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The solid solution Ga1-xGexV4S8 (x = 0 - 1) was synthesized by solid state reactions and characterized by temperature-dependent x-ray powder diffraction and static magnetic susceptibility measurements. The compounds crystallize in the cubic…

强关联电子 · 物理学 2009-06-09 Daniel Bichler , Herta Slavik , Dirk Johrendt

In addition to its promising potential for applications, GaV4S8 shows very interesting physical properties with temperature and magnetic field. These properties can be tuned by applying hydrostatic pressure in order to reveal and understand…

The lacunar spinel GeV4S8 undergoes orbital and ferroelectric ordering at the Jahn-Teller transition around 30 K and exhibits antiferromagnetic order below about 14 K. In addition to this orbitally driven ferroelectricity, lacunar spinels…

强关联电子 · 物理学 2017-01-23 S. Widmann , A. Günther , E. Ruff , V. Tsurkan , H. -A. Krug von Nidda , P. Lunkenheimer , A. Loidl

We report resistivity, thermopower and magnetic susceptibility measurements on the Nb$_4$-cluster compounds Ga$_{1.33}$Nb$_4$X$_{8}$ (X = S, Se), derived from vacancy ordered spinels A$_x$T$_4$X$_8$. The cubic selenide phase is insulating…

强关联电子 · 物理学 2007-05-23 Asad Niazi , A. K. Rastogi

We present dielectric, polarization, resistivity, specific heat, and magnetic susceptibility data on single crystals of the lacunar spinels GaNb4Se8 and GaTa4Se8, tetrahedral cluster-based materials with substantial spin-orbit coupling. We…

强关联电子 · 物理学 2022-12-19 M. Winkler , L. Prodan , V. Tsurkan , P. Lunkenheimer , I. Kézsmárki

In the present work, we provide results from specific heat, magnetic susceptibility, dielectric constant, ac conductivity, and electrical polarization measurements performed on the lacunar spinel GaV4Se8. With decreasing temperature, we…

强关联电子 · 物理学 2017-10-18 E. Ruff , A. Butykai , K. Geirhos , S. Widmann , V. Tsurkan , E. Stefanet , I. Kézsmárki , A. Loidl , P. Lunkenheimer

A detailed study of poly- and single crystalline samples of the normal spinel HgCr2S4 is reported. The structural refinement reveals enhanced values of the atomic displacements suggesting closeness to a structural instability.…

We report on THz time-domain spectroscopy on multiferroic GeV4S8, which undergoes orbital ordering at a Jahn-Teller transition at 30.5 K and exhibits antiferromagnetic order below 14.6 K. The THz experiments are complemented by dielectric…

强关联电子 · 物理学 2017-10-25 S. Reschke , Zhe Wang , F. Mayr , E. Ruff , P. Lunkenheimer , V. Tsurkan , A. Loidl

The lacunar spinel GaV4S8 exhibits orbital ordering at 44 K and shows a complex magnetic phase diagram below 12.7 K, which includes ferromagnetic and cycloidal spin order. At low but finite external magnetic fields, N\'eel-type skyrmions…

We report the synthesis, structure, and magnetic and transport properties of a new ternary intermetallic compound PrRhSn3 which crystallizes in LaRuSn3-type cubic structure (space group Pm-3n). At low applied fields the dc magnetic…

强关联电子 · 物理学 2014-07-22 V. K. Anand , D. T. Adroja , A. D. Hillier

We have carried out neutron diffraction and small angle neutron scattering measurements on a high quality single crystal of the cubic lacunar spinel multiferroic, GaV$_4$S$_8$, as a function of magnetic field and temperature to determine…

Electronic conduction in GaM$_{4}$Se$_{8}$ (M=Nb;Ta) compounds with the fcc GaMo$_{4}$S$_{8}$-type structure originates from hopping of localized unpaired electrons (S=1/2) among widely separated tetrahedral M$_{4}$ metal clusters. We show…

超导电性 · 物理学 2009-11-11 M. M. Abd-Elmeguid , B. Ni , D. I. Khomskii , R. Pocha , D. Johrendt , X. Wang , K. Syassen

We report temperature (T) dependence of dc magnetization, electrical resistivity (rho(T)), and heat-capacity of rare-earth (R) compounds, Gd3RuSn6 and Tb3RuSn6, which are found to crystallize in the Yb3CoSn6-type orthorhombic structure…

强关联电子 · 物理学 2017-06-28 Sanjay K Upadhyay , Kartik K Iyer , E. V. Sampathkumaran

We apply the finite-temperature variational cluster approach to a strongly correlated and spin-orbit coupled model for four electrons (i.e. two holes) in the $t_{2g}$ subshell. We focus on parameters suitable for antiferromagnetic Mott…

强关联电子 · 物理学 2021-07-21 Jan Lotze , Maria Daghofer

Motivated by recent studies of the cluster Mott insulator candidate compound Nb3Cl8, this study performs 93Nb and 35Cl nuclear magnetic resonance (NMR) measurements to investigate the electron correlations. Below the structural transition…

强关联电子 · 物理学 2025-03-18 Y. Z. Zhou , X. Han , J. Luo , D. T. Wu , A. F. Fang , B. Shen , B. J. Feng , Y. G. Shi , J. Yang , R. Zhou

LV4O8 (L = Yb, Y, Lu) compounds are reported to crystallize in a structure similar to that of the orthorhombic CaFe2O4 structure-type, and contain four inequivalent V sites arranged in zigzag chains. We confirm the structure and report the…

强关联电子 · 物理学 2010-11-17 S. Das , A. Niazi , Y. Mudryk , V. K. Pecharsky , D. C. Johnston

We report on optical spectroscopy on the lacunar spinels GaV$_4$S$_8$ and GeV$_4$S$_8$ in the spectral range from 100 to 23000 cm$^{-1}$ and for temperatures from 5 to 300 K. These multiferroic spinel systems reveal Jahn-Teller driven…

强关联电子 · 物理学 2017-10-06 S. Reschke , F. Mayr , Zhe Wang , P. Lunkenheimer , W. Li , D. Szaller , S. Bordács , I. Kézsmárki , V. Tsurkan , A. Loidl

We report on the low-temperature physical properties of a novel compound Ce$_{11}$Pd$_4$In$_9$ that crystallizes with the orthorhombic Nd$_{11}$Pd$_4$In$_9$-type crystal structure (space group $Cmmm$). The compound exhibits ferromagnetic…

强关联电子 · 物理学 2019-01-23 Debarchan Das , Dariusz Kaczorowski

We present an investigation of the multiferroic lacunar spinel compound GeV$_4$S$_8$ using time-domain terahertz spectroscopy. We find three absorptions which either appear or shift at the antiferromagnetic transition temperature, T$_N =…

强关联电子 · 物理学 2017-08-30 Matthew T. Warren , G. Pokharel , A. D. Christianson , D. Mandrus , R. Valdés Aguilar

Electrical conductivity, thermopower and magnetic properties of Fe-intercalated Fe0.33VSe2 has been reported between 4.2K - 300K. We observe a first order transition in the resistivity of the sintered pellets around 160K on cooling. The…

材料科学 · 物理学 2009-11-13 C. S. Yadav , A. K. Rastogi
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