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We consider tunneling transport through a Mn$_{12}$ molecular magnet using spin density functional theory. A tractable methodology for constructing many-body wavefunctions from Kohn-Sham orbitals allows for the determination of…

介观与纳米尺度物理 · 物理学 2010-02-08 L. Michalak , C. M. Canali , M. R. Pederson , M. Paulsson , V. G. Benza

Density-functional theory for superfluid systems is developed in the framework of the functional renormalization group based on the effective action formalism. We introduce the effective action for the particle-number and nonlocal pairing…

核理论 · 物理学 2021-05-11 Takeru Yokota , Haruki Kasuya , Kenichi Yoshida , Teiji Kunihiro

A novel approach to the description of superconductors in thermal equilibrium is developed within a formally exact density-functional framework. The theory is formulated in terms of three ``densities'': the ordinary electron density, the…

We present a first-principles approach to describe magnetic and superconducting systems and the phenomena of competition between these electronic effects. We develop a density functional theory: SpinSCDFT, by extending the Hohenberg-Kohn…

超导电性 · 物理学 2016-05-10 A. Linscheid , A. Sanna , F. Essenberger , E. K. U. Gross

A new formalism to describe steady-state electronic and thermal transport in the framework of density functional theory is presented. A one-to-one correspondence is proven between the three basic variables of the theory, i.e., the density…

介观与纳米尺度物理 · 物理学 2022-04-26 Nahual Sobrino , Florian Eich , Gianluca Stefanucci , Roberto D'Agosta , Stefan Kurth

Two electrons at the threshold of ionization represent a severe test case for electronic structure theory. A pseudospectral method yields a very accurate density of the two-electron ion with nuclear charge close to the critical value.…

化学物理 · 物理学 2014-08-12 Paul E. Grabowski , Kieron Burke

In the framework of density functional theory a formalism to describe electronic transport in the steady state is proposed which uses the density on the junction and the {\em steady current} as basic variables. We prove that, in a finite…

介观与纳米尺度物理 · 物理学 2016-01-12 G. Stefanucci , S. Kurth

The dissociation of molecules, even the most simple hydrogen molecule, cannot be described accurately within density functional theory because none of the currently available functionals accounts for strong on-site correlation. This problem…

强关联电子 · 物理学 2011-01-14 N. Helbig , I. V. Tokatly , A. Rubio

We employ the density functional Kohn-Sham method in the local spin-density approximation to study the electronic structure and magnetism of quasi one-dimensional periodic arrays of few-electron quantum dots. At small values of the lattice…

介观与纳米尺度物理 · 物理学 2015-06-25 K. Karkkainen , M. Koskinen , S. M. Reimann , M. Manninen

Current-carrying and superconducting systems can be treated within density-functional theory if suitable additional density variables (the current density and the superconducting order parameter, respectively) are included in the…

材料科学 · 物理学 2009-11-07 K. Capelle , G. Vignale

We present an \textit{ab initio} theory for superconductors, based on a unique mapping between the statistical density operator at equilibrium, on the one hand, and the corresponding one-body reduced density matrix $\gamma$ and the…

超导电性 · 物理学 2019-06-06 Jonathan Schmidt , Carlos L. Benavides-Riveros , Miguel A. L. Marques

We use the exact strong-interaction limit of the Hohenberg-Kohn energy density functional to construct an approximation for the exchange-correlation term of the Kohn-Sham approach. The resulting exchange-correlation potential is able to…

We use the exact strong-interaction limit of the Hohenberg-Kohn energy density functional to approximate the exchange-correlation energy of the restricted Kohn-Sham scheme. Our approximation corresponds to a highly non-local density…

强关联电子 · 物理学 2012-12-12 Francesc Malet , Paola Gori-Giorgi

We consider the pairing Hamiltonian and systematically construct its density functional in the strong-coupling limit and in the limit of large particle number. In the former limit, the functional is an expansion into central moments of…

核理论 · 物理学 2008-11-26 T. Papenbrock , Anirban Bhattacharyya

While in principle exact, Kohn-Sham density functional theory -- the workhorse of computational chemistry -- must rely on approximations for the exchange-correlation functional. Despite staggering successes, present-day approximations still…

A recently developed formalism in which Kohn-Sham calculations are combined with an ``average pair density functional theory'' is reviewed, and some new properties of the effective electron-electron interaction entering in this formalism…

材料科学 · 物理学 2009-11-11 Paola Gori-Giorgi , Andreas Savin

A theory of the proximity effect in normal metal - multiband superconductor hybrid structures is formulated within the quasiclassical Green's function formalism. It is shown that the existence of multiple superconducting bands manifests…

超导电性 · 物理学 2009-11-10 A. Brinkman , A. A. Golubov , M. Yu. Kupriyanov

Most approximate exchange-correlation functionals used within density functional theory are constructed as the sum of two distinct contributions for exchange and correlation. Separating the exchange component from the entire functional is…

凝聚态物理 · 物理学 2009-10-28 Claudia Filippi , C. J. Umrigar , Xavier Gonze

The effect of the barrier on the proximity effect in normal-superconductor junction is analyzed. A general criterion for the barrier, though large, to be effectively transparent, is given. This criterion is applied to both the conductance…

超导电性 · 物理学 2008-02-03 M. Schechter , Y. Imry , Y. Levinson

We present an alternative to the Kohn-Sham formulation of density functional theory for the ground-state properties of strongly interacting electronic systems. The idea is to start from the limit of zero kinetic energy and systematically…

强关联电子 · 物理学 2015-05-13 Paola Gori-Giorgi , Michael Seidl , G. Vignale
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