter Bauer , Lars Bojer Madsen

Using one-dimensional simulations analyzed through the lens of open quantum systems, we study the photoelectron's strong-field dynamics from an atom surrounded by a scattering environment stochastically structured. We theoretically…

量子物理 · 物理学 2026-05-21 Simon His , Camille Lévêque , Jérémie Caillat , Richard Taïeb , Jonathan Dubois

We study various temporal correlation functions of a tagged particle in one-dimensional systems of interacting point particles evolving with Hamiltonian dynamics. Initial conditions of the particles are chosen from the canonical thermal…

统计力学 · 物理学 2015-06-25 Anjan Roy , Abhishek Dhar , Onuttom Narayan , Sanjib Sabhapandit

The dynamics of electrons in the presence of a positive ion is considered for conditions of weak electron-electron couping but strong electron-ion coupling. The equilibrium electron density and electric field time correlation functions are…

统计力学 · 物理学 2007-05-23 James W. Dufty , Ilya V. Pogorelov , Bernard Talin , Annette Calisti

The interaction of electrons with strong laser fields is usually treated with semiclassical theory, where the laser is represented by an external field. There are analytic solutions for the free electron wave functions, which incorporate…

量子物理 · 物理学 2024-07-09 Sándor Varró

An effective self-consistent model is derived and used to study the dynamics of an electron gas confined in a nonparabolic and anisotropic quantum well. This approach is based on the equations of quantum hydrodynamics, which incorporate…

介观与纳米尺度物理 · 物理学 2016-05-11 Jerome Hurst , Kevin Leveque-Simon , Paul-Antoine Hervieux , Giovanni Manfredi , Fernando Haas

We investigated the high-order harmonic generation by interacting time-delayed, linearly polarized bi-chromatic laser pulses with the atomic target. The frequency ratio of secondary to primary fields ($\omega_2/\omega_1$), along with the…

原子物理 · 物理学 2023-04-26 Rambabu Rajpoot , Amol R. Holkundkar

The effect of changing the driving frequency on the plasma density and the electron dynamics in a capacitive radio-frequency argon plasma operated at low pressures of a few Pa is investigated by Particle in Cell/Monte Carlo Collisions…

等离子体物理 · 物理学 2015-04-01 S. Wilczek , J. Trieschmann , J. Schulze , E. Schuengel , R. P. Brinkmann , A. Derzsi , I. Korolov , Z. Donkó , T. Mussenbrock

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Simulations and diagnostics of high-energy-density plasmas and warm dense matter rely on models of material response properties, both static and dynamic (frequency-dependent). Here, we systematically investigate variations in dynamic…