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Electronic transport through a single-molecule magnet Mn$_{12}$ in a two-terminal set up is calculated using the non-equilibrium Green's function method in conjunction with density-functional theory. A single-molecule magnet Mn$_{12}$ is…

材料科学 · 物理学 2010-01-28 Salvador Barraza-Lopez , Kyungwha Park , Víctor García-Suárez , Jaime Ferrer

We report transport measurements through a single-molecule magnet, the Mn12 derivative [Mn12O12(O2C-C6H4-SAc)16(H2O)4], in a single-molecule transistor geometry. Thiol groups connect the molecule to gold electrodes that are fabricated by…

介观与纳米尺度物理 · 物理学 2009-11-11 H. B. Heersche , Z. de Groot , J. A. Folk , H. S. J. van der Zant , C. Romeike , M. R. Wegewijs , L. Zobbi , D. Barreca , E. Tondello , A. Cornia

Spin is a fundamental property of any many-electron system. The ability of density functional theory to accurately predict the physical properties of a system, while varying its spin, is crucial for describing magnetic materials and…

化学物理 · 物理学 2024-11-05 Alon Hayman , Eli Kraisler , Tamar Stein

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin…

介观与纳米尺度物理 · 物理学 2013-05-29 Florian Elste , Carsten Timm

An electron transport is studied in the system which consists of scanning tunneling microscopy-single molecule magnet-metal. Due to quantum tunneling of magnetization in single-molecule magnet, linear response conductance exhibits stepwise…

介观与纳米尺度物理 · 物理学 2009-11-10 Gwang-Hee Kim , Tae-Suk Kim

We present a theoretical study of momentum-resolved tunneling between parallel two-dimensional conductors whose charge carriers have a (pseudo-)spin-1/2 degree of freedom that is strongly coupled to their linear orbital momentum. Specific…

介观与纳米尺度物理 · 物理学 2013-12-12 L. Pratley , U. Zuelicke

We calculate the tunneling splittings in a Mn$_{12}$ magnetic molecule taking into account its internal many-spin structure. We discuss the precision and reliability of these calculations and show that restricting the basis (limiting the…

介观与纳米尺度物理 · 物理学 2009-10-31 H. A. De Raedt , A. H. Hams , V. V. Dobrovitski , M. Al-Saqer , M. I. Katsnelson , B. N. Harmon

A density-functional formalism for superconductivity {\em and} magnetism is presented. The resulting relations unify previously derived Kohn-Sham equations for superconductors and for non-collinear magnetism. The formalism, which…

材料科学 · 物理学 2008-11-24 Jorge Quintanilla , Klaus Capelle , Luiz N. Oliveira

Scanning tunneling spectroscopy measures how a single electron with definite energy propagates between a sample surface and the tip of a scanning tunneling microscope. In the simplest description, the differential conductance measured is…

介观与纳米尺度物理 · 物理学 2019-05-07 Mikko M. Ervasti , Fabian Schulz , Peter Liljeroth , Ari Harju

We propose cotunneling as the microscopic mechanism that makes possible inelastic electron spectroscopy of magnetic atoms in surfaces for a wide range of systems, including single magnetic adatoms, molecules and molecular stacks. We…

介观与纳米尺度物理 · 物理学 2011-08-26 F. Delgado , J. Fernández-Rossier

Spin tunneling in molecular magnets has attracted much attention, however theoretical considerations of this phenomenon up to now have not taken into account the many-spin nature of molecular magnets. We present, to our knowledge, the first…

材料科学 · 物理学 2009-10-31 M. Al-Saqer , V. V. Dobrovitski , B. N. Harmon , M. I. Katsnelson

Electron transport properties in nanostructures can be modeled, for example, by using the semiclassical Wigner formalism or the quantum mechanical Green's functions formalism. We compare the performance and the results of these methods in…

介观与纳米尺度物理 · 物理学 2009-11-10 Paula Havu , Noora Tuomisto , Riikka Vaananen , Martti J. Puska , Risto M. Nieminen

We explore multi-terminal quantum transport through a benzene molecule threaded by an Aharonov-Bohm flux $\phi$. A simple tight-binding model is used to describe the system and all the calculations are done based on the Green's function…

介观与纳米尺度物理 · 物理学 2010-06-22 Santanu K. Maiti

We present a theory of tunneling and resonant transitions in one-dimensional molecular systems which is based on Green's function theory of electron sub-barrier scattering off the structural units (or functional groups) of a molecular…

其他凝聚态物理 · 物理学 2007-05-23 I. I. Oleynik , M. A. Kozhushner , V. S. Posvyanskii

The electron transport properties of a four-terminal molecular device are computed within the framework of density functional theory and non-equilibrium Keldysh theory. The additional two terminals lead to new properties, including a…

介观与纳米尺度物理 · 物理学 2009-09-01 Kamal K. Saha , Wenchang Lu , J. Bernholc , Vincent Meunier

We present a theory of single-electron tunneling transport through a ferromagnetic nanoparticle in which particle-hole excitations are coupled to spin collective modes. The model employed to describe the interaction between quasiparticles…

介观与纳米尺度物理 · 物理学 2009-11-11 L. Michalak , C. M. Canali , V. G. Benza

We investigate electron transport through a mono-atomic wire which is tunnel coupled to two electrodes and also to the underlying substrate. The setup is modeled by a tight-binding Hamiltonian and can be realized with a scanning tunnel…

介观与纳米尺度物理 · 物理学 2010-11-25 Tomasz Kwapinski , Sigmund Kohler , Peter Hanggi

The spin-polarized transport is investigated in a new type of magnetic tunnel junction which consists of two ferromagnetic electrodes separated by a magnetic barrier and a nonmagnetic metallic spacer. Based on the transfer matrix method and…

介观与纳米尺度物理 · 物理学 2009-11-10 Ali A. Shokri , Alireza Saffarzadeh

We propose a model to explore the dynamics of spin-systems coupled by exchange interaction to the conduction band electrons of a semiconductor material that forms the channel in a ferromagnet/semiconductor/ferromagnet spin-valve structure.…

介观与纳米尺度物理 · 物理学 2008-11-04 L. Siddiqui , D. Saha , S. Datta , P. Bhattacharya

We do parametric calculations to elucidate multi-terminal electron transport properties through a molecular system where a single phenalenyl molecule is attached to semi-infinite one-dimensional metallic leads. A formalism based on the…

介观与纳米尺度物理 · 物理学 2010-05-25 Paramita Dutta , Santanu K. Maiti , S. N. Karmakar
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