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Methane is thought to have been an important greenhouse gas during the Archean, although its potential warming has been found to be limited at high concentrations due to its high shortwave absorption. We use the Met Office Unified Model, a…

The systems C$_6$H$_5$Cl, or C$_6$H$_5$Br, or 1-chloronaphthalene, or 1,2,4-trichlorobenzene, or 1-methylnaphthalene, or 1,2,4-trimethylbenzene + alkane have been investigated by means of the their excess molar properties, including, when…

Decomposition of methane using non-thermal plasmas is an attractive route for producing hydrogen-rich gases and valuable carbon nanomaterials. Understanding how plasma discharge modes influence methane decomposition in optimizing…

等离子体物理 · 物理学 2025-11-17 Sophia Gershman , Mikhail N. Shneider , Yevgeny Raitses

A systematic investigation on the effects of roaming radical reactions on global combustion properties for transportation fuels is presented. New software was developed that can automatically discover all the possible roaming pathways…

化学物理 · 物理学 2018-07-03 Richard H. West , C. Franklin Goldsmith

We present observations of methanol lines in a sample of Class 0 low mass protostars. Using a 1-D radiative transfer model, we derive the abundances in the envelopes. In two sources of the sample, the observations can only be reproduced by…

天体物理学 · 物理学 2007-05-23 S. Maret , C. Ceccarelli , A. G. G. M. Tielens , E. Caux , B. Lefloch , A. Faure , A. Castets , D. R. Flower

New experimental data are collected for methyl-cyclohexane (MCH) autoignition in a heated rapid compression machine (RCM). Three mixtures of MCH/O2/N2/Ar at equivalence ratios of $\phi$=0.5, 1.0, and 1.5 are studied and the ignition delays…

化学物理 · 物理学 2017-06-12 Bryan W. Weber , WIlliam J. Pitz , Marco Mehl , Emma Silke , Alexander C. Davis , Chih-Jen Sung

The formation of polycyclic aromatic hydrocarbons (PAHs) and their methyl derivatives occurs mainly in the dust shells of asymptotic giant branch (AGB) stars. The bands at 3.3 and 3.4 $\mu$m, observed in infrared emission spectra of several…

太阳与恒星天体物理 · 物理学 2016-04-20 T. Monfredini , F. Fantuzzi , M. A. C. Nascimento , W. Wolff , H. M. Boechat-Roberty

Autoignition delay times, ?, of methyl crotonate, methyl acrylate, ethyl butanoate, ethyl crotonate, and ethyl acrylate were studied in shock tube experiments. A series of mixtures diluted with argon, of varying fuel/oxygen equivalence…

Ammonia is a promising zero-carbon fuel for industrial and transport applications, but its combustion is hindered by flame instabilities, incomplete oxidation, and the formation of nitrogen oxides. Accurate and detailed kinetic models are…

Laminar premixed flame profiles of methane/air free flames and strained flames at different fuel/air ratios and strain rates are analysed using detailed chemistry with Lewis numbers equal to one. It is shown that the detailed chemistry…

流体动力学 · 物理学 2021-12-21 Michael Pfitzner , Paola Breda

This study introduces a catalyst-free, ambient-temperature method for synthesizing nitrogen-based compounds critical to fertilizer production, including ammonia, urea, ammonium salts, and amino acids. The process relies on…

化学物理 · 物理学 2025-06-03 Jerome J. Cuomo , Ian Goodall , C. Richard Guarnieri , Gennaro , Cuomo , Stephen Hudak

Liquid-liquid equilibrium (LLE) phase diagrams have been determined, by means of the critical opalescence method with a laser scattering technique, for the mixtures 4-phenylbutan-2-one + CH$_3$(CH$_2$)$_n$CH$_3$ ($n = 10,12,14$) and for…

We present the first experimental characterization in molecular fragile glassformers of a 'prepeak that appears significantly below the main peak of the static structure factor. The temperature and density dependences of this prepeak are…

Autoignition of n-heptane droplet/vapor/air mixtures behind an oblique shock wave are studied, through Eulerian-Lagrangian method and a skeletal chemical mechanism. The effects of gas/liquid equivalence ratio (ER), droplet diameter, flight…

流体动力学 · 物理学 2022-12-16 Hongbo Guo , Yong Xu , Ningbo Zhao , Huangwei Zhang

Based on the first-principles density functional theory electronic structure calculation, we investigate the possible phonon-mediated superconductivity in arsenene, a two-dimensional buckled arsenic atomic sheet, under electron doping. We…

超导电性 · 物理学 2018-03-28 Xin Kong , Miao Gao , Xun-Wang Yan , Zhong-Yi Lu , Tao Xiang

The Voyager 1 flyby of Titan in 1980 gave a first glimpse of the chemical complexity of Titan's atmosphere, detecting many new molecules with the infrared spectrometer (IRIS). These included propane (C3H8) and propyne (CH3C2H), while the…

In this work, we have estimated self diffusion coefficients along with the binary diffusion coefficients of mixtures of alkane (methane, ethane, propane and n-butane) in SPC/E water(H$_2$O). Molecular dynamics study of a binary mixture of…

The most popular way to produce graphene nowadays is chemical vapor deposition, where, surprisingly, H$_2$ gas is routinely supplied even though it is a byproduct itself. In this study, by identifying dominant growing pathways via…

材料科学 · 物理学 2017-11-28 Pai Li , Zhenyu Li , Jinlong Yang

Zeolite channels can be used as effective hydrocarbon traps. Earlier experiments (Czaplewski {\sl et al.}, 2002) show that the presence of large aromatic molecules (toluene) block the diffusion of light hydrocarbon molecules (propane)…

统计力学 · 物理学 2009-01-20 Sakuntala Chatterjee , Gunter M. Schütz

The current paper presents the third part of the study devoted to composites formed by fullerene C60 and two graphene nanosheets ([C60+(5,5)] and ([C60+(9, 8)] graphene nanobuds). The formation of composites is considered from the basic…

材料科学 · 物理学 2011-06-06 E. F. Sheka , L. Kh. Shaymardanova