相关论文: EPR and magnetization studies on single crystals o…
The crystalline electric field (CEF) is investigated in Pr$_3$Pt$_{23}$Si$_{11}$ and Nd$_3$Pt$_{23}$Si$_{11}$ by neutron spectroscopy (NS). At low temperature, the number of observed CEF excitations is consistent with the orthorhombic…
The ground states and finite-temperature properties of mixed diamond chains with spins 1 and 1/2 are investigated in the limit of strong easy-axis anisotropy on the spin-1 sites. Magnetization curves, entropy, specific heat and magnetic…
The Eu{+2} spins S = 7/2 in the metallic compound EuCo{2-y}As2 order into an antiferromagnetic helical structure below a Neel temperature TN = 40 to 45 K. The effective magnetic moment mu_eff of the Eu spins in the paramagnetic state from…
We present a microscopic theory of single molecule magnets. From our exact single-ion spin matrix elements for four arbitrary spins, we study the single-ion anisotropy of equal spins exhibiting $T_d$, $D_{2d}$, or $C_{4v}$ molecular group…
Despite extensive research on the skutterudites for the last decade, their electric crystalline field ground state is still a matter of controversy. We show that Electron Spin Resonance (ESR) measurements can determine the full set of…
Crystal field level scheme of a uniaxial chiral helimagnet YbNi$_3$Al$_9$, exhibiting a chiral magnetic soliton lattice state by Cu substitution for Ni, has been determined by inelastic neutron scattering. The ground and the first excited…
We report a combined experimental and theoretical study on intriguing magnetic properties of quasiferroelectric orthochromates. Large single crystals of the family of RECrO$_3$ (RE = Y, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, and Lu) compounds were…
It is shown that our multi-high-frequency (40-200 GHz) resonant cavity technique yields distortion-free high field EPR spectra for single crystal samples of the uniaxial and biaxial spin S = 10 single molecule magnets (SMMs)…
Although low-dimensional $S = 1$ antiferromagnets remain of great interest, difficulty in obtaining high-quality single crystals of the newest materials hinders experimental research in this area. Polycrystalline samples are more readily…
We study theoretically Electron Paramagentic Resonance (EPR) linewidths for single crystals of the molecular magnets Fe$_8$ and Mn$_{12}$ as functions of energy eigenstates $M_s$, frequency, and temperature when a magnetic field along the…
Single crystal of PrSi was grown by Czochralski method in a tetra-arc furnace. Powder x-ray diffraction of the as grown crystal revealed that PrSi crystallizes in FeB$-$type structure with space group $Pnma$ (no. 62). PrSi undergoes a…
Magnetic properties of high-quality Al-free nonsuperconducting GdBa_2Cu_3O_{6+y} single crystals grown by flux method have been studied. The magnetic anisotropy below the N\'eel temperature T_N~2.3K corresponds to the direction of Gd^{3+}…
CeCd$_3$P$_3$ and CeCd$_3$As$_3$ compounds adopt the hexagonal ScAl$_3$C$_3$-type structure, where magnetic Ce ions on a triangular lattice order antiferromagnetically below $T_\text{N} \sim$0.42~K. Their crystalline electric field (CEF)…
As one of typical layered structures, antiferromagnetic CuCrP$_{2}$S$_{6}$ single crystal has high potential for magnetoelectric devices and spintronic multi-terminal chips due to its unique magnetic anisotropy. However, to tune the…
An indispensable step toward understanding magnetic interactions in rare-earth magnets is to determine the spatially anisotropic single-ion properties set by crystal electric field (CEF) physics. The CEF Hamiltonian yields a discrete energy…
We present a detailed study of magnetization, resistivity, heat capacity, and X-ray and neutron powder diffraction measurements performed on single crystals of non-stoichiometric CeAuBi$_2$, Au deficiency 18$\%$, a strongly correlated…
The experimental results on the magnetic response of YBCO single crystals with unidirectional twin boundary planes in low magnetic fields (0.01 - 1 Oe) are discussed. The observed non-monotone temperature dependence of magnetization is…
We have performed X-ray powder diffraction, magnetization, electrical resistivity, heat capacity and inelastic neutron scattering (INS) to investigate the physical properties of the intermetallic series of compounds CeCuBi$_{2-x}$Sb$_{x}$.…
The magnetization, crystal structure, and thermal expansion of a nearly stoichiometric Sr$_{1.04(3)}$Er$_{2.09(6)}$O$_{4.00(1)}$ single crystal have been studied by PPMS measurements and in-house and high-resolution synchrotron X-ray powder…
We present angle-dependent high-frequency EPR studies on a single-crystal of a trigonal Mn3 cluster with an unusual structure in which the local magnetic easy-axes of the constituent Mn(III) ions are tilted significantly away from the…