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In doped manganites, the strong electron-phonon coupling due to the Jahn-Teller effect localizes the conduction-band electrons as polarons. This results in polarons are carriers responsible for transport and ferromagnetic ordering rather…

强关联电子 · 物理学 2008-12-16 Liping Chen , Yubin Ma , Xianfeng Song , Guijun Lian , Guangcheng Xiong

Polarons - fermionic charge carriers bearing a strong companion lattice deformation - exhibit a natural tendency for self-localization due to the recursive interaction between electrons and the lattice. While polarons are ubiquitous in…

A system of strongly-interacting electron-lattice polarons can exhibit charge and orbital order at sufficiently high polaron concentrations. In this study, the structure of short-range polaron correlations in the layered colossal…

We present the results of a systematic x-ray scattering study of the charge and orbital ordering in the manganite series Pr$_{1-x}$Ca$_x$MnO$_3$ with $x$=0.25, 0.4 and 0.5. The temperature dependence of the scattering at the charge and…

In addition to mechanisms already proposed to account for the formation in manganites of a small-polaron superlattice above the Curie temperature Tc and to a metallic-like sea of large polarons below Tc, we now consider other observed…

材料科学 · 物理学 2007-12-27 Mladen Georgiev

We report on an a $\mu$SR and $^{55}$Mn NMR investigation of the magnetic order parameter as a function of temperature in the optimally doped La$_{5/8}$(Ca$_y$Sr$_{1-y}$)$_{3/8}$MnO$_3$ and in the underdoped La$_{1-x}$Sr$_{x}$MnO$_3$ and…

强关联电子 · 物理学 2013-09-30 G. Allodi , R. De Renzi , K. Zheng , S. Sanna , A. Sidorenko , C. Baumann , L. Righi , F. Orlandi , G. Calestani

Modulations in manganites attributed to stripes of charge/orbital/spin order are thought to result from strong electron-lattice interactions that lock the superlattice and parent lattice periodicities. Surprisingly in La1-xCaxMnO3(x>0.5, 90…

强关联电子 · 物理学 2007-05-23 J. C. Loudon , S. Cox , A. J. Williams , J. P. Attfield , P. B. Littlewood , P. A. Midgley , N. D. Mathur

In the colossal magnetoresistance manganites polarons have been proposed as the charge carrier state which localizes across the metal-insulator transition. The character of the polarons is still under debate. We present an assessment of…

强关联电子 · 物理学 2015-06-24 Ch. Hartinger , F. Mayr , A. Loidl , T. Kopp

The short range ordered magnetic correlations have been studied in half doped La0.5Ca0.5-xSrxMnO3 (x = 0.1, 0.3 and 0.4) compounds by polarized neutron scattering technique. On doping Sr2+ for Ca2+ ion, these compounds with x = 0.1, 0.3,…

材料科学 · 物理学 2015-05-18 I. Dhiman , A. Das , R. Mittal , Y. Su , A. Kumar , A. Radulescu

Recently a growing number of experiments have provided indications of the key role of polarons (composite particles formed by a charge strongly coupled with a local lattice deformation) in doped perovskites, hosting colossal…

超导电性 · 物理学 2009-09-25 A. Lanzara , N. L. Saini , A. Bianconi , Guo-meng Zhao , K. Conder , H. Keller , K. A. Muller

The electrical resistivity, Hall coefficient, and thermopower as functions of temperature are reported for lightly electron-doped Ca(1-x)La(x)MnO(3)(0 <= x <= 0.10). Unlike the case of hole-doped ferromagnetic manganites, the magnitude and…

强关联电子 · 物理学 2009-11-11 J. L. Cohn , C. Chiorescu , J. J. Neumeier

By resonant x-ray scattering at the Mn K-edge on La7/8Sr1/8MnO3, we show that an orbital polaron lattice (OPL) develops at the metal-insulator transition of this compound. This orbital reordering explains consistently the unexpected…

强关联电子 · 物理学 2007-05-23 J. Geck , P. Wochner , S. Kiele , R. Klingeler , P. Reutler , A. Revcolevschi , B. Buechner

In complex electronic materials, coupling between electrons and the atomic lattice gives rise to remarkable phenomena, including colossal magnetoresistance and metal-insulator transitions. Charge-ordered phases are a prototypical…

Neutron scattering has been used to study the nature of the ferromagnetic transition in a single crystal of the perovskite La0.7Ca0.3MnO3. Diffuse scattering from lattice polarons develops as the Curie temperature is approached from below,…

强关联电子 · 物理学 2009-10-31 C. P. Adams , J. W. Lynn , Y. M. Mukovskii , A. A. Arsenov , D. A. Shulyatev

We apply grazing-incidence femtosecond x-ray diffraction to investigate the details of the atomic motion connected with a displacively excited coherent optical phonon. We concentrate on the low frequency phonon associated with the charge…

We apply the Dynamical Mean Field Theory to the problem of charge ordering. In the normal state as well as in the Charge Ordered (CO) state the existence of polarons, i.e. electrons strongly coupled to local lattice deformation, is…

强关联电子 · 物理学 2009-10-31 S. Ciuchi , F. de Pasquale

We report x-ray scattering studies of broad peaks located at a (0.5 0 0)/(0 0.5 0)-type wavevector in the paramagnetic insulating phases of La_{0.7}Ca_{0.3}MnO_{3} and Pr_{0.7}Ca_{0.3}MnO_{3}. We interpret the scattering in terms of…

Charge carrier localization in extended atomic systems has been described previously as being driven by disorder, point defects or distortions of the ionic lattice. Here we show for the first time by means of first-principles computations…

介观与纳米尺度物理 · 物理学 2016-05-11 Vojtěch Vlček , Helen R. Eisenberg , Gerd Steinle-Neumann , Daniel Neuhauser , Eran Rabani , Roi Baer

Optical control of magnetism, of interest for high-speed data processing and storage, has only been demonstrated with near-infrared excitation to date. However, in absorbing materials, such high photon energies can lead to significant…

A new mechanism is proposed to explain the colossal magnetoresistance and related phenomena. Moving electrons accompanied by Jahn-Teller phonon and spin-wave clouds may form composite polarons in ferromagnetic narrow-band manganites. The…

强关联电子 · 物理学 2016-08-31 Liang-Jian Zou , H. Q. Lin , Qing-Qi Zheng
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