相关论文: Attosecond Control of Ionization Dynamics
Attosecond science, the electron control by the field of ultrashort laser pulses, is maturing into lightfield-driven electronics, called petahertz electronics. Based on optical field-driven nanostructures, elements for petahertz electronics…
The ionization of an atom by a high-frequency intense laser pulse, where the energy of a single-photon is sufficient to ionize the system, is investigated from first principles. It is shown that as a consequence of an AC Stark effect in the…
The generation of attosecond X-ray pulses has garnered significant attention within the X-ray free-electron laser (FEL) community due to their potential for ultrafast time-resolved studies. Such pulses enable the investigation of electron…
Recently we reported a series of numerical simulations proving that it is possible in principle to create an electronic wave packet and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few…
Temporal correlations in pulsed electron beams reflect the microscopic dynamics of emission and interparticle interaction. In femtosecond electron emission from nanoscale field emitters, Coulomb interactions result in structured…
The possibility of achieving highly selective excitation of low metastable states of hydrogen and helium atoms by using short laser pulses with reasonable parameters is demonstrated theoretically. Interactions of atoms with the laser field…
In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…
We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…
We propose utilizing a polarization-tailored high-power laser pulse to extract and accelerate electrons from the edge of a solid foil target to produce isolated attosecond electron bunches. The laser pulse consists of two…
Photoionization is a key step in many attosecond processes. Accurately determining the photoionization time delay is critical to understanding electron dynamics during and after ionization and can guide future efforts to manipulate electron…
The carrier envelop phase (CEP) of isolated attosecond pulses (IAPs) is theoretically and experimentally investigated based on the assumption that a significant contribution originates from the measurable CEP jitter of the driving laser. By…
Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…
Recent attoclock experiments and theoretical studies regarding the strong-field ionization of atoms by few-cycle infrared pulses revealed new features that have attracted much attention. Here we investigate tunneling ionization and the…
The absorption of traveling photons resonant with electric dipole transitions of an atomic gas naturally leads to electric dipole spin wave excitations. For a number of applications, it would be highly desirable to shape and coherently…
Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…
Tunneling plays a central role in the interaction of matter with intense laser pulses, and also in time-resolved measurements on the attosecond timescale. A strong laser field influences the binding potential of an electron in an atom so…
An intuitive physical mechanism for single attosecond pulse generation in multi-cycle pulse regime is proposed. We suggest that the continuum spectra of HHG can be controlled through the modulation of carrier wave, while keeping the…
We numerically investigate the use of strong THz radiation in assisting single attosecond pulse generation by few-cycle, 800 nm laser pulses. We optimize focusing conditions to generate short and powerful single attosecond pulses of…
Electronic correlations occur on attosecond timescales, dictating how chemical bonds form, energy flows, and materials respond to light. Capturing such many-body processes requires light pulses of similar duration. The soft X-ray water…
We report on new routes to generating a train of attosecond pulses. The methods are extremely simple and robust; we need to place only a few thin dispersive materials in the optical path. We numerically demonstrate the generation of a train…