相关论文: Control of Four-Level Quantum Coherence via Discre…
We demonstrate high resolution coherent control of cold atomic Rubidium utilizing spectral phase manipulation of a femtosecond optical frequency comb. Transient coherent accumulation is directly manifested by the enhancement of signal…
Coherent control is an optical technique to manipulate quantum states of matter. The coherent control of 40-THz optical phonons in diamond was demonstrated by using a pair of sub-10-fs optical pulses. The optical phonons were detected via…
Optical frequency combs are laser sources which are capable of generating discrete, equal-spaced and highly coherent comb modes. Optical frequency comb technique provides a significant bridge to transfer the stability between optical…
We demonstrate the use of an optical frequency comb to coherently control and entangle atomic qubits. A train of off-resonant ultrafast laser pulses is used to efficiently and coherently transfer population between electronic and…
Quantum coherent control (1-3) is a powerful tool for steering the outcome of quantum processes towards a desired final state, by accurate manipulation of quantum interference between multiple pathways. Although coherent control techniques…
We demonstrate the use of a femtosecond frequency comb to coherently drive stimulated Raman transitions between terahertz-spaced atomic energy levels. More specifically, we address the $3d~^2D_{3/2}$ and $3d~^2D_{5/2}$ fine structure levels…
A symmetric four-level closed-loop $\diamondsuit$ type (the diamond structure) atomic system driven by four coherent optical fields is investigated. The system shows rich quantum interference and coherence features. When symmetry of the…
Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…
From the interaction between a frequency comb and an atomic qubit, we derive quantum protocols for the determination of the carrier-envelope offset phase, using the qubit coherence as a reference, and without the need of frequency doubling…
Optical frequency comb devices have unlocked new capabilities in telecommunications, sensing, and metrology. Yet, precise in situ control of the comb spectral envelope remains extremely challenging. By introducing mode coupling with…
Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…
We demonstrated the observation of Rb two-photon absorption directly excided by an optical frequency comb at fiber communication bands. A chain of comb spectral control is elaborately implemented to increase the power of the second harmonic…
We present a general and highly efficient scheme for performing narrow-band Raman transitions between molecular vibrational levels using a coherent train of weak pump-dump pairs of shaped ultrashort pulses. The use of weak pulses permits an…
A general mechanism for the generation of frequency combs referenced to atomic resonances is put forward. The mechanism is based on the periodic phase control of a quantum system's dipole response. We develop an analytic description of the…
Sustained mutual coherence between two combs over extended periods is a prerequisite for dual-comb spectroscopy (DCS), particularly in achieving high-resolution molecular spectroscopy and precise spectral measurements. However, achieving…
The counting and control of optical cycles of light has become common with modelocked laser frequency combs. But even with advances in laser technology, modelocked laser combs remain bulk-component devices that are hand-assembled. In…
Optical frequency combs, coherent light sources that connect optical frequencies with microwave oscillations, have become the enabling tool for precision spectroscopy, optical clockwork and attosecond physics over the past decades. Current…
We describe how an ensemble of four-level atoms in the diamond-type configuration can be applied to create a fully controllable effective coupling between two cavity modes. The diamond-type configuration allows one to use a bimodal cavity…
We discuss femtosecond Raman type techniques to control molecular vibrations, which can be implemented for internal state cooling from Feshbach states with the use of optical frequency combs with and without modulation. The technique makes…
Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…