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We present a microscopic model of the spin-gap quantum magnet (CuCl)LaNb2O7 that was previously suggested as a realization of the spin-1/2 frustrated square lattice. Taking advantage of the precise atomic positions from recent crystal…

强关联电子 · 物理学 2010-08-30 Alexander A. Tsirlin , Helge Rosner

We have successfully synthesized single crystals, solved the crystal structure, and studied the magnetic properties of a new family of copper halides (C$_4$H$_{14}$N$_2$)Cu$_2X_6$ ($X$= Cl, Br). These compounds crystallize in an…

材料科学 · 物理学 2023-06-28 P. Biswal , S. Guchhait , S. Ghosh , S. N. Sarangi , D. Samal , Diptikant Swain , Manoranjan Kumar , R. Nath

Using inelastic neutron scattering, x-ray, neutron diffraction, and the first-principle calculation techniques, we show that the crystal structure of the two-dimensional quantum spin system (CuCl)LaNb$_2$O$_7$ is orthorhombic with $Pbam$…

强关联电子 · 物理学 2015-05-19 C. Tassel , J. Kang , C. Lee , O. Hernandez , Y. Qiu , W. Paulus , E. Collet , B. Lake , T. Guidi , M. -H. Whangbo , C. Ritter , H. Kageyama , S. -H. Lee

We present a model describing the lattice distortion and incommensurate magnetic order in the spinel CdCr2O4, a good realization of the Heisenberg "pyrochlore" antiferromagnet. The magnetic frustration is relieved through the spin-Peierls…

强关联电子 · 物理学 2007-05-23 Gia-Wei Chern , C. J. Fennie , O. Tchernyshyov

GeCu2O4 exhibits a tetragonal spinel structure due to the strong Jahn-Teller distortion associated with Cu2+ ions. We show that its magnetic structure can be described as slabs composed of a pair of layers with orthogonally oriented spin…

材料科学 · 物理学 2016-12-14 T. Zou , Y. -Q. Cai , C. R. dela Cruz , V. O. Garlea , S. D. Mahanti , J. -G. Cheng , X. Ke

Inelastic neutron scattering measurements are reported for the quantum antiferromagnetic material Cu_2(C_5H_12N_2)_2Cl_4 (CuHpCl). The magnetic excitation spectrum forms a band extending from 0.9 meV to 1.4 meV. The spectrum contains two…

强关联电子 · 物理学 2009-11-07 M. B. Stone , Y. Chen , J. Rittner , H. Yardimci , D. H. Reich , C. Broholm , D. V. Ferraris , T. Lectka

We review the mechanism of spin-lattice coupling in relieving the geometrical frustration of pyrochlore antiferromagnets, in particular spinel oxides. The tetrahedral unit, which is the building block of the pyrochlore lattice, undergoes a…

强关联电子 · 物理学 2018-07-25 O. Tchernyshyov , G. -W. Chern

We study the influence of the spin lattice distortion on the properties of frustrated magnetic systems and consider the applicability of the spin-1/2 frustrated square lattice model to materials lacking tetragonal symmetry. We focus on the…

强关联电子 · 物理学 2009-06-16 Alexander A. Tsirlin , Helge Rosner

Magnetic ordering in the geometrically frustrated magnetic oxide spinels MgCr_2O_4 and ZnCr_2O_4 is accompanied by a structural change that helps relieve the frustration. Analysis of high-resolution synchrotron X-ray scattering reveals that…

We study polycrystalline samples of KCu3As2O7(OH)3, a new candidate spin-1/2 kagome antiferromagnet, by magnetic susceptibility and heat capacity measurements above 2 K. The unique arrangement of the 3z2 - r2 and x2 - y2 orbitals on the…

材料科学 · 物理学 2015-06-04 Yoshihiko Okamoto , Hajime Ishikawa , Gøran J. Nilsen , Zenji Hiroi

Structural properties of CuAl$_{2}$O$_{4}$, which was recently argued to show unusual suppression of the Jahn-Teller distortions by the spin-orbit coupling, are investigated under pressures up to 6 GPa. Analysis of X-ray powder diffraction…

强关联电子 · 物理学 2020-11-10 P. A. Agzamova , A. A. Belik , S. V. Streltsov

For nearly three decades frustrated magnetism research in three dimensions (3D) has centered on the pyrochlore geometry of corner-sharing tetrahedra and the classical spin liquid (CSL) known as spin ice. In this work, we propose that a…

A recent study [Tassel {\it et al.}, Phys. Rev. Lett. {\bf 105}, 167205 (2010)] has proposed a remarkable spin model for (CuCl)LaNb2O7, in which dimers are ferromagnetically coupled to each other on the distorted Shastry-Sutherland lattice.…

强关联电子 · 物理学 2011-08-17 Shunsuke Furukawa , Tyler Dodds , Yong Baek Kim

We investigated the electronic and magnetic structure of Sr$_{3-x}$Ca$_x$Ru$_2$O$_7$ ($0 \leq x \leq 3$) on the basis of the double-layered three-dimensional multiband Hubbard model with spin-orbit interaction. In our model, lattice…

强关联电子 · 物理学 2011-11-15 Shigeru Koikegami , Takashi Yanagisawa , Soh Koike

To leading order in displacement size, the scattering of electrons in a Cu-O plane from O displacements perpendicular to that plane is due to spin-orbit coupling. This scattering is investigated with the following results: (1) As a…

凝聚态物理 · 物理学 2020-02-03 N. E. Bonesteel

Transition metal oxides exhibit various competing phases and exotic phenomena depending on how their reaction to the rich degeneracy of the $d$-orbital. Large spin-orbit coupling (SOC) reduces this degeneracy in a unique way by providing a…

Using synchrotron X-rays and neutron diffraction we disentangle spin-lattice order in highly frustrated ZnCr$_2$O$_4$ where magnetic chromium ions occupy the vertices of regular tetrahedra. Upon cooling below 12.5 K the quandary of…

强关联电子 · 物理学 2009-05-14 S. Ji , S. -H. Lee , C. Broholm , T. Y. Koo , W. Ratcliff , S-W. Cheong , P. Zschack

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

强关联电子 · 物理学 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

Although charge-density wave (CDW) correlations exist in several families of cuprate supercon-ductors, they exhibit substantial variation in CDW wavevector and correlation length, indicating a key role for CDW-lattice interactions. We…

The collective behavior of interacting magnetic moments can be strongly influenced by the topology of the underlying lattice. In geometrically frustrated spin systems, interesting chiral correlations may develop that are related to the spin…

强关联电子 · 物理学 2007-05-23 D. Grohol , K. Matan , J. H. Cho , S. -H. Lee , J. W. Lynn , D. G. Nocera , Y. S. Lee
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