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We study how spin and orbital effects influence the capability of promoting Dzyaloshinskii-Moriya (DM) interaction by studying the two magnetic polar materials, Cu(IO3)2 (S = 1/2 with orbital contribution) and Mn(IO3)2 (S = 5/2 with…

We report the magnetic and electronic properties of the bilayer ruthenate Sr$_3$Ru$_2$O$_7$ upon Fe substitution for Ru. We find that Sr$_3$(Ru$_{1-x}$Fe$_x$)$_2$O$_7$ shows a spin-glass-like phase below 4 K for $x$ = 0.01 and commensurate…

强关联电子 · 物理学 2018-02-21 M. Zhu , Y. Wang , P. G. Li , J. J. Ge , W. Tian , D. Keavney , Z. Q. Mao , X. Ke

Effects of Sr substitution at A-site in ordered perovskite Ba3-xSrxMnNb2O9 (x = 1 and 3) have been investigated using X-ray diffraction, magnetization, dielectric/magnetodielectric and neutron diffraction measurements. The parent compound…

强关联电子 · 物理学 2020-06-24 Shivani Sharma , Premakumar Yanda , Poonam Yadav , Ivan da Silva , A. Sundaresan

The properties of AMO3 perovskite oxides, where M is a 3d transition metal, depend strongly on the level of covalency between the metal d and oxygen p orbitals. With their complex spin orders and metal-insulator transition, rare-earth…

Contrary to conventional wisdom, our purified La2-2xSr1+2xMn2O7 crystals exhibit CE-type orbital and charge order as the low-temperature ground state for a hole doping level h = 0.5. For small deviations from h = 0.5, the high temperature…

Tetragonal distorted spinel of CuMn2-xTixO4 (x = 0, 0.25 and 0.50) was prepared by solid state reaction method followed by neutron diffraction, FTIR spectroscopy, dielectric spectroscopy and magnetization measurements. The neutron…

材料科学 · 物理学 2020-12-01 P. Patra , I. Naik , S. D. Kaushik , S. Mohanta

We report a x-ray resonant diffraction study of the perovskite Pr0.6Ca0.4MnO3. At the Mn K-edge, this technique is sensitive to details of the electronic structure of the Mn atoms. We discuss the resonant x-ray spectra measured above and…

X-ray magnetic circular dichroism spectroscopy has been used to characterize the electronic structure and magnetic moment of Cr$_2^+$. Our results indicate that the removal of a single electron from the $4s\sigma_g$ bonding orbital of…

Surface-adsorbed rare-earth nanostructures are ideal platforms to investigate the interplay between intra-atomic interactions and multi-orbital spin configurations. However, addressing these properties has posed severe experimental and…

The conduction electrons in a metal experience competing interactions with each other and the atomic nuclei. This competition can lead to many types of magnetic order in metals. For example, in chromium the electrons order to form a…

The compound, Nd7Rh3, crystallizing in Th7Fe3-type hexagonal structure, was previously known to exhibit two magnetic transitions, one at 32 K and the other at 10 K (in zero magnetic field). Here, we report the existence of a field-induced…

强关联电子 · 物理学 2009-11-11 Kausik Sengupta , E. V. Sampathkumaran

We have studied the effects of the isoelectronic substitution of Ru for Fe in polycrystalline samples of the spin density wave (SDW) material PrFeAsO. Crystal structures from powder x-ray diffraction at room temperature and transport…

超导电性 · 物理学 2009-08-05 Michael A. McGuire , David J. Singh , Athena S. Sefat , Brian C. Sales , David Mandrus

We investigate the behavior of low-energy electrons in two-dimensional molybdenum disulfide when submitted to an external magnetic field. Highly degenerate Landau levels form in the material, between which light-induced excitations are…

介观与纳米尺度物理 · 物理学 2013-10-22 Félix Rose , M. O. Goerbig , Frédéric Piéchon

Upon reduction of the film thickness we observe a metal-insulator transition in epitaxially stabilized, spin-orbit coupled SrIrO$_3$ ultrathin films. By comparison of the experimental electronic dispersions with density functional theory at…

Intrinsic antiferromagnetism in van der Waals (vdW) monolayer (ML) crystals enriches the understanding regarding two-dimensional (2D) magnetic orders and holds special virtues over ferromagnetism in spintronic applications. However, the…

Thickness driven electronic phase transitions are broadly observed in different types of functional perovskite heterostructures. However, uncertainty remains whether these effects are solely due to spatial confinement, broken symmetry or…

We report the investigations of crystal structure, electrical resistivity, magnetization, specific heat, thermal conductivity, and thermoelectric power (TEP) on La0.7Sr0.3(Mn1-xRux)O3 (LSMRO) compounds with x = 0 to 0.90. From the analyses…

强关联电子 · 物理学 2007-05-23 L. M. Wang. Jyh-Iuan Wu , Y. -K. Kuo

We have succeeded in establishing the crystal-field ground state of CeRu2Al10, an orthorhombic intermetallic compound recently identified as a Kondo insulator. Using polarization dependent soft x-ray absorption spectroscopy at the Ce M4,5…

We characterise optical transitions of neodymium ions (Nd3+) in antiferromagnetic neodymium gallate (NdGaO3) with applied fields up to 3 T. The magnetic phase of this material has not previously been studied with the field along its…

Controlling magnetism and spin structures in strongly correlated systems by using electric field is of fundamental importance but challenging. Here, a high-spin ruthenate phase is achieved via a solid ionic chemical junction at…