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Photoassociation of two ultracold rubidium atoms and the subsequent formation of stable molecules in the singlet ground and lowest triplet states is investigated theoretically. The method employs laser pulses inducing transitions via…

原子物理 · 物理学 2007-05-23 Christiane P. Koch , Ronnie Kosloff , Françoise Masnou-Seeuws

Two-color photoassociation of ground state $^6$Li$^{87}$Rb molecules via the $\mathrm{B}^1\Pi$ electronic state using short pulses near a magnetic Feshbach resonance is studied theoretically. A near-resonant magnetic field is applied to mix…

原子物理 · 物理学 2014-02-04 Marko Gacesa , Subhas Ghosal , Jason Byrd , Robin Côté

We model the formation of stable heteronuclear molecules via pulsed Raman photoassociation of a two-component Bose-Einstein condensate near a strong Feshbach resonance, for both counterintuitive and intuitive pulse sequencing. Compared to…

原子物理 · 物理学 2011-10-14 Matt Mackie , Pierre Phou , Heather Boyce , Mannix Shinn , Lev Katz

Photoassociation of ultracold atoms is a resonant light-assisted collision process, in which two colliding atoms absorb a photon and form an excited molecule. Since the first observation about three decades ago, the photoassociation of…

原子物理 · 物理学 2024-03-19 Jin Cao , Bo-Yuan Wang , Huan Yang , Zhi-Jie Fan , Zhen Su , Jun Rui , Bo Zhao , Jian-Wei Pan

This review describes recent experimental and theoretical advances in forming molecules in ultracold gases of trapped alkali metal atoms, both by magnetic tuning through Feshbach resonances and by photoassociation. Molecular Bose-Einstein…

化学物理 · 物理学 2007-05-23 Jeremy M. Hutson , Pavel Soldan

The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic)…

量子物理 · 物理学 2009-07-23 M. Vatasescu

We propose to create ultracold ground state molecules in an atomic Bose-Einstein condensate by adiabatic crossing of an optical Feshbach resonance. We envision a scheme where the laser intensity and possibly also frequency are linearly…

量子物理 · 物理学 2007-05-23 Christiane P. Koch Françoise Masnou-Seeuws Ronnie Kosloff

We observe the dynamic formation of $Cs_2$ molecules near Feshbach resonances in a cold sample of atomic cesium using an external probe beam. This method is 300 times more sensitive than previous atomic collision rate methods, and allows us…

凝聚态物理 · 物理学 2016-08-16 Cheng Chin , Andrew J. Kerman , Vladan Vuletić , Steven Chu

We study collisions in an optically trapped, pure sample of ultracold Cs$_2$ molecules in various internal states. The molecular gas is created by Feshbach association from a near-degenerate atomic gas, with adjustable temperatures in the…

量子气体 · 物理学 2015-05-13 F. Ferlaino , S. Knoop , M. Berninger , M. Mark , H. -C. Naegerl , R. Grimm

We reveal the existence of high-density Feshbach resonances in the collision between the ground and metastable states of $^{171}$Yb and coherently produce the associated Feshbach molecules by photoassociation. The extremely small transition…

原子物理 · 物理学 2016-02-01 Shintaro Taie , Shunsuke Watanabe , Tomohiro Ichinose , Yoshiro Takahashi

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

量子物理 · 物理学 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

We propose an improved photoassociation scheme to produce ultracold molecules in their vibronic ground state for the generic case where non-adiabatic effects facilitating transfer to deeply bound levels are absent. Formation of molecules is…

原子物理 · 物理学 2008-10-28 Christiane P. Koch , Robert Moszynski

Photoassociation with short laser pulses has been proposed as a technique to create ultracold ground state molecules. A broad-band excitation seems the natural choice to drive the series of excitation and deexcitation steps required to form…

原子物理 · 物理学 2010-09-21 Christiane P. Koch , Mamadou Ndong , Ronnie Kosloff

Photoassociation and the Feshbach resonance are, in principle, feasible means for creating a molecular Bose-Einstein condensate from an already-quantum-degenerate gas of atoms; however, mean-field shifts and irreversible decay place…

原子物理 · 物理学 2009-11-07 Matt Mackie

We show theoretically that it is possible to create and manipulate a pair of bound states in continuum in ultracold atoms by two lasers in the presence of a magnetically tunable Feshbach resonance. These bound states are formed due to…

原子与分子团簇 · 物理学 2016-09-15 Bimalendu Deb , G. S. Agarwal

We analyze the formation of Rb_2 molecules with short photoassociation pulses applied to a cold Rb-85 sample. A pump laser pulse couples a continuum level of the ground electronic state X ^1\Sigma_{g}^+ with bound levels in the 0_{u}^+…

原子物理 · 物理学 2007-06-22 Jordi Mur-Petit , Eliane Luc-Koenig , Françoise Masnou-Seeuws

The Formation of metastable molecules (Feshbach resonances) at the collision of two atoms and subsequent stimulated transition to a lower unbound electronic molecular state, with emission of a photon of the laser radiation has been…

原子物理 · 物理学 2017-04-05 E. Gazazyan , A. Gazazyan

We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…

原子物理 · 物理学 2026-01-14 Emanuel F. de Lima

This theoretical paper investigates the formation of ground state molecules from ultracold cesium atoms in a two-color scheme. Following previous work on photoassociation with chirped picosecond pulses [Luc-Koenig et al., Phys. Rev. A {\bf…

原子物理 · 物理学 2007-05-23 Christiane P. Koch , Eliane Luc-Koenig , Françoise Masnou-Seeuws

We develop a complete theoretical description of photoassociative Stimulated Raman Adiabatic Passage (STIRAP) near a Feshbach resonance in a thermal atomic gas. We show that it is possible to use low intensity laser pulses to directly…

量子物理 · 物理学 2015-05-13 Elena Kuznetsova , Susanne F. Yelin , Marko Gacesa , Philippe Pellegrini , Robin Côté
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