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We have observed geometrical frustration of quadrupolar and magnetic moments in dysprosium tetraboride, DyB4, where the rare-earth sites form a Shastry-Sutherland lattice. Resonant x-ray scattering at the LIII absorption edge of Dy was…

强关联电子 · 物理学 2009-11-11 Daisuke Okuyama , Takeshi Matsumura , Hironori Nakao , Youichi Murakami

DyB4 has a two-dimensional Shastry-Sutherland (Sh-S) lattice with strong Ising character of the Dy ions. Despite the intrinsic frustrations, surprisingly, it undergoes two successive transitions: a magnetic ordering at TN = 20K, and a…

The tetraboride HoB4 crystallizes in a tetragonal structure (space group P4/mbm), with the Ho atoms realizing a Shastry-Sutherland lattice. It orders antiferromagnetically at TN1 = 7.1 K and undergoes further magnetic transition at TN2 =…

A study of the tetragonal to orthorhombic phase transition of GdFeAsO is presented. Planes of the reciprocal space were reconstructed form single-crystal synchrotron X-ray diffraction data. By cooling below the structural transition…

超导电性 · 物理学 2015-06-11 F. Nitsche , Th. Doert , M. Ruck

Physical properties of DyB$_4$ have been studied by magnetization, specific heat, and ultrasonic measurements. The magnetic entropy change and the ultrasonic properties in the intermediate phase II indicate that the degeneracy of internal…

A diffraction experiment using a high energy x-ray was carried out on YbInCu4. Below the Yb valence transition temperature, the splitting of Bragg peaks was detected in higher-order reflections. No superlattice reflections accompanying the…

We present a comprehensive magnetic and structural phase diagram for $\mathrm{Y_{1-x}Lu_xBaCo_4O_7}$, established through neutron diffraction and magnetization measurements. Our results outline the evolution of various nuclear structures,…

强关联电子 · 物理学 2023-12-08 Sevda Sahinbay , Hong Zheng , John F. Mitchell , Stephan Rosenkranz , Omar Chmaissem

Neutron diffraction studies have been carried out in the temperature(T) range between 10 K and 130 K on a single crystal of YBaCo4O7, which has the stacking of kagome and triangular lattices of CoO4 tetrahedra along the c-axis. Structural…

强关联电子 · 物理学 2009-11-11 Minoru Soda , Yukio Yasui , Taketo Moyoshi , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

Resonant magnetic x-ray diffraction experiments on the Shastry-Sutherland lattice TbB$_4$ were carried out under strong pulsed magnetic fields up to 30 T. TbB$_4$ exhibits a multi-step magnetization process above 16 T when magnetic fields…

其他凝聚态物理 · 物理学 2008-08-21 T. Inami , K. Ohwada , Y. H. Matsuda , Z. W. Ouyang , H. Nojiri , D. Okuyama , T. Matsumura , Y. Murakami

Magnetic ordering in the geometrically frustrated magnetic oxide spinels MgCr_2O_4 and ZnCr_2O_4 is accompanied by a structural change that helps relieve the frustration. Analysis of high-resolution synchrotron X-ray scattering reveals that…

Cooperative Jahn-Teller ordering is well-known to drive the cubic $Fd\overline{3}m$ to tetragonal $I$4$_1$/$amd$ structural distortion in Mn$_3$O$_4$ at 1170 $^{\circ}$C. Further structural distortion occurs in Mn$_3$O$_4$ upon magnetic…

材料科学 · 物理学 2014-08-26 Moureen C. Kemei , Jaye K. Harada , Ram Seshadri , Matthew R. Suchomel

We have performed X-ray diffraction experiments on a single crystalline CeCoSi to investigate the unresolved ordered phase below $T_0 \sim 12$ K. We have discovered that a triclinic lattice distortion takes place below $T_0$, which is…

The classification of structural phase transitions as displacive or order-disorder in character is usually based on spectroscopic data above the transition. We use single crystal x-ray diffraction to investigate structural correlations in…

Possible order parameters of the phase IV in CexLa1-xB6 are discussed with special attention to the lattice distortion recently observed. A \Gamma_{5u}-type octupole order with finite wave number is proposed as the origin of the distortion…

强关联电子 · 物理学 2009-08-11 Katsunori Kubo , Yoshio Kuramoto

Resonant x-ray diffraction performed at the $\rm L_{II}$ and $\rm L_{III}$ absorption edges of Ru has been used to investigate the magnetic and orbital ordering in Ca$_2$RuO$_4$ single crystals. A large resonant enhancement due to electric…

The $4f$-electron system YbAl$_3$C$_3$ with a non-magnetic spin-dimer ground state has been studied by neutron diffraction in an applied magnetic field. A long-range magnetic order involving both ferromagnetic and antiferromagnetic…

For a high-quality single crystal of UPd_3 we present the relevant elastic constants and ultrasonic attenuation data. In addition to the magnetic phase transition at T_2=4.4 +/- 0.1K and the quadrupolar transition at T_1~6.8K, we find…

强关联电子 · 物理学 2009-10-31 N. Lingg , D. Maurer , V. Müller , K. A. McEwen

The quadrupolar ordering in CeB_6 is explained in terms of the electrostatic interaction of quadrupolar moments arranged into a simple cubic lattice. The representation of magnetic and quadrupolar moments by means of quasispins of two kinds…

统计力学 · 物理学 2009-10-30 Gennadi Uimin

An octupole ordering model is studied by the mean field theory, and its relevance to the phase IV of CexLa1-xB6 is discussed. The observed lattice distortion along the [111] direction is interpreted in terms of the \Gamma_{5g}-type…

强关联电子 · 物理学 2009-08-11 Katsunori Kubo , Yoshio Kuramoto

We report the temperature-dependent synchrotron based X-ray diffraction analysis of NASICON type Na$_3$FeCr(PO$_4$)$_3$ sample, which undergoes a symmetry-lowering structural transition from a monoclinic ($C2/c$) phase with long-range…

材料科学 · 物理学 2026-04-15 Madhav Sharma , Archna Sagdeo , Rajendra S. Dhaka
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