相关论文: Enhancing single-molecule photostability by optica…
Magneto photoluminescence and excitation spectroscopy are used to probe the excited state spectrum of negatively charged trions in a InGaAs quantum dot. A single dot optical charging device allows us to selectively prepare specific few (1e,…
Controlling electrically-stimulated quantum light sources (QLS) is key for developing integrated and low-scale quantum devices. The mechanisms leading to quantum emission are complex, as a large number of electronic states of the system…
All optical detectors to date annihilate photons upon detection, thus excluding repeated measurements. Here, we demonstrate a robust photon detection scheme which does not rely on absorption. Instead, an incoming photon is reflected off an…
Efficient quantum-state detection is crucial for many precision control experiments, such as the ongoing effort to probe the electron's electric dipole moment using trapped molecular $^{232}\mathrm{ThF}^+$ ions at JILA. While quantum state…
Optical quantum information processing critically relies on Bell-state measurement, a ubiquitous operation for quantum communication and computing. Its practical realization involves the interference of optical modes and the detection of a…
We optically probe the spectrum of ground and excited state transitions of an individual, electrically tunable self-assembled quantum dot molecule. Photocurrent absorption measurements show that the spatially direct neutral exciton…
Ultracold ground-state molecules can be formed from ultracold atoms via photoassociation followed by a spontaneous emission process. Typically, the molecular products are distributed over a range of final states. Here, we propose to use an…
We explore the photon statistics of light emitted from a system comprising a single four--level atom strongly coupled to a high-finesse optical cavity mode which is driven by a coherent laser field. In the weak driving regime this system is…
A reliable photon source is required for many aspects of quantum technology. Organic molecules are attractive for this application because they can have high quantum yield and can be photostable, even at room temperature. To generate a…
Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…
The detection of single molecules has facilitated many advances in life- and material-sciences. Commonly, it founds on the fluorescence detection of single molecules, which are for example attached to the structures under study. For…
Tip-enhanced photoluminescence (TEPL) measurements are performed with sub-nanometer spatial resolution on individual molecules decoupled from a metallic substrate by a thin NaCl layer. TEPL spectra reveal progressive fluorescence quenching…
In the quantum sensing context most of the efforts to design novel quantum techniques of sensing have been constrained to idealized, noise-free scenarios, in which effects of environmental disturbances could be neglected. In this work, we…
Singlet fission, the molecular process through which photons are effectively converted into pairs of lower energy triplet excitons, holds promise as a means of boosting photovoltaic device efficiencies. In the preceding article of this…
Optical detection and spectroscopy of single molecules has become an indispensable tool in biological imaging and sensing. Its success is based on fluorescence of organic dye molecules under carefully engineered laser illumination. In this…
Electron transfer to an individual quantum dot promotes the formation of charged excitons with enhanced recombination pathways and reduced lifetimes. Excitons with only one or two extra charges have been observed and exploited for very…
The energetic positions of molecular electronic states at molecule/electrode interfaces are crucial factors for determining the transport and optoelectronic properties of molecular junctions. Strong light--matter coupling offers a potential…
The photon upconversion based on sensitized triplet-triplet annihilation (sTTA-UC) is a spin-flip mechanism exploited to recover the energy of dark triplet states in conjugated systems. In this process a high-energy fluorescent singlet is…
By using a quantized input light, we theoretically revisit the coherent two-color photo-association process in an atomic Bose-Einstein condensate. Under the single-mode approximations, we show two interesting regimes of the light…
We predict a bistability in the photon emission from a solid-state single-atom laser comprising a microwave cavity coupled to a voltage-biased double quantum dot. To demonstrate that the single-atom laser is bistable, we evaluate the photon…