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Vibration properties of Zn(1-x)Be(x)Se, a mixed II-VI semiconductor haracterized by a high contrast in elastic properties of its pure constituents, ZnSe and BeSe, are simulated by first-principles calculations of electronic structure,…

材料科学 · 物理学 2009-11-10 A. V. Postnikov , Olivier Pages , Joseph Hugel

We apply standard, first-principles calculations to a complete treatment of lattice dynamics in the harmonic approximation. The algorithm makes use of the straightforward ``frozen-phonon'' approach to the calculation of vibrational spectra…

材料科学 · 物理学 2007-05-23 Hadley M. Lawler , Eric K. Chang , Eric L. Shirley

Ab initio calculations and a direct method are applied to derive the phonon dispersion relations and phonon density of states for the ZrC crystal. The results are in good agreement with neutron scattering data. The force constants are…

材料科学 · 物理学 2013-01-28 Paweł T. Jochym , Krzysztof Parlinski

The lattice dynamics in substitutional disordered alloys with constituents having large size differences is driven by strong disorder in masses, inter-atomic force constants and local environments. In this letter, a new first-principles…

材料科学 · 物理学 2016-08-14 Oscar Grånäs , Biswanath Dutta , Subhradip Ghosh , Biplab Sanyal

First-principles phonon calculations have been widely performed for studying vibrational properties of condensed matter, where the dynamical matrix is commonly constructed via supercell force-constant calculations or the linear response…

材料科学 · 物理学 2020-11-11 Chi-Cheng Lee , Chin-En Hsu , Hung-Chung Hsueh

Taking into account the constraints imposed by the lattice symmetry, the phonon dispersion is calculated for graphene with interactions between the first and second nearest neighbors in the framework of the Born-von Karman model. Analytical…

介观与纳米尺度物理 · 物理学 2009-11-13 L. A. Falkovsky

A reliable prediction of interatomic force constants in disordered alloys is an outstanding problem. This is due to the need for a proper treatment of multisite (atleast pair) correlation within a random environment. The situation becomes…

材料科学 · 物理学 2014-04-14 Rajiv K. Chouhan , Aftab Alam , Subhradip Ghosh , Abhijit Mookerjee

We present a lattice dynamics study of orthorhombic antimony sulphide (Sb2S3) obtained using density-functional calculations in conjunction with the supercell force-constant method. The effect of Born effective charges is taken into account…

材料科学 · 物理学 2016-07-06 Yun Liu , Kun Ting Eddie Chua , Tze Chien Sum , Chee Kwan Gan

We apply the compressive sensing lattice dynamics (CSLD) method to calculate phonon dispersion for crystalline solids. While existing methods such as frozen phonon, small displacement, and linear response are routinely applied for phonon…

材料科学 · 物理学 2019-11-25 Fei Zhou , Babak Sadigh , Daniel Aberg , Yi Xia , Vidvuds Ozolins

Estimating force constants for crystal structures is crucial for calculating various phonon-related properties. However, this task becomes particularly challenging when dealing with a large number of atoms or when third- and higher-order…

材料科学 · 物理学 2024-10-29 Atsuto Seko , Atsushi Togo

Lattice dynamics for several ordered supercells with composition PbMg1/3Nb2/3O (PMN) were calculated with first-principles frozen phonon methods. Nominal symmetries of the supercells studied are reduced by lattice instabilities. Lattice…

材料科学 · 物理学 2009-11-10 S. A. Prosandeev , E. Cockayne , E. P. Burton

For an fcc crystal with central force interactions and separately for a scalar model on a square lattice, we compute exactly the phonon transmission coefficient $T(\omega)$ through a disordered planar interface between two identical semi -…

凝聚态物理 · 物理学 2009-10-31 G. Fagas , A. G. Kozorezov , C. J. Lambert , J. K. Wigmore

Ab initio calculations and a direct method have been applied to derive the phonon dispersion curves and phonon density of states for the TiC crystal. The results are compared and found to be in a good agreement with the experimental neutron…

材料科学 · 物理学 2013-01-28 Paweł T. Jochym , Małgorzata Sternik , Krzysztof Parlinski

Lattice dynamics for five ordered PMN supercells were calculated from first principles by the frozen phonon method. Maximal symmetries of all supercells are reduced by structural instabilities. Lattice modes corresponding to these…

The lattice dynamics of AgPd, Ni55Pd45, Ni95Pt05, and Cu0.715Pd0.285 intermetallic have been investigated using the DFT calculation. The phonon dispersions and phonon densities of states along for two symmetry directions are calculated by…

材料科学 · 物理学 2020-08-24 M. Aziziha , S. Akbarshahi

Femtosecond optical pulses at mid-infrared frequencies have opened up the nonlinear control of lattice vibrations in solids. So far, all applications have relied on second order phonon nonlinearities, which are dominant at field strengths…

The nature of the lattice instability connected to the structural transition and superconductivity of (Sr,Ca)$_3$Ir$_4$Sn$_{13}$ is not yet fully understood. In this work density functional theory (DFT) calculations of the phonon…

超导电性 · 物理学 2014-02-20 David A. Tompsett

A new method for extracting force constants (FC) from first principles is introduced. It requires small supercells but very accurate forces. In principle, provided that forces are accurate enough, it can extract harmonic as well as…

材料科学 · 物理学 2007-10-31 Keivan Esfarjani , Harold T. Stokes

Knowledge of lattice anharmonicity is essential to elucidate distinctive thermal properties in crystalline solids. Yet, accurate \textit{ab initio} investigations of lattice anharmonicity encounter difficulties owing to the cumbersome…

材料科学 · 物理学 2022-04-13 Zhen Zhang , Dong-Bo Zhang , Tao Sun , Renata M. Wentzcovitch

The lattice dynamics of Cu3Au, Ni70Pt30, Pd90Fe10, and Pd96Fe04 intermetallic is studied using the DFT calculations. We calculated the phonon dispersions and phonon densities of states along two high symmetry paths of the Brillouin zone by…

材料科学 · 物理学 2020-08-24 Mina Aziziha , Saeed Akbarshahi
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