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Relaxation dynamics of embedded metal nanoparticles after ultrafast laser pulse excitation is driven by thermal phenomena of different origins the accurate description of which is crucial for interpreting experimental results: hot electron…

材料科学 · 物理学 2009-11-13 Majid Rashidi-Huyeh , Sebastian Volz , Bruno Palpant

The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measured, by means of ultrafast time-resolved photoemission spectroscopy induced by extreme-ultraviolet radiation pulses. The temperature of the…

We explore the influence of the nanoporous structure on the thermal relaxation of electrons and holes excited by ultrashort laser pulses ($\sim 7$ fs) in thin gold films. Plasmon decay into hot electron-hole pairs results in the generation…

Ultrafast laser material processing has received significant attention due to a growing need for the fabrication of miniaturized devices at micro- and nanoscales. The traditional phenomenological laws, such as Fourier's law of heat…

计算物理 · 物理学 2015-11-12 Yuwen Zhang , D. Y. Tzou , J. K. Chen

Core-shell nanoparticles, particularly those having a gold core, have emerged as a highly promising class of materials due to their unique optical and thermal properties, which underpin a wide range of applications in photothermal therapy,…

计算物理 · 物理学 2025-06-06 Julien El Hajj , Gilles Ledoux , Samy Merabia

A method is proposed for determining the temperature of hot electrons in a metallic nanoparticle embedded in a dielectric matrix under ultrashort laser pulses irradiation. The amplitude and power of the longitudinal spherical acoustic…

介观与纳米尺度物理 · 物理学 2017-12-15 N. I. Grigorchuk

Transient absorption spectroscopy is routinely used to study the electron dynamics in plasmonic gold nanoparticles. Typically, the transient absorption bleach is analyzed as measure for the electron temperature. However, the implicitly…

介观与纳米尺度物理 · 物理学 2026-03-30 Nour E. H. Chetoui , Jonas Grumm , Robert Lemke , Andreas Knorr , Holger Lange

Efficient mixing and pumping of liquids at the microscale is a technology that is still to be optimized. The combination of an AC electric field with a small temperature gradient leads to a strong electro-thermal flow that can be used for…

流体动力学 · 物理学 2024-03-18 Carlos David González Gómez , Raúl A. Rica , Emilio Ruiz-Reina

The structural evolution of laser-excited systems of gold has previously been measured through ultrafast MeV electron diffraction. However, there has been a long-standing inability of atomistic simulations to provide a consistent picture of…

材料科学 · 物理学 2024-06-19 J. M. Molina , T. G. White

We investigate melting and undercooling in nanoscale (radius ~100 nm) gold particles that are levitated in a quadrupole ion (Paul) trap in a high vacuum environment. The particle is heated via laser illumination and probed using two main…

介观与纳米尺度物理 · 物理学 2022-01-27 Joyce Coppock , Quinn Waxter , Robert Wolle , B. E. Kane

We propose a new approach to understand the time-dependent temperature increasing process of gold-silica core-shell nanoparticles injected into chicken tissues under near-infrared laser irradiation. Gold nanoshells strongly absorb…

介观与纳米尺度物理 · 物理学 2018-04-04 Vu T. T. Duong , Anh D. Phan , Nghiem T. H. Lien , Do T. Hue , Do Q. Hoa , Do T. Nga , Tran H. Nhung , Nguyen A. Viet

In this paper, we present a simple and robust numerical method able to predict, with high accuracy, the photo-thermal effects occurring for a gold nanoparticles arrangement under externally applied strain. The physical system is numerically…

应用物理 · 物理学 2020-09-08 Giuseppe E. Lio , Giovanna Palermo , Antonio De Luca , Roberto Caputo

Photoexcitation of metallic nanostructures with short optical pulses can drive non-thermal electronic states, which, upon decay, lead to elevated electronic temperatures ($T_e \gtrapprox 1000\,\mathrm{K}$) eventually equilibrating with the…

介观与纳米尺度物理 · 物理学 2025-01-07 Qian Ye , Stephen K. Sanders , Andrea Schirato , Alessandro Alabastri

A sample-based stochastic model is presented to investigate the effects of uncertainties of various input parameters, including laser fluence, laser pulse duration, thermal conductivity constants for electron, and electron-lattice coupling…

计算物理 · 物理学 2016-04-28 Nazia Afrin , Yuwen Zhang , J. K. Chen

The ultrafast laser-induced solid-liquid phase transition in metals is still not clearly understood and its accurate quantitative description remains a challenge. Here we systematically investigated, both experimentally and theoretically,…

The work is dedicated to the development of the electron-lattice energy exchange theory in metal particles and it dependence of on particle size and electron temperature. We obtained the expressions for the constants of the electron-lattice…

介观与纳米尺度物理 · 物理学 2015-06-19 Petro Tomchuk , Yevgen Bilotsky

The thermal dynamics induced by ultrashort laser pulses in nanoscale systems, i.e. all-optical time-resolved nanocalorimetry is theoretically investigated from 300 to 1.5 K. We report ab-initio calculations describing the temperature…

介观与纳米尺度物理 · 物理学 2015-03-13 F. Banfi , F. Pressacco , B. Revaz , C. Giannetti , D. Nardi , G. Ferrini , F. Parmigiani

The electrons and phonons in metal films after ultra-short pulse laser heating are in highly non-equilibrium states not only between the electron sub-system and the phonon sub-system but also within the electron sub-system. An…

材料科学 · 物理学 2014-08-05 Jun Zhou , Nianbei Li , Ronggui Yang

The simulation and analysis of the thermal stability of nanoparticles, a stepping stone towards their application in technological devices, require fast and accurate force fields, in conjunction with effective characterisation methods. In…

The radiative heat transfer between gold nanoparticle layers is presented using the coupled dipole method. Gold nanoparticles are modelled as effective electric and magnetic dipoles interacting via electromagnetic fluctuations. The effect…

介观与纳米尺度物理 · 物理学 2013-12-05 Anh D. Phan , The-Long Phan , Lilia M. Woods
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