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Low energy inelastic neutron scattering on single crystals of the kagome spin liquid compound ZnCu3(OD)6Cl2 (Herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers E < 0.8 meV (~J/20). The…

The dc-magnetization of the unique S=1/2 kagome antiferromagnet Herbertsmithite has been measured down to 0.1K. No sign of spin freezing is observed in agreement with former muSR and ac-susceptibility results. The low temperature magnetic…

强关联电子 · 物理学 2009-11-13 F. Bert , S. Nakamae , F. Ladieu , D. L'Hôte , P. Bonville , F. Duc , J. -C. Trombe , P. Mendels

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling…

强关联电子 · 物理学 2010-04-07 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Qiu , D. G. Nocera , Y. S. Lee

Local magnetic properties around a nonmagnetic impurity are investigated in high-Tc cuprate superconductors. We consider a model two-dimensional d-wave superconductor with strong antiferromagnetic (AF) spin fluctuations and calculate the…

超导电性 · 物理学 2009-11-07 Y. Ohashi

We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices---barlowite Cu$_{4}$(OH)$_{6}$FBr. Magnetic susceptibility gives $\theta_{CW}$ = $-$136 K, while long-range order does not happen…

强关联电子 · 物理学 2014-12-05 Tian-Heng Han , John Singleton , John A. Schlueter

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

We analyze the experimental data for the magnetic susceptibility of the material ZnCu3(OH)6Cl2 in terms of the Kagome Lattice Heisenberg model (KLHM), discussing possible role of impurity spins, dilution, exchange anisotropy, and both…

强关联电子 · 物理学 2007-05-23 Marcos Rigol , Rajiv R. P. Singh

The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of great debate. We conducted 17-O single crystal NMR…

强关联电子 · 物理学 2015-11-09 M. Fu , T. Imai , T. -H. Han , Y. S. Lee

The local response to a uniform field around vacancies in the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet is determined by numerical quantum Monte Carlo simulations as a function of temperature. It is possible to separate the…

强关联电子 · 物理学 2009-11-11 Fabrizio Anfuso , Sebastian Eggert

Two kagome compounds, volborthite Cu3V2O7(OH)2-2H2O and herbertsmithite ZnCu3(OH)6Cl2, are compared in order to derive information about the intrinsic properties of the spin-1/2 kagome antiferromagnet. Volborthite shows a broad maximum at T…

强关联电子 · 物理学 2009-11-13 Z Hiroi , H Yoshida , Y Okamoto , M Takigawa

We analyse the antiferromagnetic spin-$1/2$ XXZ model on the kagome lattice at finite external magnetic field with the help of a nonperturbative zero-temperature renormalization group (RG) technique. Following the work of Kumar \emph{et al}…

强关联电子 · 物理学 2019-09-30 Santanu Pal , Anirban Mukherjee , Siddhartha Lal

We report muon spin rotation measurements of the local magnetic susceptibility around a positive muon in the paramagnetic state of the quasi one-dimensional spin 1/2 antiferromagnet dichlorobis (pyridine) copper (II). Signals from three…

We report results of magnetic susceptibility and 51V- and 63,65Cu-NMR measurements on a high-quality powder sample of vesignieite BaCu3V2O8(OH)2, a candidate for the spin-1/2 kagome antiferromagnet. We observed a twostep magnetic…

强关联电子 · 物理学 2017-12-01 Makoto Yoshida , Yoshihiko Okamoto , Masashi Takigawa , Zenji Hiroi

Kagome lattice Heisenberg antiferromagnets are known to be highly sensitive to perturbations caused by structural disorder. NMR is a local probe ideally suited for investigating such disorder-induced effects, but in practice large…

强关联电子 · 物理学 2023-01-09 Weishi Yuan , Jiaming Wang , Philip M. Singer , Rebecca W. Smaha , Jiajia Wen , Young S. Lee , Takashi Imai

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

强关联电子 · 物理学 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

The Dirac spin liquid ground state of the spin 1/2 Heisenberg kagome antiferromagnet has potential instabilities[1-4]. This has been suggested as the reason why it is not strongly supported in large-scale numerical calculations[5]. However,…

强关联电子 · 物理学 2013-11-13 Bryan Clark , Jesse Kinder , Eric Neuscamman , Garnet Kin-Lic Chan , Michael J. Lawler

Low-energy spin dynamics is investigated by $^{35}$ Cl NMR measurements in a frustrated antiferromagnet Ca$_3$ReO$_5$Cl$_2$. The local spin susceptibility measured with the Knight shift behaves as a one-dimensional Heisenberg…

We have successfully synthesized S = 1/2 kagome antiferromagnets MCu3(OH)6Cl2 (M = Ni and Co) by hydrothermal method with rotating pressure vessel. Structural characterization shows that both compounds have the similar crystal structure as…

强关联电子 · 物理学 2012-12-10 Yue-sheng Li , Qing-ming Zhang

We consider a magnetic impurity in the antiferromagnetic spin-1/2 chain which is equivalent to the two-channel Kondo problem in terms of the field theoretical description. Using a modification of the transfer-matrix density matrix…

强关联电子 · 物理学 2009-10-31 Sebastian Eggert , Stefan Rommer

We systematically study the low-temperature specific heats for the two-dimensional kagome antiferromagnet, Cu$_{3}$Zn(OH)$_6$FBr. The specific heat exhibits a $T^{1.7}$ dependence at low temperatures and a shoulder-like feature above it. We…